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Resonant enhancement of high harmonic generation can be obtained in plasmas containing ions with strong radiative transitions resonant with harmonic orders. The mechanism for this enhancement is still debated. We perform the first temporal…

Excitation of coherent optical phonons in solids provides a pathway for ultrafast modulation of light on a sub-ps timescale. Here, we report on efficient 3.6 THz modulation of light reflected from hybrid metal/semiconductor plasmonic…

Second-harmonic generation (SHG) is a powerful surface-specific probe for centrosymmetric materials, with broad relevance to energy and biological interfaces. Plasmonic nanomaterials have been extensively utilized to amplify this nonlinear…

Optical second-harmonic generation (SHG) is a nonlinear parametric process that doubles the frequency of incoming light. Only allowed in non-centrosymmetric materials, it has been widely used in frequency modulation of lasers, surface…

材料科学 · 物理学 2021-01-05 Wontaek Kim , Je Yhoung Ahn , Juseung Oh , Ji Hoon Shim , Sunmin Ryu

Second-harmonic generation is of paramount importance in several fields of science and technology, including frequency conversion, self-referencing of frequency combs, nonlinear spectroscopy and pulse characterization. Advanced…

We demonstrate a simple and scalable approach to increase conversion efficiencies of nonlinear metasurfaces by incorporating them into multipass cells and by letting the pump beam to interact with the metasurfaces multiple times. We…

High quality factor optical microcavities have been employed in a variety of material systems to enhance nonlinear optical interactions. While single-crystalline aluminum nitride microresonators have recently emerged as a low loss platform…

We study second harmonic generation in a planar dielectric waveguide having a low-index, polymer core layer, bounded by two multilayer stacks. This geometry allows exceptionally strong confinement of the light at the fundamental wavelength…

The outstanding optical properties for plasmon resonances in noble metal nanoparticles enable the observation of non-linear optical processes such as second-harmonic generation (SHG) at the nanoscale. Here, we investigate the SHG process in…

A high-power laser pulse at normal incidence onto a plane solid target will generate odd harmonics of its frequency. However, the spacing of the harmonic lines in this configuration is fixed. Here, we study harmonic generation using two…

光学 · 物理学 2025-01-20 Raoul Trines , Holger Schmitz , Martin King , Paul McKenna , Robert Bingham

In addition to their strong nonlinear optical response, transition metal dichalcogenides (TMDCs) possess a high refractive index in the visible and infrared regime. Therefore, by patterning those TMDCs into dielectric nanoresonators, one…

True phase-matched second-harmonic generation in a waveguide of crosslinkable ferroelectric liquid crystals is demonstrated. These materials allow the formation of macroscopically polar structures whose order can be frozen by…

软凝聚态物质 · 物理学 2009-10-31 Valentina S. U. Fazio , S. T. Lagerwall , P. Busson , A. Hult , H. Motschmann

We report on the photoconductance in two-dimensional arrays of gold nanorods which is strongly enhanced at the frequency of the longitudinal surface plasmon of the nanorods. The arrays are formed by a combination of droplet deposition and…

介观与纳米尺度物理 · 物理学 2015-06-17 S. Diefenbach , N. Erhard , J. Schopka , A. Martin , C. Karnetzky , D. Iacopino , A. W. Holleitner

Generation of terahertz harmonics by frequency multiplication with a semiconductor superlattice due to an excitation of relaxation oscillations by incident waves is investigated theoretically. It is shown that the relaxation oscillations…

介观与纳米尺度物理 · 物理学 2015-05-20 Anatoly A Ignatov

We present an analytical theory of second harmonic generation (SHG) in hybrid structures combining a nonlinear 2D crystal with a dielectric metasurface waveguide. The theory describes the excitation spectrum and enhancement of SHG at both…

光学 · 物理学 2025-11-07 Egor S. Vyatkin , Sergey A. Tarasenko

Asymmetric transmission - direction-selective control of electromagnetic transmission between two ports - is an important phenomenon typically exhibited by two-dimensional chiral systems. Here, we study this phenomenon in chiral plasmonic…

In this study, we investigate second- and third-harmonic generation processes in Au nanorod systems using the real-time time-dependent density functional tight binding method. Our study focuses on the computation of nonlinear signals based…

光学 · 物理学 2024-09-18 Sajal Kumar Giri , George C. Schatz

Optical second-harmonic generation is demonstrated to be a sensitive probe of the buried interface between the lattice matched semiconductors gallium phosphide and silicon with (001) orientation. Rotational anisotropy measurements of SHG…

介观与纳米尺度物理 · 物理学 2020-10-29 K. Brixius , A. Beyer , J. Güdde , M. Dürr , W. Stolz , K. Volz , U. Höfer

Second harmonic generation (SHG) is a coherent nonlinear phenomenon that plays an important role in laser color conversion. Lithium niobate (LN), which features both a large band gap and outstanding second-order nonlinearities, acts as an…

In this paper, we proposed and numerically demonstrated a giant enhancement up to 108 in both forward and backward propagation of the Second Harmonic Generation by combining the high-quality factor cavities of the Bound States in the…

光学 · 物理学 2022-06-24 Juan José Robayo Yepes , Fadi Issam Baida , Abdoulaye Ndao
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