相关论文: Modeling Spin-Dependent Nonadiabatic Dynamics with…
The significance of topological phases has been widely recognized in the community of condensed matter physics. The well controllable quantum systems provide an artificial platform to probe and engineer various topological phases. The…
We investigate the effect of the Berry phase on quadrupoles that occur for example in the low-energy description of spin models. Specifically we study here the one-dimensional bilinear-biquadratic spin-one model. An open question for many…
We present an efficient \textit{ab initio} algorithm for quantum dynamics simulations of interacting systems that is based on the conditional decomposition of the many-body wavefunction [Phys. Rev. Lett. 113, 083003 (2014)]. Starting with…
This work identifies geometric effects on dynamics due to nonadiabatic couplings in Born Oppenheimer systems and provides a systematic method for deriving corrections to mixed quantum-classical methods. Specifically, an exact path integral…
We report an implementation for employing the algebraic diagrammatic construction to second order [ADC(2)] ab initio electronic structure level of theory in nonadiabatic dynamics simulations in the framework of the SHARC (surface hopping…
The geometrical Berry phase is key to understanding the behaviour of quantum states under cyclic adiabatic evolution. When generalised to non-Hermitian systems with gain and loss, the Berry phase can become complex, and should modify not…
The spin of a single electron in an electrically defined quantum dot in a 2DEG can be manipulated by moving the quantum dot adiabatically in a closed loop in the 2D plane under the influence of applied gate potentials. In this paper we…
Nonadiabatic quantum interferences emerge whenever nuclear wavefunctions in different electronic states meet and interact in a nonadiabatic region. In this work, we analyze how nonadiabatic quantum interferences translate in the context of…
Pauli spin blockade (PSB) is a significant physical effect in double quantum dot (DQD) systems. In this paper, we start from the fundamental quantum model of the DQD with the electron-electron interaction being considered, and then…
Understanding how to control phase transitions in quantum systems is at the forefront of research for the development of new quantum materials and technologies. Here, we study how the coupling of a quantum system to a non-Markovian…
We study theoretically the influence of Berry phase on the real-time dynamics of the single particle focusing on the diffusive dynamics, i.e., the time-dependence of the distribution function. Our model can be applied to the real-time…
Triply degenerate points (TDPs), which correspond to new types of topological semimetals, can support novel quasiparticles possessing effective integer spins while preserving Fermi statistics. Here by mapping the momentum space to the…
Dissipative effects on the nonadiabatic transition for the two and three level systems are studied. When the system is affected by a strong dissipation through the diabatic states, the exact transition probability is enumerated making use…
We derive the general formula giving the Berry phase for an arbitrary spin, having both magnetic-dipole and electric-quadrupole couplings with external time-dependent fields. We assume that the effective E and B fields remain orthogonal…
Non-equilibrium dynamics of many-body systems is important in many branches of science, such as condensed matter, quantum chemistry, and ultracold atoms. Here we report the experimental observation of a phase transition of the quantum…
Accurate description of nonadiabatic dynamics of molecules at metal surfaces involving electron transfer has been a longstanding challenge for theory. Here, we tackle this problem by first constructing high-dimensional neural network…
Mixed-quantum classical (MQC) methods for simulating the dynamics of molecules at metal surfaces have the potential to accurately and efficiently provide mechanistic insight into reactive processes. Here, we introduce simple two-dimensional…
A three-dimensional non-Hermitian Hamiltonian with parity-time symmetry can exhibit a closed exceptional surface (EP surface) in momentum space, which is a non-Hermitian deformation of the degeneracy line (DL). Since the degeneracy line…
We present the simulation of the photochemical dynamics of cyclobutanone induced by the excitation of the 3s Rydberg state. For this purpose, we apply the complete active space self-consistent field method together with spin-orbit…
Nonadiabatic geometric quantum computation in decoherence-free subspaces has received increasing attention due to the merits of its high-speed implementation and robustness against both control errors and decoherence. However, all the…