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We report on a nuclear magnetic resonance (NMR) study of ultrananocrystalline diamond (UNCD) materials produced by detonation technique. Analysis of the 13C and 1H NMR spectra, spin-spin and spin-lattice relaxation times in purified UNCD…

材料科学 · 物理学 2009-11-13 A. M. Panich , A. I. Shames , H. -M. Vieth , E. Osawa , M. Takahashi , A. Ya. Vul

Nuclear magnetic resonance spectroscopy with solid-state spin sensors is a promising pathway for the detection of nuclear spins at the micro- and nanoscale. Although many nanoscale experiments rely on a single sensor spin for the detection…

Scattering of protons of several hundred MeV is a promising new spectroscopic tool for the study of electric dipole strength in nuclei. A case study of 208Pb shows that at very forward angles J^pi = 1- states are strongly populated via…

We present a scheme of positioning a single electron spin with sub-nanometer resolution through multiple nitrogen-vacancy centers in diamond. With unwanted noise suppressed by dynamical decoupling, the spin coherence of each center develops…

量子物理 · 物理学 2016-04-27 Wen-Long Ma , Shu-Shen Li , Geng-Yu Cao , Ren-Bao Liu

Dynamic nuclear polarization (DNP) is used in nuclear magnetic resonance (NMR) to transfer polarization from electron spins to nuclear spins. The resulting nuclear polarization enhancement can, in theory, be two or three orders of magnitude…

量子物理 · 物理学 2015-10-14 Sarah Sheldon , David G. Cory

Lead-vacancy (PbV) centers in diamond with a large ground state splitting are expected to be a building block of quantum network nodes. Due to the heaviness of the Pb atom, it is challenging to fabricate high-quality PbV centers with a…

Pulsed ESR experiments are reported for ensembles of negatively-charged nitrogen-vacancy centers (NV$^-$) in diamonds at X-band magnetic fields (280-400 mT) and low temperatures (2-70 K). The NV$^-$ centers in synthetic type IIb diamonds…

量子物理 · 物理学 2016-12-22 B. C. Rose , C. D. Weis , A. M. Tyryshkin , T. Schenkel , S. A. Lyon

Inelastic proton scattering under extreme forward angles including $0^\circ$ and at energies of a few hundred MeV has been established as a new spectroscopic tool for the study of complete dipole strength distributions in nuclei. Such data…

核实验 · 物理学 2020-05-11 Peter von Neumann-Cosel , Atsushi Tamii

The ST1 center is a point defect in diamond with bright fluorescence and a mechanism for optical spin initialization and readout. The center has impressive potential for applications in diamond quantum computing as a quantum bus to a…

Ensembles of nitrogen-vacancy (NV) centers in diamond are versatile quantum sensors with broad applications in the physical and life sciences. The concentration of neutral substitutional nitrogen ([N$_\text{s}^0$]) strongly influences…

Dynamic Nuclear Polarization (DNP) has revolutionized the field of solid-state NMR spectroscopy by significantly enhancing the sensitivity of nuclear magnetic resonance experiments. Conventionally, cross effect DNP relies on biradicals to…

化学物理 · 物理学 2023-09-28 Amaria Javed , Asif Equbal

Dynamic nuclear polarization (DNP) is an out-of-equilibrium method for generating non-thermal spin polarization which provides large signal enhancements in modern diagnostic methods based on nuclear magnetic resonance. A particular instance…

其他凝聚态物理 · 物理学 2018-04-04 Alexander Karabanov , Daniel Wiśniewski , Federica Raimondi , Igor Lesanovsky , Walter Köckenberger

Initializing quantum registers with high fidelity is a fundamental precondition for many applications like quantum information processing and sensing. The electronic and nuclear spins of a Nitrogen-Vacancy (NV) center in diamond form an…

量子物理 · 物理学 2020-04-06 K. Rama Koteswara Rao , Yihua Wang , Zingfu Zhang , Dieter Suter

Nitrogen vacancy (NV) centers in diamond have emerged as a leading quantum sensor platform, combining exceptional sensitivity with nanoscale spatial resolution by optically detected magnetic resonance (ODMR). Because fluorescence-based ODMR…

量子物理 · 物理学 2020-11-24 Laura Kim , Hyeongrak Choi , Matthew Trusheim , Dirk Englund

We determine the polarization of the bulk $^{13}$C nuclear spin system in diamond produced by interaction with optically oriented nitrogen-vacancy (NV-) defect centers. $^{13}$C nuclei are polarized into the higher energy Zeeman state with…

其他凝聚态物理 · 物理学 2015-05-14 Jonathan P. King , Patrick J. Coles , Jeffrey A. Reimer

Different approaches have improved the sensitivity of either electron or nuclear magnetic resonance to the single spin level. For optical detection it has essentially become routine to observe a single electron spin or nuclear spin.…

介观与纳米尺度物理 · 物理学 2016-06-29 Jörg Wrachtrup , Amit Finkler

We demonstrate nuclear magnetic resonance (NMR) spectroscopy of picoliter-volume solutions with a nanostructured diamond chip. Using optical interferometric lithography, diamond surfaces were nanostructured with dense, high-aspect-ratio…

介观与纳米尺度物理 · 物理学 2017-11-01 P. Kehayias , A. Jarmola , N. Mosavian , I. Fescenko , F. M. Benito , A. Laraoui , J. Smits , L. Bougas , D. Budker , A. Neumann , S. R. J. Brueck , V. M. Acosta

We use nominally forbidden electron-nuclear spin transitions in nitrogen-vacancy (NV) centers in diamond to demonstrate coherent manipulation of a nuclear spin ensemble using microwave fields at room temperature. We show that employing an…

量子物理 · 物理学 2021-04-21 P. Huillery , J. Leibold , T. Delord , L. Nicolas , J. Achard , A. Tallaire , G. Hétet

We created dense ensembles of negatively charged nitrogen-vacancy (NV-) centers in diamond by neutron and electron irradiation for applications in hybrid quantum systems and magnetometry. We characterize fluorescence intensity, optical and…

Identifying weakly coupled nuclear spins around single electron spins is a key step of implementing quantum information processing using coupled electron-nuclei spin systems or sensing like single spin nuclear magnetic resonance detection…

介观与纳米尺度物理 · 物理学 2015-01-08 Nan Zhao , Jörg Wrachtrup , Ren-Bao Liu