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Nanoparticles are often covered in ligand monolayers, which can undergo a temperature-dependent order-disorder transition that switches the particle-particle interaction from repulsive to attractive in solution. In this work, we examine how…

软凝聚态物质 · 物理学 2018-07-05 Asaph Widmer-Cooper , Phillip L. Geissler

The influence of ligands on the low frequency vibration of different thicknesses cadmium selenide colloidal nanoplatelets is investigated using resonant low frequency Raman scattering. The strong vibration frequency shifts induced by ligand…

Semiconductor nanocrystals are a promising class of materials for a variety of novel optoelectronic devices, since many of their properties, such as the electronic gap and conductivity, can be controlled. Much of this control is achieved…

化学物理 · 物理学 2017-06-06 Nadav Geva , James J. Shepherd , Lea Nienhaus , Moungi G. Bawendi , Troy Van Voorhis

Inorganic nanoparticle cores are often coated with organic ligands to render them dispersible in apolar solvents. However, the effect of the ligand shell on the colloidal stability of the overall hybrid particle is not fully understood. In…

软凝聚态物质 · 物理学 2019-02-21 Debora Monego , Thomas Kister , Nicholas Kirkwood , Paul Mulvaney , Asaph Widmer-Cooper , Tobias Kraus

The surface ligands on colloidal nanocrystals (NCs) play an important role in the performance of NCs based optoelectronic devices such as photovoltaic cells, photodetectors and light emitting diodes (LEDs). On one hand, the NC emission…

化学物理 · 物理学 2020-04-27 Prachi Rastogi , Francisco Palazon , Mirko Prato , Francesco Di Stasio , Roman Krahne

Capping ligands are crucial to synthesize colloidal nanoparticles with novel functional properties. However, the interaction between capping ligands and their interaction with the crystallographic surfaces of nanoparticles during colloidal…

材料科学 · 物理学 2021-05-19 Kyuseon Jang , Se-Ho Kim , Hosun Jun , Chanwon Jung , Jiwon Yu , Sangheon Lee , Pyuck-Pa Choi

Organic surface ligands are integral components of nanocrystals and nanoparticles that have a strong influence on their physicochemical properties, their interaction with the environment, and their ability to self-assemble and order into…

The self-assembly of binary nanoparticle superlattices from colloidal mixtures is a promising method for the fabrication of complex colloidal co-crystal structures. However, binary mixtures often form amorphous or metastable phases instead…

软凝聚态物质 · 物理学 2022-05-11 R. Allen LaCour , Timothy C. Moore , Sharon C. Glotzer

Colloidal nanocrystal gels can be assembled using a difunctional "linker" molecule to mediate bonding between nanocrystals. The conditions for gelation and the structure of the gel are controlled macroscopically by the linker concentration…

The ability of thin materials to shape-shift is a common occurrence that leads to dynamic pattern formation and function in natural and man-made structures. However, harnessing this concept to design inorganic structures at the nanoscale…

Small-angle neutron and X-ray scattering, neutron backscattering and neutron time-of-flight spectroscopy are applied to reveal the structure of the ligand shell, the temperature-dependent diffusion properties and the phonon spectrum of PbS…

The generation of nanoscale square and stripe patterns is of major technological importance since they are compatible with industry-standard electronic circuitry. Recently, a blend of diblock copolymer interacting via hydrogen-bonding was…

软凝聚态物质 · 物理学 2009-11-13 Carlos I. Mendoza , Erasmo Batta

The structural and chemical properties of metal nanoparticles are often dictated by their interactions with molecular ligand shells. These interactions are highly material-specific and can vary significantly even among elements within the…

It is widely accepted that the properties of most semiconductor nanocrystals can be tuned by their core size, shape and material. In covalent semiconductor nanocrystal materials, such as silicon, germanium or carbon, certain degree of…

介观与纳米尺度物理 · 物理学 2019-05-30 Katerina Dohnalova Newell , Prokop Hapala , Katerina Kusova , Ivan Infante

We report the synthesis and optical characterization of fully inorganic gradientshell CdSe/CdZnS nanocrystals (NCs) with high luminescence quantum yield (QY, 50 percent), which were obtained by replacing native oleic-acid (OA) ligands with…

材料科学 · 物理学 2021-11-03 Justine Baronnier , Benoit Mahler , Christophe Dujardin , Florian Kulzer , Julien Houel

Ligand coated nanoparticles are complex objects consisting of a metallic or semiconductor core with organic ligands grafted on their surface. These organic ligands provide stability to a nanoparticle suspension. In solutions, the effective…

软凝聚态物质 · 物理学 2022-03-01 Dinesh Chintha , Shivanand Kumar Veesam , Emanuele Boattini , Laura Filion , Sudeep N Punnathanam

We analyse a binary mixture of colloidal parallel hard cylindrical particles with identical diameters but dissimilar lengths $L_1$ and $L_2$, with $s=L_2/L_1=3$, confined by two parallel hard walls in a planar slit-pore geometry, using a…

软凝聚态物质 · 物理学 2019-03-27 Daniel de las Heras , Yuri Martinez-Raton , Enrique Velasco

The exciton states of strained CdTe/CdS core-shell tetrapod-shaped nanocrystals were theoretically investigated by the numerical diagonalization of a configuration interaction Hamiltonian based on the single-band effective mass…

介观与纳米尺度物理 · 物理学 2015-06-23 Yuanzhao Yao , Takashi Kuroda , Dmitry N. Dirin , Maria S. Sokolikova , Roman B. Vasiliev

This report presents a systematic understanding of the nature behind the unusual behavior of a nanosolid, and a surface as well, in mechanics, thermodynamics, acoustics, optoelectronics, magnetism, dielectrics, atomic diffusivity and…

材料科学 · 物理学 2007-05-23 Chang Q Sun

The theory of elastic interaction of micron size axially symmetric colloidal particles immersed into confined nematic liquid crystal has been proposed. General formulas are obtained for the self energy of one colloidal particle and…

软凝聚态物质 · 物理学 2015-05-14 S. B. Chernyshuk , B. I. Lev
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