相关论文: Polychromatic Excitation of Delocalized Long-Lived…

It is shown that long-lived states (LLS) involving pairs of methylene protons in nuclear magnetic resonance (NMR) can be readily excited in common molecules that contain two or more neighboring CH$_2$ groups. Accessing such LLS does not…

We introduce a broadly applicable technique to create nuclear spin singlet states in organic molecules and other many-atom systems. We employ a novel pulse sequence to produce a spin-lock induced crossing (SLIC) of the spin singlet and…

We probe small scalar coupling differences via the coherent interactions between two nuclear spin singlet states in organic molecules. We show that the spin-lock induced crossing (SLIC) technique enables the coherent transfer of singlet…

A solution with hyperpolarized nuclear spins encoded into a long-lived state has been utilized for sensing chemical phenomena. In a conventional way, nuclear spins are hyperpolarized at very low temperatures. In this work, we demonstrate…

We report observation of long-lived spin-singlet states in a 13C-1H spin pair at zero magnetic field. In 13C-labeled formic acid, we observe spin-singlet lifetimes as long as 37 seconds, about a factor of three longer than the T1 lifetime…

Long-lived (symmetry protected) hyperpolarized spin states offer important new opportunities (for example, in clinical MR imaging), but existing methods for producing these states are limited by either excess energy dissipation or high…

We report an observation of extremely long-lived spin states in systems of dipolar-coupled nuclear spins in solids. The 'suspended echo' experiment uses a simple stimulated echo pulse sequence and creates non-equilibrium states which live…

Spin-spin interactions in organic light-emitting diodes (OLEDs) based on thermally activated delayed fluorescence (TADF) are pivotal because radiative recombination is largely determined by triplet-to-singlet conversion, also called reverse…

Nuclear spins and paramagnetic centers in a solid randomly group to form clusters featuring nearly-degenerate, hybrid states whose dynamics are central to processes involving nuclear spin-lattice relaxation and diffusion. Their…

Collective charge-density modes (plasmons) of the clean two-dimensional unpolarized electron gas are stable, for momentum conservation prevents them from decaying into single-particle excitations. Collective spin-density modes (spin…

In connection to the chiral-induced spin-selectivity (CISS) effect, we theoretically analyze the electronic and spin states of edges of a finite $p$-orbital helical atomic chain with the intra-atomic spin-orbit interaction (SOI). This model…

We describe a simple scheme for the implementation and control of effective spin-spin interactions in self-assembled crystals of cold polar molecules. In our scheme spin states are encoded in two long-lived rotational states of the…

Electron spin dynamics are studied in Ga-doped ZnO single crystals by time-resolved Faraday and Kerr rotation spectroscopies. Long-lived spin coherence with two dephasing processes is discovered where the characteristic time is up to 5.2 ns…

The reaction 28Si + 181Ta has been studied at E(Lab) = 125 and 135 MeV. Coincidences between high energy particles and various X- and gamma-rays from abnormally long-lived states were observed. e.g. 7.8 - 8.6 MeV alpha-particles with…

We analyze the symmetry properties of the dipolar Hamiltonian as the main relaxation mechanism responsible for the observed NMR spectra of long lived states in methyl groups. Long lived states exhibit relaxation times that are considerably…

We use field-cycling-assisted dynamic nuclear polarization and continuous radio-frequency (RF) driving over a broad spectral range to demonstrate magnetic-field-dependent activation of nuclear spin transport from strongly-hyperfine-coupled…

S=1/2 quantum spin chains and ladders with random exchange coupling are studied by using an effective low-energy field theory and transfer matrix methods. Effects of the nonlocal correlations of exchange couplings are investigated…

Coupled pairs of nuclear spins-1/2 support one singlet state and three triplet states. Transitions between the singlet state and one of the triplet states may be driven by an oscillating low-frequency magnetic field, in the presence of…

Electron and phonon states in two different models of intentionally disordered superlattices are studied analytically as well as numerically. The localization length is calculated exactly and we found that it diverges for particular…

The periodical modulation of circularly polarized light with a frequency close to the electron spin resonance frequency induces a sharp change of the single electron spin orientation. Hyperfine interaction provides a feedback, thus fixing…