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Recently, we have demonstrated a method to record the longitudinal phase-space distribution of a pulsed cryogenic buffer gas cooled beam of barium fluoride molecules. In this paper, we use this method to determine the influence of various…

We present a comprehensive characterization of cold molecular beams from a cryogenic buffer-gas cell, providing an insight into the physics of buffer-gas cooling. Cold molecular beams are extracted from a cryogenic cell by electrostatic…

化学物理 · 物理学 2018-12-04 X. Wu , T. Gantner , M. Zeppenfeld , S. Chervenkov , G. Rempe

A novel two-stage helium buffer gas cooled beam source is introduced. The properties of the molecular beams produced from this source are investigated theoretically using the CaF as a test molecule. The gas-phase molecules are first…

原子物理 · 物理学 2020-04-14 Vijay Singh

We study the properties of a cryogenic buffer gas source that uses a low temperature two-stage buffer gas cell to produce very slow beams of ytterbium monofluoride molecules. The molecules are produced by laser ablation inside the cell and…

原子物理 · 物理学 2024-11-19 A. D. White , S. Popa , J. Mellado-Munoz , N. J. Fitch , B. E. Sauer , J. Lim , M. R. Tarbutt

An electrostatic hexapole lens is used to manipulate the transverse properties of a beam of barium fluoride molecules from a cryogenic buffer gas source. The spatial distribution of the beam is measured by recording state-selective…

Using frequency-chirped radiation pressure slowing, we precisely control the velocity of a pulsed CaF molecular beam down to a few m/s, compressing its velocity spread by a factor of 10 while retaining high intensity: at a velocity of…

原子物理 · 物理学 2017-04-05 S. Truppe , H. J. Williams , N. J. Fitch , M. Hambach , T. E. Wall , E. A. Hinds , B. E. Sauer , M. R. Tarbutt

We present the results of experiments performed on cold caesium in a pulsed sinusoidal optical potential created by counter-propagating laser beams having a small frequency difference in the laboratory frame. Since the atoms, which have…

量子物理 · 物理学 2009-11-10 P. H. Jones , M. Goonasekera , H. E. Saunders-Singer , D. R. Meacher

In this paper we report on the production and characterization of a cold beam of BaOH molecules using a cryogenic buffer-gas beam source. BaOH is a highly suitable molecule for studies of the violation of fundamental symmetries, such as the…

Cryogenic buffer-gas beams are a promising method for producing bright sources of cold molecular radicals for cold collision and chemical reaction experiments. In order to use these beams in studies of reactions with controlled collision…

化学物理 · 物理学 2015-06-18 M. I. Fabrikant , Tian Li , N. J. Fitch , N. Farrow , Jonathan D. Weinstein , H. J. Lewandowski

Employing a two-stage cryogenic buffer gas cell, we produce a cold, hydrodynamically extracted beam of calcium monohydride molecules with a near effusive velocity distribution. Beam dynamics, thermalization and slowing are studied using…

原子物理 · 物理学 2017-09-13 Hsin-I Lu , Julia Rasmussen , Matthew J. Wright , Dave Patterson , John M. Doyle

Barium monohydride (BaH) is an attractive candidate for extending laser cooling and trapping techniques to diatomic hydrides. The apparatus and high-resolution optical spectroscopy presented here demonstrate progress toward this goal. A…

原子物理 · 物理学 2017-08-08 G. Z. Iwata , R. L. McNally , T. Zelevinsky

We show that, in strongly chaotic dynamical systems, the average particle velocity can be calculated analytically by consideration of Brownian dynamics in phase space, the method of images and use of the classical diffusion equation. The…

统计力学 · 物理学 2020-01-29 Matheus S. Palmero , Gabriel I. Díaz , Peter V. E. McClintock , Edson D. Leonel

The use of structured light beams to detect the velocity of targets moving perpendicularly to the beam's propagation axis opens new avenues for remote sensing of moving objects. However, determining the direction of motion is still a…

Adaptive physics-informed super-resolution diffusion is developed for non-invasive virtual diagnostics of the 6D phase space density of charged particle beams. An adaptive variational autoencoder (VAE) embeds initial beam condition images…

机器学习 · 计算机科学 2025-01-14 Alexander Scheinker

This work presents an experimental protocol conceived to determine the vibrational distribution of barium monofluoride molecules seeded in a supersonic beam of argon. Here, as in many cases, the detection signal is related to the number of…

原子物理 · 物理学 2020-10-05 T. Courageux , A. Cournol , D. Comparat , B. Viaris de Lesegno , H. Lignier

In ultrafast experiments with gas phase molecules, the alignment of the molecular axis relative to the polarization of the interacting laser pulses plays a crucial role in determining the dynamics following this light-matter interaction.…

化学物理 · 物理学 2025-04-14 Shashank Kumar , Eric Liu , Liang Z. Tan , Varun Makhija , Niranjan Shivaram

Characterization and control of the transverse phase space of high-brightness electron beams is required at free-electron lasers or electron diffraction experiments for emittance measurement and beam optimization as well as at advanced…

Stark deceleration allows for precise control over the velocity of a pulsed molecular beam and, by the nature of its limited phase-space acceptance, reduces the energy width of the decelerated packet. We describe an alternate method of…

原子物理 · 物理学 2015-05-13 L. P. Parazzoli , N. Fitch , D. S. Lobser , H. J. Lewandowski

Advanced accelerator-based light sources such as free electron lasers (FEL) accelerate highly relativistic electron beams to generate incredibly short (10s of femtoseconds) coherent flashes of light for dynamic imaging, whose brightness…

加速器物理 · 物理学 2024-07-19 Alexander Scheinker

A cryogenic neon solid doped with barium monofluoride (BaF) is created on a cryogenic substrate using a stream of Ne gas and a high-intensity beam of BaF molecules produced in a cryogenic helium-buffer-gas laser-ablation source. The…

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