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Neutron spectroscopy measurements have been performed on single crystals of the antiferromagnetic van der Waals compound NiPS$_3$. Linear spin wave theory using a Heisenberg Hamiltonian with single-ion anisotropies has been applied to…

强关联电子 · 物理学 2022-12-19 A. R. Wildes , J. R. Stewart , M. D. Le , R. A. Ewings , K. C. Rule , G. Deng , K. Anand

In the Van der Waal material $\rm NiPS_3$, Ni atoms have spin S=1 and realize a honeycomb lattice. Six sulfur atoms surround each Ni and split their d manifold into three filled and two unfilled bands. Aimed to determine the spin…

强关联电子 · 物理学 2023-12-14 Paula Mellado

Neutron inelastic scattering has been used to measure the magnetic excitations in powdered NiPS$_3$, a quasi-two dimensional antiferromagnet with spin $S = 1$ on a honeycomb lattice. The spectra show clear, dispersive magnons with a $\sim…

材料科学 · 物理学 2018-10-17 D. Lançon , R. A. Ewings , T. Guidi , F. Formisano , A. R. Wildes

Using inelastic neutron scattering technique, we measured the spin wave dispersion over the entire Brillouin zone of room temperature multiferroic BiFeO3 single crystals with magnetic excitations extending to as high as 72.5 meV. The full…

The spin waves in single crystals of the layered van der Waals antiferromagnet CoPS$_3$ have been measured using inelastic neutron scattering. The data show four distinct spin wave branches with large ($\gtrsim 14$ meV) energy gaps at the…

材料科学 · 物理学 2023-03-08 A. R. Wildes , B. Fåk , U. B. Hansen , M. Enderle , J. R. Stewart , L. Testa , H. M. Rønnow , C. Kim , Je-Geun Park

The magnetic excitations in CoPS$_3$, a two-dimensional van der Waals (vdW) antiferromagnet with spin $S=3/2$ on a honeycomb lattice, has been measured using powder inelastic neutron scattering. Clear dispersive spin waves are observed with…

Two-dimensional van der Waals compounds with magnetic ions on a honeycomb lattice are hosts to a variety of exotic behavior. The magnetic interactions in one such compound, MnPSe$_3$, are investigated with elastic and inelastic neutron…

强关联电子 · 物理学 2021-01-20 S. Calder , A. V. Haglund , A. I. Kolesnikov , D. Mandrus

Despite extensive research, the precise spin Hamiltonian of the van der Waals antiferromagnet NiPS$_3$ -- which hosts a zigzag-ordered ground state -- remains debated. While consensus has emerged on ferromagnetic nearest-neighbor ($J_1$)…

强关联电子 · 物理学 2026-03-27 Qiang Luo , Shuhang Yang , Xiaoying Wang , Zhengyu Jiang , Chunlan Ma , Yan Zhu

Antiferromagnetic van der Waals family $\rm \textit{M}P\textit{X}_{3}\ (M=Fe,\ Mn,\ Co,\text{ and}\ Ni; X=S\text{ and}\ Se)$ have attracted significant research attention due to the possibility of realizing long-range magnetic order down to…

We calculate the magnon dispersion spectra of the two-dimensional zigzag van der Waals antiferromagnet NiPS$_3$ for monolayer, bilayer, and bulk systems as a function of an external magnetic field. We calculate the exchange and anisotropy…

Van der Waals materials hosting Kitaev interactions are promising platforms for exploring exotic quantum phenomena. Here, we report inelastic neutron scattering investigations of the van der Waals antiferromagnet VBr3, which forms a…

强关联电子 · 物理学 2026-03-03 Zeyu Kao , Yimeng Gu , Yiqing Gu , Hao Zhang , Shiyi Zheng , Naoki Murai , Seiko Ohira-Kawamura , Jun Zhao

FePS$_3$ is a van der Waals compound with a honeycomb lattice that is a good example of a two-dimensional antiferromagnet with Ising-like anisotropy. Neutron spectroscopy data from FePS3 were previously analysed using a straight-forward…

材料科学 · 物理学 2020-07-15 A. R. Wildes , M. E. Zhitomirsky , T. Ziman , D. Lançon , H. C. Walker

Inelastic neutron scattering is used to study the magnetic excitations of the $S=1$ square-lattice antiferromagnet La$_2$NiO$_4$. We find that the spin waves cannot be described by a simple classical (harmonic) Heisenberg model with only…

A neutron scattering study of the Mott-Hubbard insulator LaTiO$_{3}$ (T$_{{\rm N}}=132$ K) reveals a spin wave spectrum that is well described by a nearest-neighbor superexchange constant $J=15.5$ meV and a small Dzyaloshinskii-Moriya…

强关联电子 · 物理学 2009-10-31 B. Keimer , D. Casa , A. Ivanov , J. W. Lynn , M. v. Zimmermann , J. P. Hill , D. Gibbs , Y. Taguchi , Y. Tokura

We present inelastic neutron scattering measurements of the antiferromagnetic insulator CaMn$_2$Sb$_2$, which consists of corrugated honeycomb layers of Mn. The dispersion of magnetic excitations has been measured along the H and L…

We performed an inelastic neutron scattering experiment on a polycrystalline sample of a helimagnet Ni$_2$InSbO$_6$ to construct the spin Hamiltonian. Well-defined spin-wave excitation with a band energy of 20 meV was observed below $T_{N}…

强关联电子 · 物理学 2023-03-08 Zheyuan Liu , Taka-hisa Arima , Shinichi Itoh , Shinichiro Asai , Takatsugu Masuda

We report inelastic neutron scattering measurements on Na2IrO3, a candidate for the Kitaev spin model on the honeycomb lattice. We observe spin-wave excitations below 5 meV with a dispersion that can be accounted for by including…

We present the magnetic excitation spectrum of the quantum magnet $\rm NiPS_3$ near the zig-zag ground state of a minimal honeycomb spin Hamiltonian that includes bilinear and biquadratic spin interactions. Our analysis, using a multi-boson…

强关联电子 · 物理学 2024-10-29 Paula Mellado , Mauricio Sturla

We performed inelastic neutron scattering experiments on single crystal samples of a linear magnetoelectric material Mn$_{3}$Ta$_{2}$O$_{8}$, which exhibits a collinear antiferromagnetic order, to reveal the spin dynamics. Numerous modes…

An inelastic neutron scattering study of the spin waves corresponding to the stripe antiferromagnetic order in insulating Rb$_{0.8}$Fe$_{1.5}$S$_2$ throughout the Brillouin zone is reported. The spin wave spectra are well described by a…

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