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Neutron diffraction was used to determine the crystal structure and magnetic ordering pattern of a La2CuO4 single crystal, with and without applied magnetic field. A previously unreported, subtle monoclinic distortion of the crystal…

强关联电子 · 物理学 2009-11-11 M. Reehuis , C. Ulrich , K. Prokes , A. Gozar , G. Blumberg , Seiki Komiya , Yoichi Ando , P. Pattison , B. Keimer

Magnetic and orbital structures in KCuF$_{3}$ are revisited by the cluster self-consistent field approach developed recently. We clearly showed that due to the inherent frustration, the ground state of the system with the superexchange and…

强关联电子 · 物理学 2007-05-23 Dong-Meng Chen , Liang-Jian Zou

We present an elaborate electron-spin resonance study of the low-energy dynamics and magnetization in the ordered phase of the magnetically frustrated spinel ZnCr$_2$O$_4$. We observe several resonance modes corresponding to different…

强关联电子 · 物理学 2010-11-29 V. N. Glazkov , A. M. Farutin , V. Tsurkan , H. -A. Krug von Nidda , A. Loidl

The 3d electronic structure and phase transition in pure and Cr doped V2O3 are theoretically investigated in relation to the 3d spin-orbit interaction and lattice distortion. A model consisting of the nearest-neighbor V ion pair with full…

强关联电子 · 物理学 2016-08-31 Arata Tanaka

It is shown that the time-reversal symmetry is broken during the phase transition causing orbital ordering in a crystal with Jahn-Teller (J-T) ions. This means that such phase transitions are magnetic ones. As an example we have considered…

强关联电子 · 物理学 2023-11-27 Khisa Borlakov , Dalkhat Ediev , Amina Borlakova

The properties of Mott insulators with orbital degrees of freedom are described by spin-orbital superexchange models, which provide a theoretical framework for understanding their magnetic and optical properties. We introduce such a model…

强关联电子 · 物理学 2015-05-19 Andrzej M. Oleś , Peter Horsch

We report on first principles Self-Interaction Corrected LSD (SIC-LSD) calculations of electronic structure of LaMnO$_{3}$ in the cubic phase. We found a strong tendency to localisation of the Mn $e_{g}$ electron and to orbital ordering. We…

强关联电子 · 物理学 2009-11-11 H. Zenia , G. A. Gehring , W. M. Temmerman

Density functional calculations are performed to study the magnetic order of the severely distorted square planar cupric oxide (CuO) and local spin disorder in it in the presence of the transition metal impurities M (= Cr, Mn, Fe, Co and…

强关联电子 · 物理学 2017-04-05 B. G. Ganga , P. N. Santhosh , B. R. K. Nanda

Iron telluride (FeTe), a relative of the iron based high temperature superconductors, displays unusual magnetic order and structural transitions. Here we explore the idea that strong correlations may play an important role in these…

材料科学 · 物理学 2013-05-29 Ari M. Turner , Fa Wang , Ashvin Vishwanath

Multi-orbital physics in quasi-two-dimensional electron gases (q2DEGs) triggers unique phenomena not observed in bulk materials, such as unconventional superconductivity and magnetism. Here, we investigate the mechanism of orbital selective…

Perovskites with the generic composition ABO$_3$ exhibit an enormous variety of quantum states such as magnetism, orbital order, ferroelectricity and superconductivity. Their flexible and comparatively simple structure allows for facile…

Distortions of the oxygen octahedra influence the fundamental electronic structure of perovskite oxides, such as their bandwidth and exchange interactions. Utilizing a fully ab-initio methodology based on density functional theory plus…

强关联电子 · 物理学 2021-07-02 Alexander Hampel , Jeremy Lee-Hand , Antoine Georges , Cyrus E. Dreyer

Spinel Li$_x$Mn$_2$O$_4$ is a key cathode material that is used extensively in commercial Li-ion batteries. A challenge with this material has been that the capacity of the battery fades with cycling, an effect that can be traced to the…

We have investigated electronic structures of antiferromagnetic YBaCo_2O_5 using the local spin-density approximation (LSDA) + U method. The charge and orbital ordered insulating ground state is correctly obtained with the strong on-site…

强关联电子 · 物理学 2009-10-31 S. K. Kwon , B. I. Min

Including the orbital off-diagonal spin and charge condensates in the self consistent determination of magnetic order within a realistic three-orbital model for the $4d^4$ compound $\rm Ca_2 Ru O_4$, reveals a host of novel features…

强关联电子 · 物理学 2021-07-05 Shubhajyoti Mohapatra , Avinash Singh

We report a thorough study of Y$_{0.7}$La$_{0.3}$VO$_3$ single crystals by measuring magnetic properties, specific heat, thermal conductivity, x-ray and neutron diffraction with the motivation of revealing the lattice response to the…

强关联电子 · 物理学 2019-12-04 J. -Q. Yan , W. Tian , H. B. Cao , S. Chi , F. Ye , A. Llobet , Q. Chen , J. Ma , Y. Ren , J. -G. Cheng , J. -S. Zhou , M. A. McGuire , R. J. McQueeney

Transition metal oxides with a wide variety of electronic and magnetic properties offer an extraordinary possibility to be a platform for developing future electronics based on unconventional quantum phenomena, for instance, the topology.…

Motivated by the recently observed unconventional Hall effect in ultra-thin films of ferromagnetic SrRuO$_3$ (SRO) we investigate the effect of strain-induced oxygen octahedral distortion in the electronic structure and anomalous Hall…

材料科学 · 物理学 2021-03-31 Kartik Samanta , Marjana Ležaić , Stefan Blügel , Yuriy Mokrousov

Alkali superoxides differ from conventional transition metal magnets, exhibit magnetism from partially occupied oxygen molecular $\pi^*$-orbitals. Among them, CsO$_2$ stands out for its potential to exhibit novel quantum collective…

强关联电子 · 物理学 2024-11-12 Ryota Ono , Ravi Kaushik , Sergey Artyukhin , Martin Jansen , Igor Solovyev , Russell A. Ewings

The strain tuned magnetism of YTiO$_3$ film grown on the LaAlO$_3$ ($110$) substrate is studied by the method of the first principles, and compared with that of the ($001$)-oriented one. The obtained magnetism is totally different, which is…

材料科学 · 物理学 2015-02-16 Xin Huang , Qingyu Xu , Shuai Dong