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Combining topology and plasmonics paradigms in nanocolloidal systems may enable new means of pre-engineering desired composite material properties. Here we design and realize orientationally ordered assemblies of noble metal nanoparticles…

软凝聚态物质 · 物理学 2016-12-01 Ye Yuan , Ivan I. Smalyukh

During plastic deformation, metals change shape while continuously becoming stronger. The microscopic origin of these processes lies in the proliferation and movement of line defects, dislocations, and the subsequent self-organisation and…

The atomic structure and physical properties of few-layered <111> oriented diamond nanocrystals (diamanes), covered by hydrogen atoms from both sides are studied using electronic band structure calculations. It was shown that energy…

The optical properties of molecules close to plasmonic nanostructures greatly differ from their isolated molecule counterparts. To theoretically investigate such systems in a Quantum Chemistry perspective, one has to take into account that…

介观与纳米尺度物理 · 物理学 2016-12-26 Silvio Pipolo , Stefano Corni

Motivated by often contradictory literature reports on size dependence of surface energy of gold nanoparticles, we performed an atomistic study combining molecular dynamics and \textit{ab initio} calculations. We show that in the case of Au…

材料科学 · 物理学 2018-03-16 D. Holec , P. Dumitraschkewitz , F. D. Fischer , D. Vollath

Structural changes in a glass due to deformation are subtle and difficult to quantify using conventional imaging and diffraction techniques. Additionally, transmission electron microscopy (TEM) sample preparation using energetic ions often…

We review the development of ultrafast electron nanocrystallography as a method for investigating structural dynamics for nanoscale materials and interfaces. Its sensitivity and resolution are demonstrated in the studies of surface melting…

介观与纳米尺度物理 · 物理学 2015-05-14 Chong-Yu Ruan , Yoshie Murooka , Ramani K. Raman , Ryan A. Murdick , Richard J. Worhatch , Aric Pell

We use molecular dynamics simulations to study the melting of gold icosahedral clusters of a few thousand atoms. We pay particular attention to the behavior of surface atoms, and to the equilibrium shape of the cluster. We find that…

材料科学 · 物理学 2009-11-10 Yanting Wang , S. Teitel , Christoph Dellago

The physical and chemical properties of metal nanoparticles differ significantly from those of free metal atoms as well as from the properties of bulk metals, and therefore, they may be viewed as a transition regime between the two physical…

适应与自组织系统 · 物理学 2007-05-23 Horacio G. Rotstein , Amy Novick-Cohen , Rina Tannenbaum

The magnetic properties of platinum nano-particles ranging in size from a few to up 300 atoms are investigated through first-principle calculations. It is found that the total magnetization depends strongly on the local atomic…

介观与纳米尺度物理 · 物理学 2015-10-01 Cono Di Paola , Roberto D'Agosta , Francesca Baletto

We discuss how simulations of mechanical properties of materials require descriptions at many different length scales --- from the nanoscale where an atomic description is appropriate, through a mesoscale where dislocation based…

材料科学 · 物理学 2007-05-23 J. Schiøtz , T. Vegge , F. D. Di Tolla , K. W. Jacobsen

In metal nanoparticles (NPs) supracrystals, the metallic core provides some key properties, e.g. magnetization, plasmonic response or conductivity, with the ligand molecules giving rise to others like solubility, assembly or interaction…

Nanotechnology and the consequent emergence of miniaturized devices are driving the need to improve our understanding of the mechanical properties of a myriad of materials. Here we focus on amorphous polymeric materials and introduce a new…

Large deformations of soft elastic beads spinning at high angular velocity in a denser background fluid are investigated theoretically, numerically, and experimentally using millimeter-size polyacrylamide hydrogel particles introduced in a…

Spectral dependencies of polarized optical transmission of a metal film with a periodic array of elliptical nanoholes have been studied. Such nanostructured metal films exhibit the enhanced broadband optical transmission which can be…

凝聚态物理 · 物理学 2009-11-10 Jill Elliott , Igor I. Smolyaninov , Nikolay I. Zheludev , Anatoly V. Zayats

Motivated by results of the topological theory of glasses accounting for geometric frustration, we develop the simplest possible continuum mechanical model of defect dynamics in metallic glasses that accounts for topological, energetic, and…

材料科学 · 物理学 2017-04-26 Amit Acharya , Michael Widom

Gold nanorods grafted with short chain polymers are assembled into controlled open structures using polymer-induced depletion interactions and structurally characterized using small angle x-ray scattering. When the nanorod diameter is…

软凝聚态物质 · 物理学 2018-02-13 Ryan Poling-Skutvik , Jonghun Lee , Suresh Narayanan , Ramanan Krishnamoorti , Jacinta C. Conrad

Cells offer numerous inspiring examples where proteins and membranes combine to form complex structures that are key to intracellular compartmentalization, cargo transport, and specialization of cell morphology. Despite this wealth of…

We present a multiscale modeling approach that concurrently couples quantum mechanical, classical atomistic and continuum mechanics simulations in a unified fashion for metals. This approach is particular useful for systems where chemical…

材料科学 · 物理学 2009-11-11 Gang Lu , E. B. Tadmor , Efthimios Kaxiras

Plasmonic nanoparticles resonantly couple to and confine light below the diffraction limit. This mechanism has enabled a modern renaissance in optical materials, with potential applications ranging from sensing and circuitry to renewable…