相关论文: Probing molecules in gas cells of subwavelength th…
We investigate theoretically dark resonance spectroscopy for a dilute atomic vapor confined in a thin (micro-metric) cell. We identify the physical parameters characterizing the spectra and study their influence. We focus on a Hanle-type…
The high sensitivity of Laser Spectroscopy has made possible the exploration of atomic resonances in newly designed "nanometric" gas cells, whose local thickness varies from 20nm to more than 1000 nm. Following the initial observation of…
A nanometer-thin-cell (in the direction of laser beam propagation) has been elaborated with the thickness of the atomic vapor column varying smoothly in the range of $L = \unit[50-1500]{nm}$. The cell allows one to study the behavior of the…
We report on precision spectroscopy of sub-wavelength confined molecular gases. This was obtained by rovibrational selective reflection of $\mathrm{NH_3}$ and $\mathrm{SF_6}$ gases using a quantum cascade laser at $\lambda\approx 10.6 \mu…
We use an atomic vapor cell as a frequency tunable microwave field detector operating at frequencies from GHz to tens of GHz. We detect microwave magnetic fields from 2.3 GHz to 26.4 GHz, and measure the amplitude of the sigma+ component of…
Weak measurement (WM) with state pre- and post-selection can amplify otherwise undetectable small signals and thus promise great potentials in precision measurements. Although frequency measurements offer the hitherto highest precision…
We demonstrate continuous-frequency electric field measurements of high-intensity microwaves via optical spectroscopy in a small atomic vapor cell. The spectroscopic response of a room-temperature rubidium atomic vapor in a glass cell is…
Rescattering electrons offer great potential as probes of molecular properties on ultrafast timescales. The most famous example is molecular tomography, in which high harmonic spectra of oriented molecules are mapped to ``tomographic…
In recent years, micromachined vapor cells have been revolutionizing the field of chip-scale quantum sensors such as magnetometers and atomic clocks. In parallel, Rydberg atomic quantum sensing has emerged as a powerful technique for…
We have carried out theoretical research on ultra-high resolution spectroscopy of atoms (or molecules) in the suggested cell with a series of plane-parallel thin gas layers between spatially separated gas regions of this cell for optical…
The principle of coherent Dicke narrowing in a thin vapour cell, in which sub-Doppler spectral lineshapes are observed under a normal irradiation for a l/2 thickness, is generalized to two-photon spectroscopy. Only the sum of the two wave…
We present a comprehensive numerical investigation into the radio frequency (RF) field behavior within miniaturized all-glass and hybrid vapor cell geometries designed for Rydberg atom-based electrometry. Using full-vector finite element…
Micro-Electro-Mechanical, so called 'MEMs,' vapor cells are a key component in atom-based quantum sensors, such as clocks, gyroscopes, electric field sensors and magnetometers. MEMs vapor cell fabrication for Rydberg atom radio frequency…
Molecular vibrations and their dynamics are of outstanding importance for electronic and thermal transport in nanoscale devices as well as for molecular catalysis. The vibrational dynamics of <100 molecules are studied through three-colour…
We exploit millimeter wave technology to measure the reflection and transmission response of random dielectric media. Our samples are easily constructed from random stacks of identical, sub-wavelength quartz and Teflon wafers. The…
Rydberg-atom electrometry, as an emerging cutting-edge technology, features high sensitivity, broad bandwidth, calibration-free operation, and beyond. However, until now the key atomic vapor cells used for confining electric field-sensitive…
We have investigated electromagnetically induced transparency in the spectrum of selective reflection at the interface of Rb atom vapors and a dielectric nanocell window. A nanocell with atomic vapor column thicknesses ranging from 150 to…
This communication focuses on sensitivity issues - a long-time concern of J. Hall- in the spectroscopic analysis of Extremely Thin Cell of dilute vapor. With these small and often submicrometric slices of vapor, the most uncommon features…
Matter-wave interferometry with molecules is intriguing both because it demonstrates a fundamental quantum phenomenon and because it opens avenues to quantum-enhanced measurements in physical chemistry. One great challenge in such…
A scanning tunneling microscope is used to generate the electroluminescence of phthalocyanine molecules deposited on NaCl/Ag(111). Photon spectra reveal an intense emission line at 1.9 eV that corresponds to the fluorescence of the…