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We consider cold polar molecules confined in a helical optical lattice similar to those used in holographic microfabrication. An external electric field polarizes molecules along the axis of the helix. The large-distance inter-molecular…

其他凝聚态物理 · 物理学 2009-11-13 K. T. Law , D. E. Feldman

Molecules with their axes sharply confined in space, available through laser-induced alignment methods, are essential for many current experiments, including ultrafast molecular imaging. Most of these applications require both that the…

Ultracold molecules, because of their rich internal structures and interactions, have been proposed as a promising platform for quantum science and precision measurement. Direct laser-cooling promises to be a rapid and efficient way to…

原子物理 · 物理学 2024-06-18 Yukai Lu , Samuel J. Li , Connor M. Holland , Lawrence W. Cheuk

Ultracold molecules trapped in optical tweezers show great promise for the implementation of quantum technologies and precision measurements. We study a prototypical scenario where two interacting polar molecules placed in separate traps…

Laser control of molecular rotation is an area of active research. A number of recent studies has aimed at expanding the reach of rotational control to extreme, previously inaccessible rotational states, as well as controlling the…

量子物理 · 物理学 2015-01-13 V. Milner , J. W. Hepburn

Advances of quantum control technology have led to nearly perfect single-qubit control of nuclear spins and atomic hyperfine ground states. In contrast, quantum control of strong optical transitions, even for free atoms, are far from being…

原子物理 · 物理学 2020-06-24 Yudi Ma , Xing Huang , Xiaoqing Wang , Lingjing Ji , Yizun He , Liyang Qiu , Jian Zhao , Yuzhuo Wang , Saijun Wu

Machine learning for predicting control landscape maps of full quantum molecular dynamics is examined through a case study of the laser-induced three-dimensional (3D) alignment of asymmetric top molecules, an essential technique for…

化学物理 · 物理学 2024-12-03 Tomotaro Namba , Yukiyoshi Ohtsuki

We present a novel approach to precisely synthesize arbitrary polarization states of light with a high modulation bandwidth. Our approach consists of superimposing two laser light fields with the same wavelength, but with opposite circular…

We study the nonlinear and resonant process of two-photon ionization of atoms (He and H) in a pump-probe scheme. The pump pulse prepares the quantum system in a superposition of the ground state and an excited bound state. By varying the…

We present an analysis of two experimental approaches to controlling the directionality of molecular rotation with ultrashort laser pulses. The two methods are based on the molecular interaction with either a pair of pulses (a "double kick"…

光学 · 物理学 2015-06-11 C. Bloomquist , S. Zhdanovich , A. A. Milner , V. Milner

Recent molecular dynamics simulations show that thermal gradients can induce electric fields in water that are comparable in magnitude to electric fields seen in ionic thin films and biomembranes. This surprising non-equilibrium phenomenon…

统计力学 · 物理学 2016-12-09 Alpha A. Lee

How fast can a laser pulse ionize an atom? We address this question by considering pulses that carry a fixed time-integrated energy per-area, and finding those that achieve the double requirement of maximizing the ionization that they…

原子物理 · 物理学 2017-06-07 David Kammerlander , Alberto Castro , Miguel A. L. Marques

We show that congruent electric, magnetic and non-resonant optical fields acting concurrently on a polar paramagnetic (and polarisable) molecule offer possibilities to both amplify and control the directionality of the ensuing molecular…

化学物理 · 物理学 2016-01-12 Ketan Sharma , Bretislav Friedrich

Recently, laser cooling methods have been extended from atoms to molecules. The complex rotational and vibrational energy level structure of molecules makes laser cooling difficult, but these difficulties have been overcome and molecules…

原子物理 · 物理学 2019-02-18 M. R. Tarbutt

Complete control of single-electron states in a two-dimensional semiconductor quantum-ring model is established, opening a path into coherent laser-driven single-gate qubits. The control scheme is developed in the framework of optimal…

其他凝聚态物理 · 物理学 2008-05-08 E. Rasanen , A. Castro , J. Werschnik , A. Rubio , E. K. U. Gross

The generation of optically coherent ultrashort pulses by mode-locked lasers has revolutionized advancements in modern science and technology. These pulses often arise from the formation of dissipative solitons, which emerge due to a…

光学 · 物理学 2025-05-08 Jesús Yelo-Sarrión , François Leo , Simon-Pierre Gorza

Due to their rich level structure, molecules are well-suited for probing time variation of fundamental constants, precisely measuring parity violation and time-reversal non-invariance effects, studying quantum mechanical aspects of chemical…

量子物理 · 物理学 2015-05-30 S. Ding , D. N. Matsukevich

A scheme is proposed to achieve substantial controllable phase modulation for a probe field propagating through a thermal atomic vapor in double-$\Lambda$ configuration. The phase modulation is based on the linear susceptibility of the…

量子物理 · 物理学 2015-06-19 Lida Zhang , Jörg Evers

We proposed a general Zeeman slower scheme applicable to the majority of the laser-coolable molecules. Different from previous schemes, the key idea of our scheme lies in that the compensation of the detuning with the magnetic field is done…

原子物理 · 物理学 2019-11-13 Qian Liang , Wenhao Bu , Yuhe Zhang , Tao Chen , Bo Yan

We demonstrate full quantum state control of two species of single atoms using optical tweezers and assemble the atoms into a molecule. Our demonstration includes 3D ground-state cooling of a single atom (Cs) in an optical tweezer,…