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Second-harmonic generation microscopy is a powerful technique capable of probing local crystal symmetries and electric fields at interfaces. However, it often suffers from weak signal strength and is difficult to understand in multilayer…

We develop a quantitative mathematical theory that offers new perspectives on nonlinear harmonic generation in plasmonic structures arising from symmetry breaking. Focusing on second harmonic generation--the most fundamental process and the…

偏微分方程分析 · 数学 2026-05-04 Hongyu Liu , Zhi-Qiang Miao , Jingfeng Yao , Chengxun Yuan , Guang-Hui Zheng

The generation process of second harmonic (SH) radiation from holes periodically arranged on a metal surface is investigated. Three main modulating factors affecting the optical response are identified: the near-field distribution at the…

介观与纳米尺度物理 · 物理学 2015-01-08 Sergio G. Rodrigo , V. Laliena , L. Martín-Moreno

Generation of second-harmonic waves is one of the universal nonlinear phenomena that have found numerous technical applications in many modern technologies, in particular, in photonics. This phenomenon also has great potential in the field…

介观与纳米尺度物理 · 物理学 2024-03-01 K. O. Nikolaev , S. R. Lake , G. Schmidt , S. O. Demokritov , V. E. Demidov

Second-order nonlinear optical processes do not manifest in the bulk of centrosymmetric materials, but may occur in the angstroms-thick layer at surfaces. At such length-scales, quantum mechanical effects come into play which could be…

光学 · 物理学 2021-05-11 Muhammad Khalid , Cristian Ciracì

Comparative analysis of second harmonic generation in ordinary and backward-wave settings is presented. Extraordinary properties of frequency doubling nonlinear optical reflectivity and pulse shaping through phase matching of ordinary and…

光学 · 物理学 2016-02-02 Alexander K. Popov , Sergey A. Myslivets

Collective responses of localized surface plasmon resonances, known as surface lattice resonances (SLRs) in metal nanoparticle arrays, can lead to high quality factors (~100), large local-field enhancements and strong light-matter…

光学 · 物理学 2018-05-23 Mikko J. Huttunen , Payman Rasekh , Robert W. Boyd , Ksenia Dolgaleva

The second-order nonlinear optical susceptibility $\Pi^{(2)}$ for second harmonic generation is calculated for gapped graphene. The linear and second-order nonlinear plasmon excitations are investigated in context of second harmonic…

介观与纳米尺度物理 · 物理学 2015-06-17 Godfrey Gumbs , Yonatan Abranyos , Upali Aparajita , Oleksiy Roslyak

The nonlinear magneto-plasmonics aims to utilize plasmonic excitations to control the mechanisms and taylor the efficiencies of the non-linear light frequency conversion at the nanoscale. We investigate the mechanisms of magnetic second…

The enhanced electric field at plasmonic resonances in nanoscale antennas can lead to efficient harmonic generation, especially when the plasmonic geometry is asymmetric on either inter-particle or intra-particle levels. The planar…

The second harmonic generation is one of the most important applications of nonlinear effect, which has attracted great interests in nonlinear optics and microwave in the past decades. To the best of our knowledge, however, generating the…

光学 · 物理学 2015-05-14 Hao Chi Zhang , Yifeng Fan , Jian Guo , Xiaojian Fu , Lianming Li , Cheng Qian , Tie Jun Cui

We present a theoretical study of second-harmonic generation from a singular metasurface. The singular metasurfaces strongly interact with the incident light, where the large field enhancement forms an intense surface polarization that…

光学 · 物理学 2023-01-10 Fan Yang , Cristian Ciracì

Second harmonic generation is a powerful tool directly connected to the symmetry of materials. Phase transitions, lattice rotations or electromagnetic coupling in multiferroic compounds can be revealed by using second harmonic…

光学 · 物理学 2010-01-11 Pablo Molina , Mariola O Ramirez , Basilio J. Garcia , Luisa E. Bausa

Nonlinear second harmonic optical activity of graphene covering a gold photon sieve was determined for different polarizations. The photon sieve consists of a subwavelength gold nanohole array placed on glass. It combines the benefits of…

介观与纳米尺度物理 · 物理学 2016-01-14 Michael Lobet , Michael Sarrazin , Francesca Cecchet , Nicolas Reckinger , Alexandru Vlad , Jean-François Colomer , Dan Lis

Polaritons can provide strong optical field enhancement allowing to boost light-matter interaction. Here, we experimentally observe enhancement of mid-infrared second-harmonic generation (SHG) using grating-coupled surface phonon polaritons…

We aim to clarify the role that absorption plays in nonlinear optical processes in a variety of metallic nanostructures and show how it relates to emission and conversion efficiency. We define a figure of merit that establishes the…

We have investigated second harmonic generation (SHG) from Ag-coated LiNbO3 (LN) core-shell nanocuboids and found that giant SHG can occur via deliberately designed double plasmonic resonances. By controlling the aspect ratio, we can tune…

光学 · 物理学 2014-11-19 Ming-Liang Ren , Si-Yuan Liu , Ben-Li Wang , Bao-Qin Chen , Jiafang Li , Zhi-Yuan Li

We study the nonlinear process of second harmonic generation in photonic time-crystals, materials with refractive index that varies abruptly and periodically in time, and obtain the phase matching condition for this process. We find…

A new concept for second-harmonic generation (SHG) in an optical nanocircuit is proposed. We demonstrate both theoretically and experimentally that the symmetry of an optical mode alone is sufficient to allow SHG even in centro-symmetric…

We present a new theoretical approach to the study of second and third harmonic generation from metallic nanostructures and nanocavities filled with a nonlinear material, in the ultrashort pulse regime. We model the metal as a two-component…