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Realizing nonlinear optical response in the low photon density limit in solid-state systems has been a long-standing challenge. Semiconductor microcavities in the strong coupling regime hosting exciton-polaritons have emerged as attractive…

Hybrid interlayer excitons in bilayer MoS2 are a promising platform for nonlinear optics due to their intrinsic dipolar character, which combines in-plane and out-ofplane dipole moments. In this work, we directly probe the nonlinear…

Interlayer excitons (IXs) in hetero-bilayers of transition metal dichalcogenides (TMDs) represent an exciting emergent class of long-lived dipolar composite bosons in an atomically thin, near-ideal two-dimensional (2D) system. The…

We consider the scenario of excitons in a semiconductor bilayer that are strongly coupled to cavity photons, leading to the formation of dipolar exciton polaritons (dipolaritons). Using a realistic pseudopotential for the dipolar…

介观与纳米尺度物理 · 物理学 2026-02-27 Yasufumi Nakano , Olivier Bleu , Brendan C. Mulkerin , Jesper Levinsen , Meera M. Parish

Coulomb bound electron-hole pairs, excitons, govern the optical properties of semi-conducting transition metal dichalcogenides like MoS$_2$ and WSe$_2$. We study optical transitions at the K-point for 2H homobilayer MoS$_2$ in Density…

Interacting bosonic quasiparticles are the cornerstone for exploring many-body physics and nonlinear quantum phenomena in correlated light-matter systems. Strongly interacting dipolar excitons in van der Waals heterostructures have…

Nonperturbative coupling between cavity photons and excitons leads to formation of hybrid light-matter excitations termed polaritons. In structures where photon absorption leads to creation of excitons with aligned permanent dipoles, the…

介观与纳米尺度物理 · 物理学 2018-11-30 Emre Togan , Hyang-Tag Lim , Stefan Faelt , Werner Wegscheider , Atac Imamoglu

Two dimensional semiconductors provide an ideal platform for exploration of linear exciton and polariton physics, primarily due to large exciton binding energy and strong light-matter coupling. These features, however, generically imply…

介观与纳米尺度物理 · 物理学 2020-04-22 Li Bing Tan , Ovidiu Cotlet , Andrea Bergschneider , Richard Schmidt , Patrick Back , Yuya Shimazaki , Martin Kroner , Atac Imamoglu

Microscopic insights into nonlinear interactions are essential for advancing polaritonic devices. Existing studies often rely on phenomenological models that overlook important many-body processes. Based on a material-specific and…

介观与纳米尺度物理 · 物理学 2026-03-31 Jonas K König , Jamie M Fitzgerald , Daniel Erkensten , Ermin Malic

Transition metal dichalcogenides integrated within a high-quality microcavity support well-defined exciton polaritons. While the role of intralayer excitons in 2D polaritonics is well studied, interlayer excitons have been largely ignored…

介观与纳米尺度物理 · 物理学 2022-12-07 Jonas K. König , Jamie M. Fitzgerald , Joakim Hagel , Daniel Erkensten , Ermin Malic

Ensembles of indirect or interlayer excitons (IXs) are intriguing systems to explore classical and quantum phases of interacting bosonic ensembles. IXs are composite bosons that feature enlarged lifetimes due to the reduced overlap of the…

The interaction of intralayer and interlayer excitons is studied in a two-dimensional semiconductor, homobilayer MoS$_2$. It is shown that the measured optical susceptibility reveals both the magnitude and the sign of the coupling…

Transition-metal dichalcogenide bilayers exhibit a rich exciton landscape including layer-hybridized excitons, i.e. excitons which are of partly intra- and interlayer nature. In this work, we study hybrid exciton-exciton interactions in…

介观与纳米尺度物理 · 物理学 2023-06-28 Daniel Erkensten , Samuel Brem , Raul Perea-Causin , Joakim Hagel , Fedele Tagarelli , Edoardo Lopriore , Andras Kis , Ermin Malic

Strong optical nonlinearities play a central role in realizing quantum photonic technologies. In solid state systems, exciton-polaritons, which result from the hybridization of material excitations and cavity photons, are an attractive…

Exciton-polaritons are mutually interacting quantum hybridizations of confined photons and electronic excitations. Here we demonstrate a system of optically guided, electrically polarized exciton-polaritons ('dipolaritons') that displays up…

介观与纳米尺度物理 · 物理学 2018-04-18 Itamar Rosenberg , Dror Liran , Yotam Mazuz-Harpaz , Kenneth West , Loren Pfeiffer , Ronen Rapaport

Quantum simulation is a promising approach to understand complex strongly correlated many-body systems using relatively simple and tractable systems. Photon-based quantum simulators have great advantages due to the possibility of direct…

介观与纳米尺度物理 · 物理学 2018-02-14 Hai-Xiao Wang , Alan Zhan , Ya-Dong Xu , Huan-Yang Chen , Wen-Long You , Arka Majumdar , Jian-Hua Jiang

The realization of exciton-polaritons -- hybrid excitations of semiconductor quantum well excitons and cavity photons -- has been of great technological and scientific significance. In particular, the short-range collisional interaction…

量子气体 · 物理学 2018-07-17 Valentin Walther , Robert Johne , Thomas Pohl

Emergent strongly-correlated electronic phenomena in atomically-thin transition metal dichalcogenides are an exciting frontier in condensed matter physics, with examples ranging from bilayer superconductivity~\cite{zhao2023evidence} and…

Bosons hopping across sites and interacting on-site are the essence of the Bose-Hubbard model (BHM). Inspired by the success of BHM simulators with atoms in optical lattices, proposals for implementing the BHM with photons in coupled…

光学 · 物理学 2016-06-29 S. R. K. Rodriguez , A. Amo , I. Sagnes , L. Le Gratiet , E. Galopin , A. Lemaitre , J. Bloch

In transition metal dichalcogenides layers of atomic scale thickness, the electron-hole Coulomb interaction potential is strongly influenced by the sharp discontinuity of the dielectric function across the layer plane. This feature results…

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