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Although complex, hierarchical nanoscale geometries with tailored degrees of disorder are commonly found in biological systems, few simple self-assembly routes to fabricating synthetic analogues have been identified. We present two…

We investigate the 3D structure and drying dynamics of complex mixtures of emulsion droplets and colloidal particles, using confocal microscopy. Air invades and rapidly collapses large emulsion droplets, forcing their contents into the…

Dynamical heterogeneities in a colloidal fluid close to gelation are studied by means of computer simulations. A clear distinction between some fast particles and the rest, slow ones, is observed, yielding a picture of the gel composed by…

软凝聚态物质 · 物理学 2009-11-10 Antonio M. Puertas , Matthias Fuchs , Michael E. Cates

Understanding interactions between microparticles and lipid membranes is of increasing importance, especially for unraveling the influence of microplastics on our health and environment. Here, we study how a short-ranged adhesive force…

软凝聚态物质 · 物理学 2017-10-11 Casper van der Wel , Doris Heinrich , Daniela J. Kraft

The results of a numerical investigation of fluidized beds of spherical particles in a narrow vertical cylindrical pipe, with particular attention to the spontaneous settling along the wall, are reported. Starting from a steady fluidized…

Extensive molecular dynamics simulations reveal that the interactions between proteins and poly(ethylene glycol)(PEG) can be described in terms of the surface composition of the proteins. PEG molecules accumulate around non-polar residues…

We present the results of an experimental investigation into buoyant rigid spheres rising through highly concentrated collections of hydrated hydrogel particles. The volume fraction of particles is such that the mechanical properties of the…

软凝聚态物质 · 物理学 2026-01-13 Tom Mullin , Tommaso Pettinari , Joshua A. Dijksman

Our understanding of the structural features of foams and emulsions has advanced significantly over the last 20 years. However, with a search for "super-stable" liquid dispersions, foam and emulsion science employs increasingly complex…

The study of interactions between biomimetic membranes and micron-sized particles is crucial for understanding various biological processes. Here, we control microparticle spontaneous engulfment by giant lipid vesicles by tuning particle…

软凝聚态物质 · 物理学 2025-01-22 Clément Marque , Gaetano D'Avino , Domenico Larobina , Aude Michel , Ali Abou-Hassan , Antonio Stocco

Functional polymers, such as poly(ethylene glycol) (PEG) terminated with a single phosphonic acid, hereafter PEGik-Ph are often applied to coat metal oxide surfaces during post synthesis steps, but are not sufficient to stabilize sub-10 nm…

We analyze diffusion of small particles in a solid polymeric medium taking into account a short range particle-polymer interaction. The system is modeled by a particle diffusion on a ternary lattice where the sites occupied by polymer…

统计力学 · 物理学 2015-06-11 Federico Camboni , Andreas Koher , Igor M. Sokolov

For applications in nanomedicine, particles need to be functionalized to prevent protein corona formation and or aggregation. Most advanced strategies take advantage of functional polymers and assembly techniques. Nowadays there is an…

应用物理 · 物理学 2021-09-21 V. Baldim , A. Graillot , N. Bia , C. Loubat , J. -F. Berret

The preparation of many composites requires the intermixing of several macromolecular fluids along with the addition of solid filler particles. These fillers are usuallly polydisperse and there is an extensive experimental evidence that…

软凝聚态物质 · 物理学 2015-06-25 Andrea Corsi , P. D. Gujrati

Investigations of free-standing liquid films enjoy an increasing popularity due to their relevance for many fundamental and applied scientific problems. They constitute soap bubbles and foams, serve as membranes for gas transport or as…

We propose a new mechanism to create self-assembled porous media with highly tunable geometrical properties and permeabilities: We first allow a particle-stabilized emulsion to form from a mixture of two fluids and colloidal particles.…

软凝聚态物质 · 物理学 2024-08-08 Stefan Frijters , Jens Harting

Dip-coating consists in withdrawing a substrate from a bath to coat it with a thin liquid layer. This process is well-understood for homogeneous fluids, but heterogeneities such as particles dispersed in the liquid lead to more complex…

软凝聚态物质 · 物理学 2022-03-02 Deok-Hoon Jeong , Michael Ka Ho Lee , Virgile Thiévenaz , Martin Z. Bazant , A. Sauret

We use confocal microscopy to image colloidal gels formed from highly polydisperse particles. We suspend our polydisperse particles in a density matched solvent, and let the particles spontaneously aggregate through the van der Waals force.…

软凝聚态物质 · 物理学 2026-02-24 Benjamin F. Lonial , Eric R. Weeks

The properties of suspensions of fine particles in dielectric liquid (electrorheological fluids) subjected to an electric field lead to a drastic change of the apparent viscosity of the fluid. For high applied fields (~ 3-5 kV/mm) the…

化学物理 · 物理学 2007-05-23 Quentin Guegan , J. -N. Foulc , F. Ayela , O. Tillement

This feature article presents insights concerning the correlation of PECVD and PEALD thin film structures with their barrier or membrane properties. While in principle similar precursor gases and processes can be applied, the adjustment of…

Surfaces of surfactant-templated polyacrylamide hydrogels were imaged by atomic force microscopy (AFM), and the surface morphology was studied by numerical scaling analysis. The templated gels were formed by polymerizing acrylamide plus a…

软凝聚态物质 · 物理学 2007-05-23 Mukundan Chakrapani , S. J. Mitchell , D. H. Van Winkle , P. A. Rikvold