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A theoretical model for high-order harmonic generation (HHG) in bulk solids is considered. Our approach treats laser-induced inter- and intraband currents on an equal footing. The sum of these currents is the source of the high-order…

量子物理 · 物理学 2017-07-12 Peter Foldi

Recent studies have demonstrated that the polarization states of high harmonics from solids can differ from those of the driving pulses. To gain insights on the microscopic origin of this behavior, we perform one-particle intraband-only…

We consider several aspects of high-order harmonic generation in solids: the effects of elastic and inelastic scattering; varying pulse characteristics; and inclusion of material-specific parameters through a realistic band structure. We…

其他凝聚态物理 · 物理学 2013-02-07 A. F. Kemper , B. Moritz , J. K. Freericks , T. P. Devereaux

The generation of high-order harmonics in bulk solids subjected to intense ultrashort laser pulses has opened up new avenues for research in extreme nonlinear optics and light-matter interaction on sub-cycle timescales. Despite significant…

High-harmonic generation by a laser-driven solid slab is simulated using time-dependent density functional theory. Multiple harmonic plateaus up to very high harmonic orders are observed already at surprisingly low field strengths. The full…

原子物理 · 物理学 2017-11-29 Kenneth K. Hansen , Tobias Deffge , Dieter Bauer

In frequently studied two-band models for solid-state high-harmonic generation, interband harmonics in principle can range from the minimum to the maximum bandgap. However, it is known that a laser-intensity dependent cutoff exists that may…

光学 · 物理学 2024-03-13 Lina Bielke , Hannah Jürß , Vincent Burgtorf , Dieter Bauer

Kerr-type nonlinearities form the basis for our physical understanding of nonlinear optical phenomena in condensed matter, such as self-focusing, solitary waves, and wave mixing. In strong fields, they are complemented by higher-order…

We investigate high-order harmonic generation in inhomogeneous media for reduced dimensionality models. We perform a phase-space analysis, in which we identify specific features caused by the field inhomogeneity. We compute high-order…

原子物理 · 物理学 2016-05-25 C. Zagoya , M. Bonner , H. Chomet , E. Slade , C. Figueira de Morisson Faria

We studied the high-harmonic generation by the interaction of sub-cycle laser pulses with the He atom. The sub-cycle pulses are modeled using the complex source vector beam model, which is an exact solution to Maxwell's equations and…

光学 · 物理学 2023-02-08 Amol R. Holkundkar , Rambabu Rajpoot , Jayendra N. Bandyopadhyay

The strong ellipticity dependence of high-harmonic generation in gases enables numerous experimental techniques that are nowadays routinely used, for instance, to create isolated attosecond pulses. Extending such techniques to high-harmonic…

We investigate high-order harmonic generation (HHG) in graphene with a quantum master equation approach. The simulations reproduce the observed enhancement in HHG in graphene under elliptically polarized light [N. Yoshikawa et al, Science…

材料科学 · 物理学 2021-02-03 Shunsuke A. Sato , Hideki Hirori , Yasuyuki Sanari , Yoshihiko Kanemitsu , Angel Rubio

Motivated by the emerging experiments [e.g. \textit{Z. Nie et al. Nat. Photon. \textbf{12}, 489 (2018)}] on producing infrared (IR) single cycle pulses in the spectral region 5 - 14 $\mu m$, we theoretically investigate their role for…

原子物理 · 物理学 2020-12-01 Abdelmalek Taoutioui , Hicham Agueny

An interesting property of high harmonic generation in solids is its laser polarization dependent nature which in turn provides information about the crystal and band structure of the generation medium. Here we report on the linear…

One key parameter in the high-order harmonic generation (HHG) phenomenon is the exact frequency of the generated harmonic field. Its deviation from perfect harmonics of the laser frequency can be explained considering (i) the single-atom…

We generate high-order harmonics of a mid-infrared laser from a silicon single crystal and find their origin in the recollision of coherently accelerated electrons with their holes, analogously to the atomic and molecular case, and to ZnO…

We experimentally observe longer than long trajectory influence in high order harmonic generation (HHG) by varying the peak intensity of the driving laser field through either direct attenuation, or by chirping the laser pulse. Using a…

光学 · 物理学 2022-12-12 S. Bengtsson , E. R. Simpson , N. Ibrakovic , S. Ek , A. Olofsson , T. Causer , J. Mauritsson

We consider a quantum mechanical model for the high-order harmonic generation in bulk solids. The bandgap is assumed to be considerably larger than the exciting photon energy. Using dipole approximation, the dynamical equations for…

量子物理 · 物理学 2017-11-09 Viktor Szaszkó-Bogár , Katalin Varjú , Péter Földi

We demonstrated nonperturbative high harmonics induced by intense mid-infrared light up to 18th order that well exceed the material bandgap in monolayer transition metal dichalcogenides. The intensities of the even-order high-harmonic…

介观与纳米尺度物理 · 物理学 2019-08-20 Naotaka Yoshikawa , Kohei Nagai , Kento Uchida , Yuhei Takaguchi , Shogo Sasaki , Yasumitsu Miyata , Koichiro Tanaka

The generation of high harmonics in laser-irradiated light homonuclear diatomics (H2+, N2 and O2) compared to that in atomic counterparts (of nearly identical binding energy) is studied within the velocity gauge version of conventional…

原子物理 · 物理学 2009-11-11 Vladimir I. Usachenko , Pavel E. Pyak , Shih-I Chu

We analytically and numerically investigate the emission of high-harmonic radiation from model solids by intense few-cycle mid-infrared laser pulses. In single-active-electron approximation, we expand the active electron's wavefunction in a…

其他凝聚态物理 · 物理学 2019-07-26 Francisco Navarrete , Marcelo F. Ciappina , Uwe Thumm
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