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The recent report of superconductivity in the Cu-doped PbPO compound stimulates the extensive researches on its physical properties. Herein, the detailed atomic and electronic structures of this compound are investigated, which are the…

超导电性 · 物理学 2023-08-09 Jianfeng Zhang , Huazhen Li , Ming Yan , Miao Gao , Fengjie Ma , Xun-Wang Yan , Z. Y. Xie

Based on the first-principles electronic structure calculations, we investigate the magnetic and electronic properties of transition-metal-doped Pb$_{10}$(PO$_4$)$_6$O with the Pb atom substituted by various transition metals. The $3d$…

材料科学 · 物理学 2023-10-02 Bingxin Liu , Tong Liu , Xun-Wang Yan , Zong-Liang Li

Based on DFT calculations, we present the basic electronic structure of CuPb9(PO4)6O (Cu-doped lead apatite, LK-99), in two scenarios: (1) where the structure is constrained to the P3 symmetry and (2) where no symmetry is imposed. At the…

The flurry of theoretical and experimental studies following the report of room-temperature superconductivity at ambient pressure in Cu-substituted lead apatite Cu$_x$Pb$_{10-x}$(PO$_4$)$_6$O (`LK99') have explored whether and how this…

强关联电子 · 物理学 2024-01-11 Katherine Inzani , John Vinson , Sinéad M. Griffin

Correlation effects in CuO$_2$ layers give rise to a complicated landscape of collective excitations in high-T$_{\rm c}$ cuprates. Their description requires an accurate account for electronic fluctuations at a very broad energy range and…

强关联电子 · 物理学 2018-11-09 E. A. Stepanov , L. Peters , I. S. Krivenko , A. I. Lichtenstein , M. I. Katsnelson , A. N. Rubtsov

The hope that copper doped lead apatite Pb$_9$Cu(PO$_4$)$_6$O is a room-temperature superconductor has largely been dashed by global research efforts. Nevertheless, according to the current state of knowledge, the material has interesting…

强关联电子 · 物理学 2023-08-29 Makoto Shimizu , Junya Otsuki , Harald O. Jeschke

We study the correlated electronic structure and local spin behaviour of the copper-substituted lead-vanadium bromine apatite Pb$_9$Cu(VO$_4$)$_6$Br$_2$ using DFT+DMFT with a two-orbital Cu-centred low-energy model. Simulations are done for…

强关联电子 · 物理学 2025-12-17 Ihor Sukhenko , Volodymyr Karbivskyy

Two recent preprints in the physics archive (arXiv) have called attention as they claim experimental evidence that a Cu-substituted apatite material (dubbed LK-99) exhibits superconductivity at room temperature and pressure. If this proves…

超导电性 · 物理学 2024-05-17 J. Cabezas-Escares , N. F. Barrera , R. H. Lavroff , A. N. Alexandrova , C. Cardenas , F. Munoz

The search for room-temperature superconductors has been a long-standing goal in condensed matter physics. In this study, we investigate the electronic and geometric properties of lead apatite with and without Cu doped within the frame work…

超导电性 · 物理学 2023-11-27 Kun Tao , Rongrong Chen , Lei Yang , Jin Gao , Desheng Xue , Chenglong Jia

We report a new peculiar effect of the interaction between a sublattice of frustrated quantum spin-1/2 chains and a sublattice of pseudospin-1/2 centers (quantum electric dipoles) uniquely co-existing in the complex oxide Li2ZrCuO4. 7Li…

The pursuit of room-temperature ambient-pressure superconductivity in novel materials has sparked interest, with recent reports suggesting such properties in Cu-substituted lead apatite, known as LK-99. However, these claims lack…

材料科学 · 物理学 2023-09-01 Songge Yang , Guangchen Liu , Yu Zhong

Electronic structure calculations are used to analyze the electronic and magnetic properties in {K$_{2}$Fe$_{4+x}$Se$_{5}$}. Fe atoms can be divided into two distinct groups. The $x{=}0$ (parent) compound forms an insulating, collinear,…

材料科学 · 物理学 2012-09-04 Liqin Ke , Mark van Schilfgaarde , Vladimir Antropov

A recent report of room temperature superconductivity at ambient pressure in Cu-substituted apatite (`LK99') has invigorated interest in the understanding of what materials and mechanisms can allow for high-temperature superconductivity.…

超导电性 · 物理学 2023-08-04 Sinéad M. Griffin

The pseudogap metal phase of the hole-doped cuprate superconductors has two seemingly unrelated characteristics: a gap in the electronic spectrum in the `anti-nodal' region of the square lattice Brillouin zone, and discrete broken…

强关联电子 · 物理学 2017-12-06 Shubhayu Chatterjee , Subir Sachdev , Mathias Scheurer

Magnetic structures of organic Mott insulators X[Pd(dmit)2]2 (X=Me4P, Me4Sb), of which electronic states are located near quantum spin liquid (X=EtMe3Sb), are demonstrated by 13C NMR. Antiferromagnetic spectra and nuclear relaxations show…

强关联电子 · 物理学 2019-05-01 Shigeki Fujiyama , Reizo Kato

A microscopic theory for the NMR anomalies of the planar Cu and O sites in superconducting La_1.85Sr_0.15CuO_4 is presented that quantitatively explains the observations without the need to invoke anit-ferromagnetic spin fluctuations on the…

超导电性 · 物理学 2016-09-28 Jamil Tahir-Kheli

The electronic nematic state without magnetization emerges in various strongly correlated metals such as Fe-based and cuprate superconductors. To understand this universal phenomenon, we focus on the nematic state in Ti-oxypnictide…

强关联电子 · 物理学 2016-06-15 Hironori Nakaoka , Youichi Yamakawa , Hiroshi Kontani

We have investigated electronic structures of a room temperature diluted magnetic semiconductor : Co-doped anatase $\rm TiO_{2}$. We have obtained the half-metallic ground state in the local-spin-density approximation(LSDA) but the…

材料科学 · 物理学 2009-11-07 Min Sik Park , S. K. Kwon , B. I. Min

In this work we study the interplay between the crystal structure and magnetism of the pyroarsenate \alpha-Cu_2As_2O_7 by means of magnetization, heat capacity, electron spin resonance and nuclear magnetic resonance measurements as well as…

The most recent discovery, the Cu-doped lead apatite LK-99, is a proposed room-temperature superconductor operating under ambient pressure. However, this discovery has brought a slew of conflicting results from different scientific groups.…

超导电性 · 物理学 2023-09-18 Jun Li , Qi An
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