相关论文: Coherent detection of hidden spin-lattice coupling…
In the rich phases of van der Waals (vdW) materials featuring intertwined electronic order and collective phenomena, characterizing elementary dynamics that entail the low-energy Hamiltonian and electronic degrees of freedom is of paramount…
Emergent cooperative motions of individual degrees of freedom, i.e. collective excitations, govern the low-energy response of system ground states under external stimulations and play essential roles for understanding many-body phenomena in…
We combine polarized infrared magneto-transmission and Faraday angle rotation measurements to map the collective excitations of the van der Waals antiferromagnet FePS$_3$. Below the N\'{e}el temperature ($T_\mathrm{N} \approx 118$ K), the…
We utilize ultrafast photoexcitation to drive coherent lattice oscillations in the layered ferrimagnetic crystal Mn3Si2Te6, which significantly stiffen below the magnetic ordering temperature. We suggest that this is due to an…
FePS3 is a layered van der Waals (vdW) Ising antiferromagnet that has recently been studied in the context of true 2D magnetism, and emerged as an ideal material platform for investigating strong spin-phonon coupling, and non-linear…
Complex chalcogenides in the $M$PS$_3$ family of materials ($M$ = Mn, Fe, Co, and Ni) display remarkably different phase progressions depending upon the metal center orbital filling, character of the P-P linkage, and size of the van der…
Two-dimensional (2D) Van der Waals compounds exhibit interesting electronic and magnetic properties due to complex intra-layer and inter-layer interactions, which are of immense importance in realizing exotic physics as well as advanced…
Magnetic order in van der Waals magnets can strongly influence their lattice dynamics, yet how this interaction manifests across different phonon length scales remains unclear. Optical phonons probe bond-scale exchange modulation and…
Strong coupling between light and elementary excitations is emerging as a powerful tool to engineer the properties of solid-state systems. Spin-correlated excitations that couple strongly to optical cavities promise control over collective…
The magnetic excitations in CoPS$_3$, a two-dimensional van der Waals (vdW) antiferromagnet with spin $S=3/2$ on a honeycomb lattice, has been measured using powder inelastic neutron scattering. Clear dispersive spin waves are observed with…
A coherent THz optical lattice mode is triggered by femtosecond laser pulses in the antiferromagnetic van der Waals semiconductor FePS$_3$. The 380 nm thick exfoliated flake was placed on a substrate and laser-driven lattice and spin…
The hybridization of magnons (spin waves) with phonons, if sufficiently strong and comprising long wavelength excitations, may offer a new playground when manipulating the magnetically ordered systems with light. Applying a magnetic field…
Antiferromagnets display enormous potential in spintronics owing to its intrinsic nature, including terahertz resonance, multilevel states, and absence of stray fields. Combining with the layered nature, van der Waals (vdW) antiferromagnets…
Antiferromagnetic van der Waals family $\rm \textit{M}P\textit{X}_{3}\ (M=Fe,\ Mn,\ Co,\text{ and}\ Ni; X=S\text{ and}\ Se)$ have attracted significant research attention due to the possibility of realizing long-range magnetic order down to…
The layered van der Waals (vdW) ferroelectric CuInP2S6 (CIPS) exhibits unique cation hopping-driven phenomena that bring about unconventional properties with intriguing mechanisms and hold promises for advanced applications in…
The crystal lattice governs the emergent electronic, magnetic, and optical properties of quantum materials, making structural tuning through strain, pressure, or chemical substitution a key approach for discovering and controlling novel…
Two-dimensional van der Waals compounds with magnetic ions on a honeycomb lattice are hosts to a variety of exotic behavior. The magnetic interactions in one such compound, MnPSe$_3$, are investigated with elastic and inelastic neutron…
The $R\mathrm{Te}_3$ ($R = \text{rare earth}$) family of layered van der Waals (vdW) compounds hosts coexisting magnetic and charge density wave (CDW) orders, yet the interplay between these degrees of freedom remains little explored.…
The rapidly growing class of atomically thin and tunable van der Waals materials is intensely investigated both in the context of fundamental science and for new technologies. There is in this connection a widespread need for new ways to…
CoPS3 stands out in the family of the van der Waals antiferromagnets XPS3 (X=Mn, Ni, Fe, Co) due to the unquenched orbital momentum of the magnetic Co2+ ions which is known to facilitate the coupling of spins to both electromagnetic waves…