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As the Si-based transistors scale down to atomic dimensions, the basic principle of current electronics, which heavily relies on the tunable charge degree of freedom, faces increasing challenges to meet the future requirements of speed,…

材料科学 · 物理学 2023-10-13 Allen Jian Yang , Su-Xi Wang , Jianwei Xu , Xian Jun Loh , Qiang Zhu , Xiao Renshaw Wang

The unprecedented demand for sophisticated, self-powered, compact, ultrafast, cost-effective, and broadband light sensors for a myriad of applications has spurred a lot of research, precipitating in a slew of studies over the last decade.…

应用物理 · 物理学 2024-02-20 Nagaraj Nandihalli

Current technologies for X-ray detection rely on scintillation from expensive inorganic crystals grown at high-temperature, which so far has hindered the development of large-area scintillator arrays. Thanks to the presence of heavy atoms,…

仪器与探测器 · 物理学 2016-11-21 M. D. Birowosuto , D. Cortecchia , W. Drozdowski , K. Brylew , W. Lachmanski , A. Bruno , C. Soci

The possibility of creating heterostructure of two-dimensional (2D) materials has emerged as a viable route towards realizing novel optoelectronic devices. However, the low light absorption due to their small absorption cross section,…

介观与纳米尺度物理 · 物理学 2023-03-14 Shubhrasish Mukherjee , Didhiti Bhattacharya , Samit Kumar Ray , Atindra Nath Pal

Ruddlesden-Popper hybrid iodide 2D perovskites are put forward as stable alternatives to their 3D counterparts. Using first-principles calculations, we demonstrate that equilibrium concentrations of point defects in the 2D perovskites…

材料科学 · 物理学 2022-10-10 Haibo Xue , Zehua Chen , Shuxia Tao , Geert Brocks

Using density-functional theory calculations, we analyze the optical absorption properties of lead (Pb)-free metal halide perovskites (AB$^{2+}$X$_3$) and double perovskites (AB$^+$B$^{3+}$X$_6$) (A = Cs or monovalent organic ion, B$^{2+}$…

材料科学 · 物理学 2017-06-19 Weiwei Meng , Xiaoming Wang , Zewen Xiao , Jianbo Wang , David Mitzi , Yanfa Yan

Photodetectors converting light signals into detectable photocurrents are ubiquitously in use today. To improve the compactness and performance of next-generation devices and systems, low dimensional materials provide rich physics to…

2D materials are compatible with many material platforms as they adhere to other materials strictly by van der Waals interactions. This, together with the variety of band gaps found among transition metal dichalcogenides (TMDCs), makes them…

Because of their strong excitonic photoluminescence (PL) and electroluminescence (EL), together with an excellent electronic tunability, transition metal dichalcogenide (TMD) semiconductors are promising candidates for novel optoelectronic…

介观与纳米尺度物理 · 物理学 2019-03-08 Lukas Dobusch , Simone Schuler , Vasili Perebeinos , Thomas Mueller

Van der Waals (vdW) heterostructures consisting of two dimensional materials offer a platform to obtain material by design and are very attractive owing to novel electronic states. Research on 2D van der Waals heterostructures (vdWH) has so…

介观与纳米尺度物理 · 物理学 2017-05-11 Kyle Ray , Alexander E. Yore , Tong Mou , Sauraj Jha , K. K. H. Smithe , Bin Wang , Eric Pop , A. K. M. Newaz

Two-dimensional (2D) material photodetectors have gained great attention as potential elements for optoelectronic applications. However, the linearity of the photoresponse is often compromised by the carrier interaction, even in 2D…

介观与纳米尺度物理 · 物理学 2023-12-12 Jinpeng Xu , Xiaoguang Luo , Xi Lin , Xi Zhang , Fan Liu , Yuting Yan , Siqi Hu , Mingwen Zhang , Nannan Han , Xuetao Gan , Yingchun Cheng , Wei Huang

Quantum wells made of two-dimensional organic-inorganic hybrid perovskites (2D-PKs) offer a high degree of flexibility in tailoring optoelectronic properties through carrier confinement and functional interlayers. Compared to their 3D…

Monolayer transition metal dichalcogenides are uniquely-qualified materials for photonics because they combine well defined tunable direct band gaps and selfpassivated surfaces without dangling bonds. However, the atomic thickness of these…

Transition metal dichalcogenides have emerged as promising materials for nano-photonic resonators due to their large refractive index, low absorption within a large portion of the visible spectrum and compatibility with a wide range of…

The optical properties of transition metal dichalcogenide monolayers are widely dominated by excitons, Coulomb-bound electron-hole pairs. These quasi-particles exhibit giant oscillator strength and give rise to narrow-band, well-pronounced…

介观与纳米尺度物理 · 物理学 2018-07-13 Christian Schneider , Mikhail M. Glazov , Tobias Korn , Sven Höfling , Bernhard Urbaszek

The hybrid perovskite CH3NH3PbX3 (X= Cl, Br, I) is a promising material for developing novel optoelectronic devices. Owing to the intrinsic non-layer structure, it remains challenging to synthesize molecularly thin CH3NH3PbX3 with large…

Density functional theory calculations are used to show that it is possible to dope semiconducting transition metal dichalcogenides (TMD) such as MoS$_2$ and WS$_2$ with electrons and/or holes either by chemical substitution or by…

介观与纳米尺度物理 · 物理学 2014-09-16 A. Carvalho , A. H. Castro Neto

We have studied the optical conductivity of two-dimensional (2D) semiconducting transition metal dichalcogenides (STMDC) using ab-initio density functional theory (DFT). We find that this class of materials presents large optical response…

材料科学 · 物理学 2013-11-06 A. Carvalho , R. M. Ribeiro , A. H. Castro Neto

2D Ruddlesden - Popper perovskites are promising candidates for energy harvesting applications due to their tunable optical properties and excellent ambient stability. Moreover, they are solution-processable and compatible with upscalable…

Two-dimensional crystals, single sheets of layered materials, often show distinct properties desired for optoelectronic applications, such as larger and direct band gaps, valley- and spinorbit effects. Being atomically thin, the low amount…

材料科学 · 物理学 2018-11-14 Roman Kempt , Agnieszka Kuc , Jae Hyo Han , Jinwoo Cheon , Thomas Heine