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Using Ba(Fe$_{0.975}$Co$_{0.025}$)$_2$As$_{2}$ as an exemplar material exhibiting second order electronic-nematic and antiferromagnetic transitions, we present measurements that reveal anomalies in the elastoresistance $\left(\frac{\partial…

There is growing interest in heat pumps based on materials that show thermal changes when phase transitions are driven by changes of electric, magnetic or stress field. Importantly, regeneration permits sinks and loads to be thermally…

材料科学 · 物理学 2019-10-09 S. Crossley , B. Nair , R. W. Whatmore , X. Moya , N. D. Mathur

By using the semi-wet synthesis method, lead-free ferroelectric materials Ba0.9Sr0.1Ti1-xSnxO3 with x = 0, 0.02, 0.05, and 0.10 (abbreviated as BSTS) were prepared and their structural, electric and electrocaloric properties were…

Elastocaloric cooling has been identified as a promising alternative to high global warming potential vapor compression cooling. Two key bottlenecks to adoption are the need for bulky/expensive actuators to provide sufficient uniaxial…

材料科学 · 物理学 2021-05-19 Darin J. Sharar , Joshua Radice , Ronald Warzoha , Brendan Hanrahan , Andrew Smith

The electrocaloric effect (ECE) of BaZr$_{x}$Ti$_{1-x}$O$_3$ (BZT) is closely related to the relaxor state transition of the materials. This work presents a systematic study on the ECE and the state transition of the BZT, using a combined…

Anomalous electrocaloric effect (ECE) with decreasing temperature upon application of an electric field is known to occur in antiferroelectrics (AFEs), and previous understanding refers to the field-induced canting of electric dipoles if…

材料科学 · 物理学 2022-12-28 Ningbo Fan , Jorge Íñiguez , L. Bellaiche , Bin Xu

The electrocaloric effect (ECE) in BaTiO3 is simulated using two different first-principles based effective Hamiltonian molecular dynamics methods. The calculations are performed for a wide range of temperatures (30--900 K) and external…

材料科学 · 物理学 2013-11-12 Takeshi Nishimatsu , Jordan A. Barr , Scott P. Beckman

The existence and feasibility of the multicaloric, polycrystalline material 0.8Pb(Fe1/2Nb1/2)O3-0.2Pb(Mg1/2W1/2)O3, exhibiting magnetocaloric and electrocaloric properties, are demonstrated. Both the electrocaloric and magnetocaloric…

Using the previously developed model we study the electrocaloric effect (ECE) in antiferroelectric crystals of squaric acid. At low temperatures, the polarization reorientation by the electric field applied along the crystallographic $a$…

材料科学 · 物理学 2023-03-15 A. P. Moina

Lead-free BaTi0.89Sn0.11O3 (BTSn) ceramic was elaborated via a solid-state reaction method and its dielectric, ferroelectric, energy storage, electromechanical as well as electrocaloric properties were investigated at 25 kV/cm. Pure…

Ferroelectricity at room temperature has been demonstrated in nanometer-thin quasi 2D croconic acid thin films, by the polarization hysteresis loop measurements in macroscopic capacitor geometry, along with observation and manipulation of…

We report on calorimetry under applied hydrostatic pressure and magnetic field at the antiferromagnetic (AFM)-ferromagnetic (FM) transition of Fe$_{49}$Rh$_{51}$. Results demonstrate the existence of a giant barocaloric effect in this…

Multiferroic materials have undergone extensive research in the past two decades in an effort to produce a sizable room-temperature magneto-electric (ME) effect in either exclusive or composite materials for use in a variety of electronic…

First-principles-based atomistic simulations are used to reveal ferroelectric phases and phase transitions induced in a semiconductor ferroelectric, CsGeBr$_3$, by external loads: hydrostatic pressure, uniaxial and biaxial stresses, and…

材料科学 · 物理学 2024-03-18 Joshua Townsend , Ravi Kashikar , S. Lisenkov , I. Ponomareva

While BiFeO3-based solid solutions show great promise for applications in energy conversion and storage, realizing this promise necessitates understanding the structure-property relationship in particular pertaining to the relaxor-like…

The electroviscous effect deals with the change in the viscosity of fluids due to an external electric field. Here, we report experimental studies on the electroviscous effects in a ferroelectric nematic liquid crystal. It was synthesised…

软凝聚态物质 · 物理学 2023-03-21 M. Praveen Kumar , Jakub Karcz , Przemyslaw Kula , Smarajit Karmakar , Surajit Dhara

Studying the response of materials to strain can elucidate subtle properties of electronic structure in strongly correlated materials. So far, mostly the relation between strain and resistivity, the so called elastoresistivity, has been…

Two-dimensional materials hosting ferroelectricity and ferromagnetism are crucial for low-power and high-speed information processing technologies. However, intrinsic 2D multiferroics in the monolayer limit are rare. Here, we demonstrate…

介观与纳米尺度物理 · 物理学 2023-10-25 Imran Ahamed , Atasi Chakraborty , Pushpendra Yadav , Rik Dey , Yogesh Singh Chauhan , Somnath Bhowmick , Amit Agarwal

Modelling elastocaloric effect (eCE) is crucial for the design of environmentally friendly and energy-efficient eCE based solid-state cooling devices. Here, a thermodynamically consistent non-isothermal phase-field model (PFM) coupling…

材料科学 · 物理学 2023-03-10 Wei Tang , Qihua Gong , Min Yi , Bai-Xiang Xu , Long-Qing Chen

The magneto-electrocaloric effect which can be defined as the coupling between magnetocaloric and electrocaloric effects attracts currently considerable attention due to the advantages provided by the caloric effect in designing solid-state…