相关论文: Frustration on a centred pyrochlore lattice in met…
Geometrical frustration among interacting spins combined with strong quantum fluctuations destabilize long-range magnetic order in favour of more exotic states such as spin liquids. By following this guiding principle, a number of spin…
A unique type of frustrated lattice is found in two A-site ordered spinel oxides, LiGaCr4O8 and LiInCr4O8. Because of the large size mismatch between Li+ and Ga3+/In3+ ions at the A site, the pyrochlore lattice, made up of Cr3+ ions…
Metastable Co$_2$Ti$_3$O$_8$ was synthesized through a topochemical reaction using Li$_2$CoTi$_3$O$_8$ as the precursor, resulting in a vacancy-ordered spinel structure. Crystal structure analysis confirmed that Co ions selectively occupy…
Frustration in magnetic materials arising from competing exchange interactions can prevent the system from adopting long-range magnetic order and can instead lead to a diverse range of novel quantum and topological states with exotic…
We report the characterisation of natural samples of the cubic pyrite mineral MnS2 using very high resolution synchrotron X-ray diffraction techniques. At low temperatures we find a new low temperature polymorph, which results from coupling…
The collective behavior of interacting magnetic moments can be strongly influenced by the topology of the underlying lattice. In geometrically frustrated spin systems, interesting chiral correlations may develop that are related to the spin…
Frustrated three dimensional quantum magnets are notoriously impervious to theoretical analysis. Here we use a combination of three computational methods to investigate the three dimensional pyrochlore $S=1/2$ quantum antiferromagnet, an…
Frustrated magnetic systems exhibit highly degenerate ground states and strong fluctuations, often leading to new physics. An intriguing example of current interest is the antiferromagnet on a diamond lattice, realized physically in A-site…
The temperature dependent ac and dc magnetization and heat capacity data of Ca$_3$CoIrO$_6$, a spin-chain compound crystallizing in a K$_4$CdCl$_6$-derived rhombohedral structure, show the features due to magnetic ordering of a…
Lattice-coupled antiferromagnetic spin model is analyzed for a number of frustrated lattices: triangular, Kagome, and pyrochlore. In triangular and Kagome lattices where ground state spins are locally ordered, the spin-lattice interaction…
We report magnetization and heat-capacity measurements on the ordered-spinel oxide Li$_2$NiGe$_3$O$_8$, where Ni$^{2+}$ ions with $S = 1$ form a single three-dimensional trillium lattice. Powder x-ray diffraction confirms a cubic…
It is predicted that strongly interacting spins on a frustrated lattice may lead to a quantum disordered ground state or even form a quantum spin liquid with exotic low-energy excitations. However, a thorough tuning of the frustration…
Magnetic frustration, the competition among exchange interactions, often leads to novel magnetic ground states with unique physical properties which can hinge on details of interactions that are otherwise difficult to observe. Such states…
We study the classical Heisenberg model on a recently identified three dimensional corner-shared equilateral triangular lattice, a magnetic sublattice to a large class of systems with the symmetry group P2$_1$3. Since the degree of…
The crystal structures and magnetic properties of three previously unreported A2B2F7 pyrochlore materials, NaSrMn2F7, NaCaFe2F7, and NaSrFe2F7 are presented. In these compounds, either S=2 Fe2+ or S=5/2 Mn2+ is on the B site, while…
The charge ordered structure of ions and vacancies characterizing rare-earth pyrochlore oxides serves as a model for the study of geometrically frustrated magnetism. The organization of magnetic ions into networks of corner-sharing…
Geometric frustration arises when lattice structure prevents simultaneous minimization of local interactions. It leads to highly degenerate ground states and, subsequently, complex phases of matter such as water ice, spin ice and frustrated…
Above 40K, the magnetic susceptibility of the heavy Fermion spinel LiV2O4 has many features in common with those of geometrically frustrated magnetic insulators, while its room temperature resistivity comfortably exceeds the Mott-Regel…
Magnetic pyrochlore oxides, including the spin ice materials, have proved to be a rich field for the study of geometrical frustration in 3 dimensions. Recently, a new family of magnetic oxides has been synthesised in which the half of the…
We perform a general study of spin ordering on the pyrochlore lattice with a 3:1 proportionality of two spin polarizations. Equivalently, this describes valence bond solid conformations of a quantum dimer model on the diamond lattice. We…