相关论文: Pump Pulse Bandwidth-Activated Nonlinear Phononic …
The anharmonic response of charge-density wave (CDW) order to strong laser-pulse perturbations in 1T-TaS_2 and TbTe_3 is investigated by means of a multiple-pump-pulse time-resolved femtosecond optical spectroscopy. We observe remarkable…
Information technology demands high-speed optoelectronic devices, but going beyond the one terahertz (THz) barrier is challenging due to the difficulties associated with generating, detecting, and processing high-frequency signals. Here, we…
We investigate experimentally both the amplitude and phase channels of the collective modes in the quasi-1D charge-density-wave (CDW) system, K0.3MoO3, by combining (i) optical impulsive-Raman pump-probe and (ii) terahertz time-domain…
Coherent phonons describe the collective, ultrafast motion of atoms and play a central role in light-induced structural dynamics. Here, we employ terahertz scanning tunneling microscopy (THz-STM) to excite and detect coherent phonons in…
Density Functional Theory (DFT) calculations not only allow to predict the vibrational and optical properties of solids but also to understand and disentangle the mechanisms playing a key role in the generation of coherent optical phonons.…
Terahertz (THz) nonlinear optics offer powerful tools to investigate and manipulate electronic dynamics in condensed matter. Confining high-peak-power THz pulses within near field can effectively generates extremely localized…
The optical properties of the quarter-filled single-band CDW systems have been reexamined in the model with the electron-phonon coupling related to the variations of electron site energies. It appears that the indirect, electron-mediated…
Time-resolved spectroscopies using intense THz pulses appear as a promising tool to address collective electronic excitations in condensed matter. In particular recent experiments showed the possibility to selectively excite collective…
The strong interlayer coupling in black phosphorus (BP), arising from wavefunction overlap between layers, is critical for understanding its electronic and optical properties. Here, we utilize terahertz (THz) spectroscopy to study phonon…
Hybrid lattice-light modes, known as phonon-polaritons, represent the backbone of advanced protocols based on THz pumping of infrared modes. Here we provide a theoretical framework able to capture the different roles played by…
In this work, a 3-D simulation is performed to study for the solid-fluid coupling effect driven by piezoelectric materials and utilizes asymmetric obstacles to control the flow direction. The result of simulation is also verified. For a…
The shape of a few-cycle terahertz (THz) laser pulse can be optimized to provide control over conduction band populations in graphene. To demonstrate this control in a theoretical way, a spectral parametrization of the driving pulse using…
Converting a THz signal into the optical domain is of great interest for THz sensing and spectroscopy. Here intense broadband THz pulses with a central frequency of $\Omega$$_{THz}$ are mixed with an optical pump at $\omega$$_p$ and a…
Strong optical pulses at mid-infrared and terahertz frequencies have recently emerged as a powerful tool to manipulate and control the solid state and especially complex condensed matter systems with strongly correlated electrons. The…
Coherent phonon-polaritons have attracted a considerable amount of interest owing to their relevance to nonlinear optics and terahertz (THz)-wave emissions. Therefore, it is important to analyze the THz electric-fields of phonon-polaritons.…
We demonstrate a new four-wave mixing (4WM) geometry based on structured light. By utilizing near-field diffraction through a narrow slit, the pump beam is asymmetrically structured to modify the phase matching condition, generating…
Nonlinear processes involving frequency-mixing of light fields set the basis for ultrafast coherent spectroscopy of collective modes in solids. In certain semimetals and semiconductors, generation of coherent phonon modes can occur by a…
We study in detail coherent phase control of femtosecond resonance-mediated (2+1) three-photon absorption and its dependence on the spectral bandwidth of the excitation pulse. The regime is the weak-field regime of third perturbative order.…
Measuring terahertz waveforms in terahertz spectroscopy often relies on electrooptic sampling employing a ZnTe crystal. Although the nonlinearities in such zincblende semiconductors induced by intense terahertz pulses have been studied at…
The coupling of phonons with collective modes and single-particle gap excitations associated with one (1d) and two-directional (2d) electronically-driven charge-density wave (CDW) ordering in metallic RTe_3 is investigated as a function of…