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Non-Gaussian displacement distributions are universal predictors of dynamic heterogeneity in slowly varying environments. Here, we explore heterogeneous dynamics in supercooled liquid using molecular dynamics simulations and show the…

软凝聚态物质 · 物理学 2023-08-29 Vinay Vaibhav , Suman Dutta

The aim of this report is to review a theoretical approach that has been proposed recently to describe dynamic fluctuations in glassy systems (work in collaboration with H. Castillo, C. Chamon, P. Charbonneau, J. L. Iguain, M. Kennett, D.…

无序系统与神经网络 · 物理学 2011-11-09 Leticia F. Cugliandolo

The physics of highly excited Rydberg atoms is governed by blockade or exclusion interactions that hinder the excitation of atoms in the proximity of a previously excited one. This leads to cooperative effects and a relaxation dynamics…

统计力学 · 物理学 2018-09-12 Carlos Pérez-Espigares , Igor Lesanovsky , Juan P. Garrahan , Ricardo Gutiérrez

The dramatic slowing down of relaxation dynamics of liquids approaching the glass transition remains a highly debated problem, where the crux of the puzzle resides in the elusive increase of the activation barrier $\Delta E(T)$ with…

软凝聚态物质 · 物理学 2024-06-19 Geert Kapteijns , David Richard , Eran Bouchbinder , Thomas B. Schrøder , Jeppe C. Dyre , Edan Lerner

We propose that the properties of glass transition can be understood on the basis of elastic waves. Elastic waves originating from atomic jumps in a liquid propagate local expansion due to the anharmonicity of interatomic potential. This…

无序系统与神经网络 · 物理学 2015-05-13 Kostya Trachenko , V. V. Brazhkin

The solidity of glassy materials is believed to be due to the cage formed around each particle by its neighbors, but in reality the details of cage-formation remain elusive [1-4]. This cage starts to be formed at the onset…

软凝聚态物质 · 物理学 2020-12-02 Bo Li , Kai Lou , Walter Kob , Steve Granick

When supercooled, liquids viscosity increases dramatically as the glass transition temperature is approached. While the physical origin of this behavior is still not understood, it is now well established that the addition of a few…

软凝聚态物质 · 物理学 2024-11-25 Victor Teboul

Dynamical heterogeneities have been introduced in the context of the glass transition of molecular liquids and the lengthscale associated with them has been argued to be at the origin of the observed quasi-universal behaviour of glassy…

软凝聚态物质 · 物理学 2015-03-17 Olivier Dauchot , Douglas J. Durian , Martin van Hecke

We propose that the dynamics of supercooled liquids and the formation of glasses can be understood from the existence of a zero temperature dynamical critical point. To support our proposal, we derive from simple physical assumptions a…

软凝聚态物质 · 物理学 2009-11-10 Stephen Whitelam , Ludovic Berthier , Juan P. Garrahan

The description of activated relaxation of glassy systems in the multidimensional configurational space is a long-standing open problem. We develop a phenomenological description of the out-of-equilibrium dynamics of a model with a rough…

无序系统与神经网络 · 物理学 2014-10-09 Chiara Cammarota , Enzo Marinari

Measuring, characterizing and modelling the slow dynamics of glassy soft matter is a great challenge, with an impact that ranges from industrial applications to fundamental issues in modern statistical physics, such as the glass transition…

软凝聚态物质 · 物理学 2009-11-11 Luca Cipelletti , Laurence Ramos

Recent work has demonstrated the strong qualitative differences between the dynamics near a glass transition driven by short-ranged repulsion and one governed by short-ranged attraction. Here, we study in detail the behavior of non-linear,…

统计力学 · 物理学 2010-04-16 P. Charbonneau , D. R. Reichman

Despite decades of intense study, the mechanisms underlying the extraordinary dynamics of supercooled liquids as they approach the glass transition remain, at best, mis-characterized, and at worst, misunderstood. A long standing endeavor is…

无序系统与神经网络 · 物理学 2017-01-04 Nicholas B. Weingartner , Chris Pueblo , K. F. Kelton , Zohar Nussinov

We here discuss the results of 3d MonteCarlo simulations of a minimal lattice model for gelling systems. We focus on the dynamics, investigated by means of the time autocorrelation function of the density fluctuations and the particle mean…

软凝聚态物质 · 物理学 2007-05-23 E. Del Gado , A. Fierro , L. de Arcangelis , A. Coniglio

We analyse numerically thermal fluctuations of the static overlap between equilibrium configurations in a glass-forming liquid approaching the glass transition. We find that the emergence of slow dynamics near the onset temperature…

统计力学 · 物理学 2013-08-23 Ludovic Berthier

We study the dynamics of the East model, comprising a chain of uncoupled spins in a downward-pointing field. Glassy effects arise at low temperatures $T$ from the kinetic constraint that spins can only flip if their left neighbour is up. We…

统计力学 · 物理学 2007-05-23 P. Sollich , M. R. Evans

We formulate a microscopic, force-level, activated dynamics-based statistical-mechanical theory for the continuous startup nonlinear shear-rheology of ultra-dense glass-forming hard-sphere fluids and colloidal suspensions in the context of…

软凝聚态物质 · 物理学 2023-03-22 Ashesh Ghosh , Kenneth S. Schweizer

The mechanism of diffusion in supercooled liquids is investigated from the potential energy landscape point of view, with emphasis on the crossover from high- to low-T dynamics. Molecular dynamics simulations with a time dependent mapping…

统计力学 · 物理学 2009-11-07 T. Keyes , J. Chowdhary

We theoretically study thermally activated elementary dynamical processes that precede full structural relaxation in ultra-dense particle liquids interacting via strong short range attractive forces. Our approach is based on a microscopic…

软凝聚态物质 · 物理学 2020-07-01 Ashesh Ghosh , Kenneth S. Schweizer

We present a first-principles formalism for studying dynamical heterogeneities in glass forming liquids. Based on the Non-Equilibrium Self-Consistent Generalized Langevin Equation theory, we were able to describe the time-dependent local…

软凝聚态物质 · 物理学 2022-04-06 J. Lira-Escobedo , J. R. Velez-Cordero , Pedro E. Ramírez-González