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Superconductivity in infinite-layer nickelates holds exciting analogies with that of cuprates, with similar structures and $3d$-electron count. Using resonant inelastic x-ray scattering (RIXS) we studied electronic and magnetic excitations…

A charge order (CO) with a wavevector $\mathbf{q}\simeq\left(\frac{1}{3},0,0\right)$ is observed in infinite-layer nickelates. Here we use first-principles calculations to demonstrate a charge-transfer-driven CO mechanism in infinite-layer…

强关联电子 · 物理学 2023-09-11 Hanghui Chen , Yi-feng Yang , Guang-Ming Zhang , Hongquan Liu

The dynamics of the charge ordered (CO) state under non-equilibrium conditions created by strong dc-electric field (~106 V/cm) and photo-illumination with short (~ 6 ns) laser pulses is investigated in Bi1-xCaxMnO3 (x > 0.5) epitaxial…

强关联电子 · 物理学 2007-05-23 S. Chaudhuri , R. C. Budhani

Several reports about infinite-layer nickelate thin films suggest that the superconducting critical temperature versus chemical doping phase diagram has a dome-like shape, similar to cuprates. Here, we demonstrate a highly reproducible…

We report scanning tunnelling microscopy (STM) and x-ray photoemission spectroscopy (XPS) measurements on uncapped and SrTiO3 (STO) capped NdNiO2 realized by pulsed-laser deposition and topotactic reduction process. We find that untreated…

超导电性 · 物理学 2024-02-06 Martando Rath , Yu Chen , Guillaume Krieger , H. Sahib , Daniele Preziosi , Marco Salluzzo

A defining signature of strongly correlated electronic systems is the existence of competing phases with similar ground state energies, resulting in a rich phase diagram. While in the recently discovered nickelate superconductors, a high…

Recent experiments in Pr(Nd)$_{0.5}$Ca$_{0.5}$MnO$_3$ thin films exhibited (multiple) reentrant charge ordering (CO) transitions with change of {\it temperature} T under fixed magnetic field H, which are in contrast to the results for the…

强关联电子 · 物理学 2010-05-24 Qingshan Yuan , Thilo Kopp

The observation of superconductivity in infinite layer nickelate (Nd,Sr)NiO$_{2}$ thin films has led to rapid theoretical and experimental investigations of these copper-oxide-analogue systems [1-15]. Superconductivity has also been found…

We report the observation of superconductivity in infinite-layer Ca-doped LaNiO$_2$ (La$_{1-x}$Ca$_x$NiO$_2$) thin films and construct their phase diagram. Unlike the metal-insulator transition in Nd- and Pr-based nickelates, the undoped…

超导电性 · 物理学 2022-02-25 S. W. Zeng , C. J. Li , L. E. Chow , Y. Cao , Z. T. Zhang , C. S. Tang , X. M. Yin , Z. S. Lim , J. X. Hu , P. Yang , A. Ariando

We have utilized neutron powder diffraction to probe the crystal structure of layered Na$_{x}$CoO$_{2}$ near the half doping composition of $x=$0.46 over the temperature range of 2 to 600K. Our measurements show evidence of a dynamic…

强关联电子 · 物理学 2008-06-16 D. N. Argyriou , O. Prokhnenko , K. Kiefer , C. J. Milne

The recent discovery of ambient-pressure superconductivity with $T_c$ above 40 K in La$_3$Ni$_2$O$_7$ thin films represents a significant advance in the field of nickelate superconductor. Motivated by the experimental reports, here we study…

超导电性 · 物理学 2026-02-19 Yuxun Zhong , Wéi Wú , Dao-Xin Yao

Using \emph{ab initio} band structure methods and DFT+dynamical mean-field theory approach we explore the possible formation of spin and charge stripes in the Ni-O plane of hole-doped infinite-layer nickelates, $R$NiO$_2$. Our results…

强关联电子 · 物理学 2022-10-12 K. G. Slobodchikov , I. V. Leonov

Magnetic anisotropy in disordered rare-earth-transition metals (RE-TM) compounds arises from RE atoms occupying asymmetric environments within the TM lattice. However, the underlying mechanism that promotes such environments remains not…

材料科学 · 物理学 2026-01-23 J. Díaz , J. Rodríguez-Fernández , J. Rubio-Zuazo

Ab initio band theory including correlations due to intra-atomic repulsion is applied to study charge disproportionation and charge- and spin-ordering in insulating Na$_{0.5}$CoO$_2$. Various ordering patterns (zigzag and two striped) for…

强关联电子 · 物理学 2007-05-23 K. -W. Lee , W. E. Pickett

Infinite layer nickelates have garnered significant attention due to their potential for high-temperature superconductivity. Despite extensive research, the interplay between oxygen stoichiometry and electronic properties in infinite layer…

The temperature evolution of structural effects associated with charge (CO) and spin order (SO) in La$_{1.67}$Sr$_{0.33}$NiO$_{4}$ has been investigated using neutron powder diffraction. We report an anomalous shrinking of the $c/a$ lattice…

Recently superconductivity at 9 - 15 K was discovered in an infinite-layer nickelate (Nd$_{0.8}$Sr$_{0.2}$NiO$_2$ films), which has received enormous attention. Since the $Ni^{1+}$ ionic state in NdNiO$_2$ may have the $3d^9$ outer-shell…

超导电性 · 物理学 2020-04-06 Qing Li , Chengping He , Jin Si , Xiyu Zhu , Yue Zhang , Hai-Hu Wen

We have successfully grown epitaxial La$_{1.67}$Sr$_{0.33}$NiO$_4$ films with a small crystalline mosaic using pulsed laser deposition. With synchrotron radiation, the x-ray diffraction peaks associated with charge stripes have been…

强关联电子 · 物理学 2009-11-13 C. K. Xie , J. I. Budnick , W. A. Hines , B. O. Wells , Feizhou He , A. R. Moodenbaugh

Nickel-based superconductors provide a long-awaited experimental platform to explore possible cuprate-like superconductivity. Despite similar crystal structure and $d$ electron filling, these systems exhibit several differences. Nickelates…

We used resonant elastic x-ray scattering at the Cu $L_3$ and Dy $M_5$ edges to investigate charge order in thin films of underdoped DyBa$_2$Cu$_3$O$_{6+x}$ (DyBCO) epitaxially grown on NdGaO$_3$ (110) substrates. The films show an…

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