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We discuss the mechanism of coherent phonon generation by Stimulated Ionic Raman Scattering, a process different from conventional excitation with near visible optical pulses. Ionic Raman scattering is driven by anharmonic coupling between…

超导电性 · 物理学 2015-05-25 R. Mankowsky , M. Först , T. Loew , J. Porras , B. Keimer , A. Cavalleri

We have applied femtosecond pump-probe technique with variable pump wavelength to study coherent lattice dynamics in Bi single crystal. Comparison of the coherent amplitude as a function of pump photon energy for two different in symmetry…

材料科学 · 物理学 2015-05-20 A. A. Melnikov , O. V. Misochko , S. V. Chekalin

Cuprate superconductors host a multitude of low-energy optical phonons. Using time- and angle-resolved photoemission spectroscopy, we study coherent phonons in Bi$_{2}$Sr$_{2}$Ca$_{0.92}$Y$_{0.08}$Cu$_{2}$O$_{8+\delta}$. Sub-meV modulations…

强关联电子 · 物理学 2019-05-07 S. -L. Yang , J. A. Sobota , Y. He , D. Leuenberger , H. Soifer , H. Eisaki , P. S. Kirchmann , Z. -X. Shen

We examine coherent phonons in a strongly driven sample of optimally-doped high temperature superconductor YBa$_2$Cu$_3$O$_{7-\delta}$. We observe a non-linear lattice response of the 4.5\,THz copper-oxygen vibrational mode at high…

Optical excitation in the cuprates has been shown to induce transient superconducting correlations above the thermodynamic transition temperature, $T_C$, as evidenced by the terahertz frequency optical properties in the non-equilibrium…

超导电性 · 物理学 2020-03-25 B. Liu , M. Först , M. Fechner , D. Nicoletti , J. Porras , T. Loew , B. Keimer , A. Cavalleri

We report on the impulsive generation of coherent optical phonons in CdTe0.68Se0.32 nanocrystallites embedded in a glass matrix. Pump probe experiments using femtosecond laser pulses were performed by tuning the laser central energy to…

介观与纳米尺度物理 · 物理学 2009-11-10 A. V. Bragas , C. Aku-Leh , S. Costantino , Alka Ingale , J. Zhao , R. Merlin

We investigate the structural modulations induced by optical excitation of a polar phonon mode in YBa$_2$Cu$_3$O$_7$, using first-principles calculations based on density functional theory. We focus on the intense-excitation regime in which…

超导电性 · 物理学 2016-10-26 Michael Fechner , Nicola A. Spaldin

We report results of inelastic neutron scattering measurements of phonon dispersions in optimally doped YBa2Cu3O6.95 and compare them with model calculations. The focus is on the in-plane oxygen bond-stretching phonon branches. The study of…

强关联电子 · 物理学 2009-11-10 L. Pintschovius , D. Reznik , W. Reichardt , Y. Endoh , H. Hiraka , J. M. Tranquada , H. Uchiyama , T. Masui , S. Tajima

Time resolved measurements provide a new way to disentangle complex interactions in quantum materials due to their different timescales. We used pump-probe Raman scattering to investigate the apical oxygen vibration in…

超导电性 · 物理学 2021-12-07 N. Pellatz , S. Roy , J-W. Lee , J. L. Schad , H. Kandel , N. Arndt , C. B. Eom , A. F. Kemper , D. Reznik

We present a Raman scattering study of Ca$_2$RuO$_4$, in which we investigate the temperature-dependence of the lattice dynamics and the electron-phonon interaction below the metal-insulator transition temperature ({\it T}$_{\rm MI}$).…

强关联电子 · 物理学 2009-11-11 H. Rho , S. L. Cooper , S. Nakatsuji , H. Fukazawa , Y. Maeno

A systematic Raman study in the visible carried out on the YBa2Cu316,18Ox (x=6-7) compounds, with isotopic substitution of 18O for 16O, has detected a doping dependent deviation from harmonic behavior for the frequency shift of the in-phase…

超导电性 · 物理学 2017-11-22 E. Liarokapis

We report on a photo-induced transient state of YBa2Cu2O6+x in which transport perpendicular to the Cu-O planes becomes highly coherent. This effect is achieved by excitation with mid-infrared optical pulses, tuned to the resonant frequency…

超导电性 · 物理学 2014-06-04 S. Kaiser , C. R. Hunt , D. Nicoletti , W. Hu , I. Gierz , H. Y. Liu , M. Le Tacon , T. Loew , D. Haug , B. Keimer , A. Cavalleri

In ionic Raman scattering, infrared-active phonons mediate a scattering process that results in the creation or destruction of a Raman-active phonon. This mechanism relies on nonlinear interactions between phonons and has in recent years…

We investigate coherent phonon oscillations of BaFe$_2$As$_2$ using optical pump-probe spectroscopy. Time-resolved optical reflectivity shows periodic modulations due to $A_{1g}$ coherent phonon of $c$-axis arsenic vibrations. Optical probe…

Excitation of four coherent phonon modes of different symmetries has been realized in copper metaborate CuB$_2$O$_4$ via impulsive stimulated Raman scattering (ISRS). Phonons were detected by monitoring changes in the linear optical…

The lattice dynamics of Ba$_2$CuGe$_2$O$_7$, a compound which develops Dzyaloshinsky-Moriya (DM) helical magnetism below $T_N$ = 3.2 K, has been studied by measuring the infrared reflectivity of a single crystal with the radiation polarized…

We present a systematic study of the interplay between lattice parameters and the energy of the optical phonons as well as the antiferromagnetic coupling strength, $J$, in the high-$T_{\text{c}}$ superconducting cuprate…

Signatures of photo-induced superconductivity have been reported in cuprate materials subjected to a coherent phonon drive. A 'cold' superfluid was extracted from the transient Terahertz conductivity and was seen to coexist with 'hot'…

Nonlinear processes involving frequency-mixing of light fields set the basis for ultrafast coherent spectroscopy of collective modes in solids. In certain semimetals and semiconductors, generation of coherent phonon modes can occur by a…

Quantum coherent coupling between a zone-center phonon and two acoustic phonons was observed in two GaAs/AlAs superlattices (8 nm/8 nm and 5.4 nm/5.4 nm) at ambient temperature. Using degenerate coherent phonon spectroscopy, a multi-cycle…

材料科学 · 物理学 2019-07-25 Feng He , Nathanial Sheehan , Seth R Bank , Raymond L Orbach , Yaguo Wang
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