相关论文: Fundamental Investigation of Reactive-Convective T…
We present the first experiments of dissolution-driven convection of carbon dioxide (CO$_2$) in a confined brine-saturated porous medium at high pressures. We designed a novel Hele-Shaw cell that allows for both visual and quantitative…
Convective dissolution is the process by which CO$_2$ injected in deep geological formations dissolves into the aqueous phase, which allows storing it perennially by gravity. The process results from buoyancy-coupled Darcy flow and solute…
Geological storage of CO$_2$ in deep saline aquifers is a promising measure to mitigate global warming by reducing the concentration of this greenhouse gas in the atmosphere. When CO$_2$ is injected in the geological formation, it dissolves…
We consider experimentally the instability and mass transport of a porous-medium flow in a Hele-Shaw geometry. In an initially stable configuration, a lighter fluid (water) is located over a heavier fluid (propylene glycol). The fluids mix…
We numerically examine solutal convection in porous media, driven by the dissolution of carbon dioxide (CO2) into water---an effective mechanism for CO2 storage in saline aquifers. Dissolution is associated with slow diffusion of free-phase…
Carbon dioxide (CO$_2$) sequestration in saline aquifers has been introduced as one of the most practical, long-term, and safe solutions to tackle a growing threat originating from the emission of CO$_2$. Successfully executing and planning…
We investigate the convective instability resulting from the dissolution of carbon dioxide (CO$_{2}$) into water in a heterogeneous Hele-Shaw cell utilizing both experimental and numerical approaches. Experiments are conducted in a…
The dissolution and subsequent mass transfer of carbon dioxide gas into liquid barriers plays a vital role in many environmental and industrial applications. In this work, we study the downward dissolution and propagation dynamics of CO2…
We consider the process of convective dissolution in homogeneous and isotropic porous media. The flow is unstable due to the presence of a solute that induces a density difference responsible for driving the flow. The mixing dynamics is…
We combine modeling and measurements to investigate the dynamics of convective carbon dioxide (CO$_2$) dissolution in a pressure-volume-temperature cell, extending a recent study by Wen et al. (J. Fluid Mech., vol. 854, 2018, pp. 56--87) at…
We perform large-scale numerical simulations of convection in 3D porous media at Rayleigh-Darcy numbers up to $Ra=8\times10^4$. To investigate the convective mixing of carbon dioxide (CO$_2$) in geological formations, we consider a…
The partial differential equations describing immiscible, but soluble, carbon dioxide (CO2) displacement of brine are developed including local mass-transfer effects. Scaling relationships for characteristic time among laboratory and…
Motivated by geological carbon dioxide (CO$_2$) storage, many recent studies have investigated the fluid dynamics of solutal convection in porous media. Here we study the convective dissolution of CO$_2$ in a closed system, where the…
One of the key risks for a Carbon Capture Storage (CCS) is injectivity decline. Evaporation of the connate brine in near-wellbore region during CO2 injection may result in drying-up the rock yielding the mobilisation and migration of clay…
We present time-resolved pore-scale experiments in which CO2-saturated brine was injected into a water-wet Ketton limestone sample containing residual hydrocarbon under reservoir conditions (8 MPa, 50 {\deg}C) and monitored by 4D X-ray…
Chemical reactions can accelerate, slow down or even be at the very origin of the development of dissolution-driven convection in partially miscible stratifications, when they impact the density profile in the host fluid phase. We…
Pools of carbon dioxide are found in natural geological accumulations and in engineered storage in saline aquifers. It has been thought that once this CO2 dissolves in the formation water, making it denser, convection streams will transport…
Depleted carbonate hydrocarbon reservoirs are promising sites for geological CO2 storage, yet the presence of residual hydrocarbons introduces complex pore-scale interactions that influence the dynamics of solid dissolution. This study…
Subsurface sequestration of CO2 has received attention from the global scientific community in response to climate change concerns due to higher concentrations of CO2 in the atmosphere. Mathematical models have thus been developed to aid…
Diffusive transport has implications for the long-term status of underground storage of hydrogen (H$_2$) fuel and carbon dioxide (CO$_2$), technologies which are being pursued to mitigate climate change and advance the energy transition.…