相关论文: Simultaneous field-free molecular orientation and …
Polarized atomic ensembles play a crucial role in precision measurements. We demonstrate a novel method of creating atomic polarization in an alkali vapor in a continuous-wave regime. The method relies on a combination of optical pumping by…
We have studied the formation of ultracold RbSr molecules with laser pulses. After discussing the advantages of the Mott insulator phase for the control with pulses, we present two classes of strategies. The first class involves two…
The recent demonstration of a terahertz (THz) molecular gas laser pumped by a mid-infrared quantum cascade laser (QCL) has opened up new perspectives for this family of sources, traditionally relying on CO2-laser pumping. A so far open…
The spectrum of terahertz (THz) emission in gases via ionizing two-color femtosecond pulses is analyzed by means of a semi-analytic model and finite-difference-time-domain simulations in 1D and 2D geometries. We show that produced THz…
Due to electronic many-body effects, the ionization of a molecule can trigger ultrafast electron dynamics appearing as a migration of the created hole charge throughout the system. Here we propose a scheme for control of the charge…
Optical pumping of excited exciton states in semiconductor quantum wells is a tool for realisation of ultra-compact terahertz (THz) lasers based on stimulated optical transition between excited (2p) and ground (1s) exciton state. We show…
The methods producing cold molecules from cold atoms tend to leave molecular ensembles with substantial residual internal energy. For instance, Cs2 molecules initially formed via photoassociation of cold Cs atoms are in several vibrational…
Raman laser pulses are used to induce coherent tunnelling between neighbouring sites of a vertical 1D optical lattice. Such tunneling occurs when the detuning of a probe laser from the atomic transition frequency matches multiples of the…
A method for decelerating a continuous beam of neutral polar molecules is theoretically demonstrated. This method utilizes non-uniform, static electric fields and regions of adiabatic population transfer to generate a mechanical force that…
A general method for rotational microwave spectroscopy and control of polar molecular ions via direct microwave addressing is considered. Our method makes use of spatially varying AC Stark shifts, induced by far off-resonant, focused laser…
The advent of ultrafast science with pulsed electron beams raised the need in controlling the temporal features of the electron pulses. One promising suggestion is the nano-selective quantum optics with multi-electrons, which scales…
We present a theoretical study of the mixed-field orientation of molecules without rotational symmetry. The time-dependent one-dimensional and three-dimensional orientation of a thermal ensemble of 6-chloropyridazine-3-carbonitrile…
The directional control of molecular dissociation with the laser electric field waveform is a paradigm and was demonstrated for a variety of molecules. In most cases, the directional control occurs via a dissociative ionization pathway. The…
We present some approaches to the computation of ultra-fast laser pulses capable of selectively breaking molecular bonds. The calculations are based on a mixed quantum-classical description: The electrons are treated quantum mechanically…
A scheme for polarization control using two laser beams in a non-linear optical medium is studied using both co- and counter-propagating beam geometries. In particular, we show that under certain conditions it is possible for two laser…
We demonstrate experimentally a method of all-optical selective rotational control in gas mixtures. Using an optical centrifuge - an intense laser pulse whose linear polarization rotates at an accelerated rate, we simultaneously excite two…
Applications ranging from nonlinear terahertz spectroscopy to remote sensing require broadband and intense THz radiation which can be generated by focusing two-color laser pulses into a gas. In this setup, THz radiation originates from the…
Combining the features of molecular wires and femtosecond laser pulses gives the unique opportunity to optically switch electron currents in molecular devices with very high speed. Based on a weak-coupling approximation between wire and…
The extremely high power densities and short durations of single pulses of x-ray free electron lasers (XFELs) have opened new opportunities in atomic physics, where complex excitation-relaxation chains allow for high ionization states in…
Multimode optical fibers have seen increasing applications in communication, imaging, high-power lasers and amplifiers. However, inherent imperfections and environmental perturbations cause random polarization and mode mixing, making the…