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Carrier spins in semiconductor nanocrystals are promising candidates for quantum information processing. Using a combination of time-resolved Faraday rotation and photoluminescence spectroscopies, we demonstrate optical spin polarization…

Benefiting from both molecular tunability and versatile methods for deployment, optically interfaced molecular spins are a promising platform for quantum technologies such as sensing and imaging. Room-temperature optically detected coherent…

Future communication and computation technologies that exploit quantum information require robust and well-isolated qubits. Electron spins in III-V semiconductor quantum dots, while promising candidates, see their dynamics limited by…

Optically active defects in solids with accessible spin states are promising candidates for solid state quantum information and sensing applications. To employ these defects as quantum building blocks, coherent manipulation of their spin…

Solid-state spins are promising as interfaces from stationary qubits to single photons for quantum communication technologies. Semiconductor quantum dots have excellent optical coherence, exhibit near unity collection efficiencies when…

Quantum networks and sensing require solid-state spin-photon interfaces that combine single-photon generation and long-lived spin coherence with scalable device integration, ideally at ambient conditions. Despite rapid progress reported…

Realization of devices based on quantum laws might lead to building processors that outperform their classical analogues and establishing unconditionally secure communication protocols. Solids do usually present a serious challenge to…

For the realisation of scalable solid-state quantum-bit systems, spins in semiconductor quantum dots are promising candidates. A key requirement for quantum logic operations is a sufficiently long coherence time of the spin system.…

介观与纳米尺度物理 · 物理学 2015-05-14 T. Korn , M. Kugler , M. Griesbeck , R. Schulz , A. Wagner , M. Kubová , C. Gerl , D. Schuh , W. Wegscheider , C. Schüller

Single electron spins in semiconductor quantum dots (QDs) are a versatile platform for quantum information processing, however controlling decoherence remains a considerable challenge. Recently, hole spins have emerged as a promising…

Quantum computation requires many qubits that can be coherently controlled and coupled to each other. Qubits that are defined using lithographic techniques are often argued to be promising platforms for scalability, since they can be…

介观与纳米尺度物理 · 物理学 2020-04-27 L. Petit , H. G. J. Eenink , M. Russ , W. I. L. Lawrie , N. W. Hendrickx , J. S. Clarke , L. M. K. Vandersypen , M. Veldhorst

Spins confined in quantum dots are a leading candidate for solid-state quantum bits that can be coherently controlled by optical pulses. There are, however, many challenges to developing a scalable multibit information processing device…

介观与纳米尺度物理 · 物理学 2012-09-26 Sophia E. Economou , Juan I. Climente , Antonio Badolato , Allan S. Bracker , Daniel Gammon , Matthew F. Doty

Spins in solids are cornerstone elements of quantum spintronics. Leading contenders such as defects in diamond, or individual phosphorous dopants in silicon have shown spectacular progress but either miss established nanotechnology or an…

Coherent manipulation of quantum bits (qubits) on time scales much shorter than the coherence time is a key prerequisite for quantum information processing. Electron spins in quantum dots (QDs) are particularly attractive for…

介观与纳米尺度物理 · 物理学 2011-10-03 A. Greilich , Sophia E. Economou , S. Spatzek , D. R. Yakovlev , D. Reuter , A. D. Wieck , T. L. Reinecke , M. Bayer

The coherent spin dynamics of electrons and holes are studied in a FA0.9Cs0.1PbI2.8Br0.2 perovskite bulk crystal, using time-resolved Kerr ellipticity in a two-color pump-probe scheme. The probe photon energy is tuned to the exciton…

Quantum mechanical phenomena, such as electronic coherence and entanglement, play a key role in achieving the unrivalled efficiencies of light-energy conversion in natural photosynthetic light-harvesting complexes, and triggered the growing…

量子物理 · 物理学 2011-02-02 Richard Hildner , Daan Brinks , Niek F. van Hulst

Coherent coupling between single quantum objects is at the heart of modern quantum physics. When coupling is strong enough to prevail over decoherence, it can be used for the engineering of correlated quantum states. Especially for…

We demonstrate coherent optical control of a single hole spin confined to an InAs/GaAs quantum dot. A superposition of hole spin states is created by fast (10-100 ps) dissociation of a spin-polarized electron-hole pair. Full control of the…

介观与纳米尺度物理 · 物理学 2012-01-09 T. M. Godden , J. H. Quilter , A. J. Ramsay , Yanwen Wu , P. Brereton , S. J. Boyle , I. J. Luxmoore , J. Puebla-Nunez , A. M. Fox , M. S. Skolnick

Nuclear spins in certain solids couple weakly to their environment, making them attractive candidates for quantum information processing and inertial sensing. When coupled to the spin of an optically-active electron, nuclear spins can be…

量子物理 · 物理学 2022-11-11 Alexander A. Wood , Russell M. Goldblatt , Robert E. Scholten , Andy M. Martin

The electronic spin degrees of freedom in semiconductors typically have decoherence times that are several orders of magnitude longer than other relevant timescales. A solid-state quantum computer based on localized electron spins as qubits…

量子物理 · 物理学 2007-05-23 A. Imamoglu , D. D. Awschalom , G. Burkard , D. P. DiVincenzo , D. Loss , M. Sherwin , A. Small

The ability to manipulate coherently individual quantum objects organized in arrays is a prerequisite to any scalable quantum information platform. For electron spin qubits, it requires the fine tuning of large arrays of tunnel-coupled…

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