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We demonstrate a coherence time of 2.1(1)~s for electron spin superposition states of a single trapped $^{40}$Ca$^+$ ion. The coherence time, measured with a spin-echo experiment, corresponds to residual rms magnetic field fluctuations…

We present a data-efficient framework for constructing general classical spin Hamiltonians by combining the spin-cluster expansion (SCE) with fully self-consistent noncollinear spin density functional theory (DFT). The key idea is to fit…

材料科学 · 物理学 2026-05-26 Tomonori Tanaka , Yoshihiro Gohda

We present an implementation of time-dependent density functional perturbation theory for spin fluctuations, based on planewaves and pseudopotentials. We compute the dynamic spin susceptibility self-consistently by solving the…

材料科学 · 物理学 2018-01-24 Kun Cao , Henry Lambert , Paolo G. Radaelli , Feliciano Giustino

A pinch point singularity in the structure factor characterizes an important class of condensed matter that is a counterpoint to the paradigm of broken symmetry. This class includes water ice, charge ice and spin ice. Of these, dipolar spin…

强关联电子 · 物理学 2020-03-16 Mikael Twengström , Patrik Henelius , Steven T. Bramwell

An open problem in applied mathematics is to predict interesting molecules which are realistic targets for chemical synthesis. In this paper, we use a spin Hamiltonian-type model to predict molecular magnets (MMs) with magnetic moments that…

Numerical modelling of coherent spin relaxation in nanomagnets, formed by magnetic molecules of high spins, is accomplished. Such a coherent spin dynamics can be realized in the presence of a resonant electric circuit coupled to the magnet.…

介观与纳米尺度物理 · 物理学 2009-11-13 V. I. Yukalov , V. K. Henner , P. V. Kharebov

Defects with associated electron and nuclear spins in solid-state materials have a long history relevant to quantum information science going back to the first spin echo experiments with silicon dopants in the 1950s. Since the turn of the…

States with long coherence are a crucial requirement for qubits and quantum memories. Nuclear spins in epitaxial quantum dots are a great candidate, offering excellent isolation from external environments and on-demand coupling to optical…

介观与纳米尺度物理 · 物理学 2025-02-18 Harry E. Dyte , Santanu Manna , Saimon F. Covre da Silva , Armando Rastelli , Evgeny A. Chekhovich

We study the spin-relaxation time in materials where a large spin-orbit coupling (SOC) is present which breaks the spatial inversion symmetry. Such a spin-orbit coupling is realized in zincblende structures and heterostructures with a…

强关联电子 · 物理学 2017-10-23 Lénárd Szolnoki , Annamária Kiss , Balázs Dóra , Ferenc Simon

Engineered spin-electric coupling enables spin qubits in semiconductor nanostructures to be manipulated efficiently and addressed individually. While synthetic spin-orbit coupling using a micromagnet is widely used for driving qubits based…

We report on the 29Si nuclear spin decoherence time at room temperature for a pure (99.99999%, 7N) and carrier-less (p-type, doping level of 10^15cm-3) silicon in which 29Si nuclei are naturally abundant (4.7%). Despite the experimental…

材料科学 · 物理学 2007-05-23 Shinji Watanabe , Susumu Sasaki

We study decoherence of propagating spin-1/2 excitations in generic (non-integrable and/or disordered) spin chains. We find the relevant decoherence times to be shorter in both the near-critical and diffusive regimes (if any), which fact…

强关联电子 · 物理学 2009-11-10 D. V. Khveshchenko

We develop in this letter an analytical approach using form- factors to compute time dependent correlations in integrable quantum impurity problems. As an example, we obtain for the first time the frequency dependent conductivity…

凝聚态物理 · 物理学 2009-10-28 F. Lesage , H. Saleur , S. Skorik

Optically addressable spin defects are excellent candidate platform for quantum sensing and quantum network. Nuclear spins coupled to color centers naturally enable long lived quantum memories and local qubits registers. To fully leverage…

We have measured the decay of NMR multiple quantum coherence intensities both under the internal dipolar Hamiltonian as well as when this interaction is effectively averaged to zero, in the cubic calcium fluoride (CaF2) spin system and the…

其他凝聚态物理 · 物理学 2013-05-29 HyungJoon Cho , Paola Cappellaro , David G. Cory , Chandrasekhar Ramanathan

We measure the ensemble transverse relaxation time (T2*) and spin-echo coherence time (T2) of the proton spin of HD molecules trapped in solid parahydrogen. By using high-purity parahydrogen matrices, we are able to measure significantly…

量子物理 · 物理学 2026-04-21 Alexandar P. Rollings , Jonathan D. Weinstein

The dynamics of single electron and nuclear spins in a diamond lattice with different 13C nuclear spin concentration is investigated. It is shown that coherent control of up to three individual nuclei in a dense nuclear spin cluster is…

On the quest to understand and reduce environmental noise in Si spin qubits, hyperfine interactions between electron and nuclear spins impose a major challenge. Silicon is a promising host material because one can enhance the spin coherence…

介观与纳米尺度物理 · 物理学 2024-05-20 Lukas Cvitkovich , Peter Stano , Christoph Wilhelmer , Dominic Waldhör , Daniel Loss , Yann-Michel Niquet , Tibor Grasser

The authors present a quantity termed charge-spin susceptibility, which measures the charge response to spin degrees of freedom in strongly correlated materials. This quantity is simple to evaluate using both standard density functional…

超导电性 · 物理学 2021-02-23 J. N. B. Rodrigues , Lucas K. Wagner

Crystal defects can confine isolated electronic spins and are promising candidates for solid-state quantum information. Alongside research focusing on nitrogen vacancy centers in diamond, an alternative strategy seeks to identify new spin…