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Temperature-driven polyamorphism has been reported in various supercooled liquids and glasses. The dynamical and structural routes followed by the system during such crossovers are however not universal and appear to be related to intrinsic…

无序系统与神经网络 · 物理学 2018-08-29 S. Hechler , B. Ruta , M. Stolpe , E. Pineda , Z. Evenson , O. Gross , W. Hembree , A. Bernasconi , R. Busch , I. Gallino

The viscosity of glass-forming liquids increases by many orders of magnitude if their temperature is lowered by a mere factor of 2-3 [1,2]. Recent studies suggest that this widespread phenomenon is accompanied by spatially heterogeneous…

无序系统与神经网络 · 物理学 2015-05-28 Walter Kob , Sandalo Roldan-Vargas , Ludovic Berthier

We consider two thin layers of immiscible liquids on a heated solid horizontal substrate. The free liquid-liquid and liquid-gas interfaces of such a two-layer (or bilayer) liquid film may be unstable due to effective molecular interactions…

斑图形成与孤子 · 物理学 2007-05-23 Andrey Pototsky , Michael Bestehorn , Domnic Merkt , Uwe Thiele

A recent study has demonstrated that phase separation in binary liquid mixtures is arrested in the presence of elastic networks and can lead to a nearly uniformly-sized distribution of the dilute-phase droplets. At longer timescales, these…

软凝聚态物质 · 物理学 2020-10-28 Mrityunjay Kothari , Tal Cohen

The dynamics of supercooled liquid and glassy systems are usually studied within the Lagrangian representation, in which the positions and velocities of distinguishable interacting particles are followed. Within this representation,…

无序系统与神经网络 · 物理学 2009-09-28 Claudio Chamon , Leticia F. Cugliandolo , Gabriel Fabricius , Jose Luis Iguain , Eric R. Weeks

We combine the hyper-netted chain approximation of liquid state theory with the mode-coupling theory of the glass transition to analyze the structure and dynamics of soft spheres interacting via harmonic repulsion. We determine the locus of…

统计力学 · 物理学 2010-03-29 Ludovic Berthier , Elijah Flenner , Hugo Jacquin , Grzegorz Szamel

Recently, ultrastable glasses have been created through vapor deposition. Subsequently, computer simulation algorithms have been proposed that mimic the vapor deposition process and result in simulated glasses with increased stability. In…

软凝聚态物质 · 物理学 2015-01-15 Hannah Staley , Elijah Flenner , Grzegorz Szamel

The precipitation of a glass forming solute from solution is modelled using a lattice model previously introduced to study dissolution kinetics of amorphous materials. The model includes the enhancement of kinetics at the surface of a glass…

软凝聚态物质 · 物理学 2019-05-15 Ian Douglass , Peter Harrowell

We study heterogeneities in a binary Lennard-Jones system below the glass transition using molecular dynamics simulations. We identify mobile and immobile particles and measure their distribution of vibrational amplitudes. For temperatures…

无序系统与神经网络 · 物理学 2013-05-29 Katharina Vollmayr-Lee , Annette Zippelius

A quasi 2-dimensional recursive lattice formed by planar elements have been designed to investigate the surface thermodynamics of Ising spin glass system with the aim to study the metastability of supercooled liquids and the ideal glass…

统计力学 · 物理学 2015-02-24 Ran Huang , Purushottam D. Gujrati

Glass-to-glass and liquid-to-liquid phase transitions were observed many years ago in bulk and confined water with or without applied pressure. It is shown that they result from the competition of two-liquid phases separated by an enthalpy…

无序系统与神经网络 · 物理学 2017-03-21 Robert F Tournier

While deeply supercooled liquids exhibit divergent viscosity and increasingly heterogeneous dynamics as the temperature drops, their structure shows only seemingly marginal changes. Understanding the nature of relaxation processes in this…

材料科学 · 物理学 2022-11-03 Matthias Lerbinger , Armand Barbot , Damien Vandembroucq , Sylvain Patinet

We investigate a binary Lennard-Jones mixture with molecular dynamics simulations. We consider first a system cooled linearly in time with the cooling rate gamma. By varying gamma over almost four decades we study the influence of the…

统计力学 · 物理学 2015-06-25 K. Vollmayr-Lee , W. Kob , K. Binder , A. Zippelius

When a liquid is cooled below its melting temperature, if crystallization is avoided, it forms a glass. This phenomenon, called glass transition, is characterized by a marked increase of viscosity, about 14 orders of magnitude, in a narrow…

无序系统与神经网络 · 物理学 2008-08-23 Simone Capaccioli , Giancarlo Ruocco , Francesco Zamponi

We perform kinetic Monte Carlo simulations of a distinguishable-particle lattice model of structural glasses with random particle interactions. By varying the interaction distribution and the average particle hopping energy barrier, we…

软凝聚态物质 · 物理学 2021-01-04 Chun-Shing Lee , Matteo Lulli , Ling-Han Zhang , Hai-Yao Deng , Chi-Hang Lam

The hypersphere model is a simple one-parameter model of the potential energy landscape of viscous liquids, which is defined as a percolating system of same-radius hyperspheres randomly distributed in $\mathbb{R}^{3N}$ in which $N$ is the…

软凝聚态物质 · 物理学 2025-05-02 Mark F. B. Railton , Eva Uhre , Jeppe C. Dyre , Thomas B. Schrøder

Out-of-equilibrium systems, inherently complex and challenging to understand, are prevalent across various disciplines, including physics where they arise in contexts such as fluid dynamics. In particular, critical out-of-equilibrium…

统计力学 · 物理学 2025-10-14 J. M. Marcos

In the wake of previous studies on the rattling-and-jumping diffusion in smectic liquid crystal phases of colloidal rods, we analyze here for the first time the heterogeneous dynamics in columnar phases. More specifically, we perform…

软凝聚态物质 · 物理学 2015-05-19 Simone Belli , Alessandro Patti , René van Roij , Marjolein Dijkstra

We address the hydrodynamics of operator spreading in interacting integrable lattice models. In these models, operators spread through the ballistic propagation of quasiparticles, with an operator front whose velocity is locally set by the…

统计力学 · 物理学 2018-12-26 Sarang Gopalakrishnan , David A. Huse , Vedika Khemani , Romain Vasseur

Disordered systems under applied loading display slow creep flows at finite temperature, which can lead to the material rupture. Renormalization group arguments predicted that creep proceeds via thermal avalanches of activated events.…

无序系统与神经网络 · 物理学 2024-01-19 Tom W. J. de Geus , Alberto Rosso , Matthieu Wyart