相关论文: The role of anharmonicity in single-molecule spin-…

Spin-crossover (SCO) molecules are versatile magnetic switches with applications in molecular electronics and spintronics. Downscaling devices to the single-molecule level remains, however, a challenging task since the switching mechanism…

We investigate the microscopic mechanism of quantum energy transfer in the nonequilibrium spin-boson model. By developing a nonequilibrium polaron-transformed Redfield equation based on fluctuation decoupling, we dissect the energy transfer…

We present a novel approximation scheme to describe the influence of a harmonic bath on the dynamics of a two-level particle over almost the whole regime of temperatures and coupling to the environment, for a wide class of bath spectral…

We discuss how the crossovers in models like spin-boson model are changed by adding the coupling of the central spin to localised modes- the latter modelled as a 'spin bath'. These modes contain most of the environmental entropy and energy…

The spin-boson (SB) model is a standard prototype for quantum dissipation, which we generalize in this work, to explore the dissipative effects on a one-dimensional spin-orbit (SO) coupled particle in the presence of a sub-ohmic bath. We…

As a step towards a more realistic modeling of vibrations in single-molecule devices, we investigate the effects of charge-dependent vibrational frequencies and anharmonic potentials on electronic transport. For weak phonon relaxation, we…

We study the decoherence of a spin in a quantum dot due to its hyperfine coupling to a randomly fluctuating bath of nuclear spins. The system is modelled by the central spin model with the spin bath initially being at infinite temperature.…

We use the "generalized hierarchical equation of motion" proposed in Paper I to study decoherence in a system coupled to a spin bath. The present methodology allows a systematic incorporation of higher order anharmonic effects of the bath…

Spin noise spectroscopy (SNS) has become a mainstream approach to probe the dynamics of a spin ensemble in and out of equilibrium. Current models describing spin noise in interacting samples are based on an effective single particle…

The spin-boson model, describing a two-level system coupled to a bath of harmonic oscillators, is a generic model for quantum dissipation, with manifold applications. It has also been studied as a simple example for an impurity quantum…

The key feature of a quantum spin coupled to a harmonic bath---a model dissipative quantum system---is competition between oscillator potential energy and spin tunneling rate. We show that these opposing tendencies cause environmental…

Dynamics of the (sub-)Ohmic spin-boson model under various bath initial conditions is investigated by employing the Dirac-Frenkel time-dependent variational approach with the multiple Davydov $\mathrm{D_1}$ ansatz in the interaction…

We discuss the dynamics of a spin coupled to a damped harmonic oscillator. This system can be mapped to a spin-boson model with a structured bath, i.e. the spectral function of the bath has a resonance peak. We diagonalize the model by…

In a recent Letter, Guarnieri et al. [1] reported on the possibility of generating steady-state coherence (SSC) in the energy basis of a two-level system by the sole action of a single thermal bath also for weak system-bath coupling and due…

We investigate the dynamics of a large anisotropic spin whose easy-axis component is coupled to a bosonic bath with a spectral function $J(\w)\propto \omega^s$. Such a spin complex might be realized in a single-molecular magnet. Using the…

The influence of dissipation on quantum tunneling in the spin-boson model with a sub-Ohmic bath is studied by a variational calculation. By examining the evolution of solutions of the variational equation with the coupling strength near the…

In this work, we performed extensive first-principles simulations of high-harmonic generation in the topological Diract semimetal Na3Bi using a time-dependent density functional theory framework, focusing on the effect of spin-orbit…

Anharmonic lattice vibrations play a key role in many physical phenomena. They govern the heat conductivity of solids, strongly affect the phonon spectra, play a prominent role in soft mode phase transitions, allow ultrafast engineering of…

Rectification of heat transfer in nanodevices can be realized by combining the system inherent anharmonicity with structural asymmetry. we analyze this phenomenon within the simplest anharmonic system -a spin-boson nanojunction model. We…

We develop a quantum mechanical formalism to treat the strong coupling between an electromagnetic mode and a vibrational excitation of an ensemble of organic molecules. By employing a Bloch-Redfield-Wangsness approach, we show that the…