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This paper reviews non-resonant, meV-resolution inelastic x-ray scattering (IXS), as applied to the measurement of atomic dynamics of crystalline materials. It is designed to be an introductory, though in-depth, look at the field for those…

材料科学 · 物理学 2020-08-26 Alfred Q. R. Baron

This paper reviews non-resonant meV-resolved inelastic x-ray scattering (IXS) as a complementary method to inelastic neutron scattering (INS). Two aspects of IXS that are notable in this context are (1) that IXS allows straightforward…

软凝聚态物质 · 物理学 2024-06-18 Alfred Q. R. Baron

We investigate the presence of an acoustic-quasi-elastic interaction contribution in the IXS spectra of liquid water at 301K using inelastic x-ray scattering with sub-meV energy resolution at momentum transfers 0.77<=Q<=4.20 /nm. The…

软凝聚态物质 · 物理学 2021-07-22 Daisuke Ishikawa , Alfred Q. R. Baron

Inelastic X-ray scattering (IXS) is an important tool for studies of equilibrium dynamics in condensed matter. A new spectrometer recently proposed for ultra-high-resolution IXS (UHRIX) has achieved 0.6~meV and 0.25~nm$^{-1}$ spectral and…

The experimental results relevant for the understanding of the microscopic dynamics in liquid metals are reviewed, with special regards to the ones achieved in the last two decades. Inelastic Neutron Scattering played a major role since the…

无序系统与神经网络 · 物理学 2009-11-11 Tullio Scopigno , Giancarlo Ruocco , Francesco Sette

We describe a new method for imaging ultrafast dynamics in condensed matter using inelastic x-ray scattering (IXS). We use the concepts of causality and irreversibility to construct a general solution to the inverse scattering problem (or…

其他凝聚态物理 · 物理学 2009-06-12 P. Abbamonte , G. C. L. Wong , D. Cahill , J. P. Reed , R. H. Coridan , N. W. Schmidt , G. H. Lai , Y. I. Joe , D. Casa

Resonant inelastic x-ray scattering (RIXS) provides remarkable opportunities to interrogate ultrafast dynamics in liquids. Here we use RIXS to study the fundamentally and practically important hydroxyl radical in liquid water, OH(aq).…

Molecular dynamics in pure water and aqueous salt solutions remain incompletely understood, partly due to the apparent contradictions between results from different spectroscopic techniques. In this work, we demonstrate, by detailed…

软凝聚态物质 · 物理学 2025-12-22 Rolf Zeißler , Florian Pabst , Thomas Blochowicz

New inelastic X-ray scattering experiments have been performed on liquid lithium in a wide wavevector range. With respect to the previous measurements, the instrumental resolution, improved up to 1.5 meV, allows to accurately investigate…

无序系统与神经网络 · 物理学 2009-10-31 T. Scopigno , U. Balucani , G. Ruocco , F. Sette

We propose a method for realizing true, real-space imaging of charge dynamics in a periodic system, with angstrom spatial resolution and attosecond time resolution. In this method, inelastic x-ray scattering (IXS) is carried out with a…

强关联电子 · 物理学 2015-06-05 Yu Gan , Anshul Kogar , Peter Abbamonte

Continued improvement of the energy resolution of resonant inelastic x-ray scattering (RIXS) spectrometers is crucial for fulfilling the potential of this technique in the study of electron dynamics in materials of fundamental and…

仪器与探测器 · 物理学 2017-09-11 Jungho Kim , D. Casa , Ayman Said , Richard Krakora , B. J. Kim , Elina Kasman , Xianrong Huang , T. Gog

In the past decade, Resonant Inelastic X-ray Scattering (RIXS) has made remarkable progress as a spectroscopic technique. This is a direct result of the availability of high-brilliance synchrotron X-ray radiation sources and of advanced…

An inelastic X-ray scattering experiment has been performed in liquid aluminum with the purpose of studying the collective excitations at wavevectors below the first sharp diffraction peak. The high instrumental resolution (up to 1.5 meV)…

无序系统与神经网络 · 物理学 2009-10-31 T. Scopigno , U. Balucani , G. Ruocco , F. Sette

We show that the momentum flexibility of inelastic x-ray scattering may be exploited to invert its loss function, alowing real time imaging of density disturbances in a medium. We show the disturbance arising from a point source in liquid…

凝聚态物理 · 物理学 2009-11-10 P. Abbamonte , K. D. Finkelstein , M. D. Collins , S. M. Gruner

Excitons in a complex organic molecular crystal were studied by inelastic x-ray scattering (IXS) for the first time. The dynamic dielectric response function is measured over a large momentum transfer region, from which an exciton…

其他凝聚态物理 · 物理学 2007-05-23 K. Yang , L. P. Chen , Y. Q. Cai , N. Hiraoka , S. Li , J. F. Zhao , D. W. Shen , H. F. Song , H. Tian , L. H. Bai , Z. H. Chen , Z. G. Shuai , D. L. Feng

Inelastic X-ray scattering data have been collected for liquid sodium at T=390 K, i.e. slightly above the melting point. Owing to the very high instrumental resolution, pushed up to 1.5 meV, it has been possible to determine accurately the…

无序系统与神经网络 · 物理学 2009-11-07 T. Scopigno , U. Balucani , G. Ruocco , F. Sette

We compare several different ways of measuring the energy resolution for meV-resolved inelastic x-ray scattering (IXS): using scattering from poly(methyl methacrylate), PMMA, using scattering from borosilicate glass (Tempax), and using…

材料科学 · 物理学 2021-03-17 Daisuke Ishikawa , Alfred Q. R. Baron

Recent improvements in instrumentation have established resonant inelastic x-ray scattering (RIXS) as a valuable new probe of the magnetic excitations in the cuprates. This article introduces RIXS, focusing on the Cu $L_3$ resonance, and…

超导电性 · 物理学 2015-02-17 M. P. M. Dean

The development of medium-energy inelastic X-ray scattering (IXS) optics with meV and sub-meV resolution has attracted considerable efforts in recent years. Meanwhile, there are also concerns or debates about the fundamental and feasibility…

光学 · 物理学 2011-09-12 Xian-Rong Huang

X-ray absorption spectroscopy (XAS) is a powerful experimental technique to probe the local order in materials with core electron excitations. Experimental interpretation requires supporting theoretical calculations. For water, these…

计算物理 · 物理学 2022-05-17 Fujie Tang , Zhenglu Li , Chunyi Zhang , Steven G. Louie , Roberto Car , Diana Y. Qiu , Xifan Wu
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