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Measured photoionization time delays may exhibit large variations as a function of the emission angles, even for spherically symmetric targets, as shown in recent RABBITT (reconstruction of attosecond beating by interference of two-photon…

原子物理 · 物理学 2022-12-29 D. I. R. Boll , L. Martini , A. Palacios , O. A. Fojón

Attosecond ionization time-delays at photoelectron energies above typically 10 eV are usually interpreted using the so called asymptotic approximation as a sum of the atomic or molecular delays with a universal laser-induced contribution.…

We employ the recently developed multi-photon R-matrix method for molecular above-threshold photoionization to obtain second-order ionization amplitudes that govern the interference in RABITT experiments. This allows us to extract RABITT…

原子物理 · 物理学 2022-05-03 Jakub Benda , Zdeněk Mašín , Jimena D. Gorfinkiel

Phase and time delays of atomic above-threshold ionization are usually experimentally explored by the reconstruction of attosecond harmonic beating by interference of two-photon transitions (RABBIT) technique. Theoretical studies of RABBIT…

原子物理 · 物理学 2024-03-25 Sebastián D. López , Matias L. Ocello , Diego G. Arbó

We describe in detail how attosecond delays in laser-assisted photoionization can be computed using perturbation theory based on two-photon matrix elements. Special emphasis is laid on above-threshold ionization, where the electron…

原子物理 · 物理学 2015-06-19 J. M. Dahlström , E. Lindroth

We utilize the reconstruction of attosecond beating by interference of two-photon transitions (RABBIT) technique to study the phase of a Rabi-cycling atom using circularly polarized extreme ultraviolet and infrared (IR) fields, where the IR…

原子物理 · 物理学 2024-01-31 Yijie Liao , Edvin Olofsson , Jan Marcus Dahlström , Liang-Wen Pi , Yueming Zhou , Peixiang Lu

Reconstruction of Attosecond Beating By Interference of Two-photon Transitions (RABBITT) is a technique that can be used to determine the phases of atomic transition elements in photoionization processes. In the traditional RABBITT scheme,…

Recent angle-resolved RABBITT experiments have shown that the photoionization time delay depends on the emission angle of the photoelectron. In this work we demonstrate that for photoemission from helium accompanied by shake-up (correlation…

原子物理 · 物理学 2020-09-30 Stefan Donsa , Manuel Ederer , Renate Pazourek , Joachim Burgdörfer , Iva Březinová

We study experimentally the influence of the intensity of the infrared (IR) probe field on attosecond pulse train (APT) phase measurements performed with the RABITT method (Reconstruction of Attosecond Beating by Interference in Two-Photon…

原子物理 · 物理学 2009-07-22 M. Swoboda , J. M. Dahlstrom , T. Ruchon , P. Johnsson , J. Mauritsson , K. J. Schafer , A. L'Huillier

Following up on a recent paper [Bharti et al., Phys. Rev. A 109 (2024) 023110], we compare the predictions from severalR-matrix with time-dependence calculations for a modified three-sideband version of the "reconstruction of attosecond…

原子物理 · 物理学 2024-04-05 A. T. Bondy , J. C. del Valle , S. Saha , K. R. Hamilton , D. Bharti , A. Harth , K. Bartschat

The reconstruction of attosecond beating by interference of two-photon transitions (RABBIT) is one of the most widely used techniques for obtaining both the relative phases of harmonics forming an attosecond pulse train and the phase of…

光学 · 物理学 2023-09-13 R. E. F. Silva , Á. Jiménez-Galán

We present a theoretical study of the photoelectron attosecond beating at the basis of RABBIT (Reconstruction of Attosecond Beating By Interference of Two-photon transitions) in the presence of autoionizing states. We show that, as a…

原子物理 · 物理学 2015-01-14 Álvaro J. Galán , Luca Argenti , Fernando Martín

Reconstruction of attosecond beating by interference of two-photon transitions (RABBITT) is a powerful photoelectron spectroscopy, offering direct access to internal dynamics of the target. It is being increasingly applied to molecular…

化学物理 · 物理学 2023-04-10 Serguei Patchkovskii , Jakub Benda , Dominik Ertel , David Busto

We study laser-assisted photodetachment time delays by attosecond pulse trains from the closed-shell negative ions F- and Cl-. We investigate the separability of the delay into two contributions: (i) the Wigner-like delay associated with…

原子物理 · 物理学 2017-09-13 Eva Lindroth , Jan Marcus Dahlström

The Wigner delay is defined as the energy derivative of the scattering phase of a particle in a given potential, unveiling the time taken (or gained) due to the interaction. The characterisation of this delay plays a central role in…

Parity mixing in photoionization, i.e. when emitted electrons have different parities but the same energy, causes interference observable only in angle-resolved measurements. The interference typically manifests as a symmetry violation in…

原子物理 · 物理学 2026-04-20 Maria M. Popova , Sergei N. Yudin , Alexei N. Grum-Grzhimailo , Elena V. Gryzlova

We report a joint experimental and theoretical study of a three-sideband (3-SB) modification of the "reconstruction of attosecond beating by interference of two-photon transitions" (RABBIT) setup. The 3-SB RABBIT scheme makes it possible to…

原子物理 · 物理学 2023-01-24 D Bharti , H Srinivas , F Shobeiry , K R Hamilton , R Moshammer , T Pfeifer , K Bartschat , A Harth

We develop a novel technique for modeling of atomic and molecular ionization in superposition of XUV and IR fields with characteristics typical for attosecond streaking and RABBITT experiments. The method is based on solving the…

原子物理 · 物理学 2016-06-29 Vladislav V. Serov , A. S. Kheifets

We report on a novel method for photo-association of strongly polar trilobite Rydberg molecules. This exotic ultralong-range dimer, consisting of a ground-state atom bound to the Rydberg electron via electron-neutral scattering, inherits…

We investigate a possible mechanism for the autoionization of ultracold Rydberg gases, based on the resonant coupling of Rydberg pair states to the ionization continuum. Unlike an atomic collision where the wave functions begin to overlap,…

原子物理 · 物理学 2015-05-13 T. Amthor , J. Denskat , C. Giese , N. N. Bezuglov , A. Ekers , L. Cederbaum , M. Weidemüller
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