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In many scientific fields, there is an interest in understanding the way in which complex chemical networks evolve. The chemical networks which researchers focus upon, have become increasingly complex and this has motivated the development…

We propose an ultrahigh-efficiency, broadband and multi-channel all-optical switching scheme based on broadband coherent perfect absorption (CPA) in a linear and nonlinear regimes in a cavity quantum electrodynamics (CQED) system. Two…

量子物理 · 物理学 2024-03-12 Liyong Wang , Yinxue Zhao , Jiajia Du

Biphasic chemical reactions compartmentalized in small droplets offer advantages, such as streamlined procedures for chemical analysis, enhanced chemical reaction efficiency and high specificity of conversion. In this work, we…

软凝聚态物质 · 物理学 2020-07-10 Zhengxin Li , Akihito Kiyama , Hongbo Zeng , Detlef Lohse , Xuehua Zhang

We propose a scheme to realize quantum controlled phase flip (CPF) between two rare earth ions embedded in respective microsphere cavity via interacting with a single-photon pulse in sequence. The numerical simulations illuminate that the…

量子物理 · 物理学 2009-11-10 Yun-Feng Xiao , Xiu-Min Lin , Jie Gao , Yong Yang , Zheng-Fu Han , Guang-Can Guo

We demonstrate the emergence of nonreciprocal superradiant phase transitions and novel multicriticality in a cavity quantum electrodynamics (QED) system, where a two-level atom interacts with two counter-propagating modes of a…

量子物理 · 物理学 2024-10-01 Gui-Lei Zhu , Chang-Sheng Hu , Hui Wang , Wei Qin , Xin-You Lü , Franco Nori

We present an ab initio correlated approach to study molecules that interact strongly with quantum fields in an optical cavity. Quantum electrodynamics coupled cluster theory provides a non-perturbative description of cavity-induced effects…

化学物理 · 物理学 2020-12-07 Tor S. Haugland , Enrico Ronca , Eirik F. Kjønstad , Angel Rubio , Henrik Koch

Recently the first chemical systems which show the amplification of enantiometric excess (ee) was found. Inspired by these experiments, we propose a few chemical reaction models in a closed system. The reactions consist of autocatalytic…

生物物理 · 物理学 2007-05-23 Yukio Saito , Hiroyuki Hyuga

The mechanical influence on objects due to their interaction with light has been a central topic in atomic physics for decades. Thus, one finds that many concepts developed to describe cavity optomechanical systems with solid-state…

量子物理 · 物理学 2012-04-20 Dan M. Stamper-Kurn

The design of an experiment on the spontaneous crystallization of a laser-cooled, but thermal atomic cloud into a hexagonally structured phase is discussed. Atomic interaction is mediated by the dipole potential of an optical lattice formed…

Coherent interfaces between optical photons and long-lived matter qubits form a key resource for a broad range of quantum technologies. Cavity quantum electrodynamics (cQED) offers a route to achieve such an interface by enhancing…

量子物理 · 物理学 2021-01-11 Erika Janitz , Mihir K. Bhaskar , Lilian Childress

Catalysis is indispensable to chemical processes and relevant to many aspects of modern life. Owing to the intriguing electronic structures and good ionic properties, multivalent transition metal oxides have attracted attention as key…

Cavity quantum electrodynamics (cavity QED) describes the coherent interaction between matter and an electromagnetic field confined within a resonator structure, and is providing a useful platform for developing concepts in quantum…

Atomic nuclei are composite systems, and they may be dynamically excited during nuclear reactions. Such excitations are not only relevant to inelastic scattering but they also affect other reaction processes such as elastic scattering and…

核理论 · 物理学 2022-05-25 K. Hagino , K. Ogata , A. M. Moro

Single atoms coupled to a cavity offer unique opportunities as quantum optomechanical devices because of their small mass and strong interaction with light. A particular regime of interest in optomechanics is that of "single-photon strong…

量子物理 · 物理学 2022-04-01 Javier Argüello-Luengo , Darrick E. Chang

In recent years tremendous progress in the field of light-matter interactions has unveiled that strong coupling to the modes of an optical cavity can alter chemistry even at room temperature. Despite these impressive advances, many…

化学物理 · 物理学 2020-05-20 Dominik Sidler , Michael Ruggenthaler , Heiko Appel , Angel Rubio

Cavity quantum electrodynamics (CQED) investigates the interaction between light confined in a resonator and particles, such as atoms. In recent years, CQED experiments have reached the optical domain resulting in many interesting…

量子物理 · 物理学 2020-12-14 Michael Scheucher , Jürgen Volz , Arno Rauschenbeutel

The strong coupling between molecules and photons in resonant cavities offers a new toolbox to manipulate photochemical reactions. While the quenching of photochemical reactions in the strong coupling regime has been demonstrated before,…

介观与纳米尺度物理 · 物理学 2019-12-24 Jacop Fregoni , Giovanni Granucci , Maurizio Persico , Stefano Corni

The striking nonlinear effects exhibited by cavity QED systems make them a powerful tool in modern condensed matter and atomic physics. A recently discovered example is the quantized pumping of energy into a cavity by a strongly-coupled,…

量子物理 · 物理学 2022-05-05 David M. Long , Philip J. D. Crowley , Alicia J. Kollár , Anushya Chandran

A light-matter hybrid quasiparticle, called a polariton, is formed when molecules are strongly coupled to an optical cavity. Recent experiments have shown that polariton chemistry can manipulate chemical reactions. Polariton chemistry is a…

化学物理 · 物理学 2024-01-11 Xinyang Li , Nicholas Lubbers , Sergei Tretiak , Kipton Barros , Yu Zhang

Cavity-mediated light-matter coupling can dramatically alter opto-electronic and physico-chemical properties of a molecule. Ab initio theoretical predictions of these systems need to combine non-perturbative, many-body electronic structure…

量子物理 · 物理学 2024-06-19 Derek S. Wang , Tomáš Neuman , Johannes Flick , Prineha Narang