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Light scattering limits the penetration depth of non-invasive Raman spectroscopy in biological media. While safe levels of irradiation may be adequate to analyze superficial tissue, scattering of the pump beam reduces the Raman signal to…

Propagation of light in a highly scattering medium is among the most fascinating optical effect that everyone experiences on an everyday basis and possesses a number of fundamental problems which have yet to be solved. Conventional wisdom…

We present a method for deriving limits on Raman scattering in structured media and exploit it to constrain the maximum Raman signal resulting from a planewave incident on either a single Raman molecule in the vicinity of a structured…

This is a preliminary acount of a theory for Raman scattering by current-carrying molecular junctions. The approach combines a non-equilibrium Green's function (NEGF) description of the non-equilibrium junction with a generalized scattering…

介观与纳米尺度物理 · 物理学 2009-04-09 Michael Galperin , Mark A. Ratner , Abraham Nitzan

The inelastic scatterings of matter systems, such as Raman scattering, contain rich information on mechanical vibrations like as resonant frequencies, which lead to various applications, for example, a sensor for specific molecules.…

量子物理 · 物理学 2021-10-04 Sho Tamaki , Tomohiro Yokoyama , Hajime Ishihara

High-gain resonant nonlinear Raman scattering on trapped cold atoms within a high-fineness ring optical cavity is simply explained under a nonlinear opto-mechanical mechanism, and a proposal using it to detect frequency of micro-trap on…

原子物理 · 物理学 2014-03-24 Lin Zhang

Resonant Raman scattering is investigated in monolayer WS$_2$ at low temperature with the aid of an unconventional spectroscopy technique, $i.e.$, Raman scattering excitation (RSE). The RSE spectrum is made up by sweeping the excitation…

介观与纳米尺度物理 · 物理学 2017-07-13 Maciej R. Molas , Karol Nogajewski , Marek Potemski , Adam Babinski

We consider the coherent stimulated Raman process developing in an optically dense disordered atomic medium, which can also incoherently scatter the light over all outward directions. The Raman process is discussed in the context of a…

量子物理 · 物理学 2008-10-20 O. S. Mishina , N. V. Larionov , A. S. Sheremet , I. M. Sokolov , D. V. Kupriyanov

A semiclassical model is used to investigate the possibility of selectively exciting one of two closely spaced, uncoupled Raman transitions. The duration of the intense pump pulse that creates the Raman coherence is shorter than the…

化学物理 · 物理学 2009-11-10 S. A. Malinovskaya , P. H. Bucksbaum , P. R. Berman

We explain quantitatively why resonant Raman scattering spectroscopy, an extensively used experimental tool in studying elementary electronic excitations in doped low dimensional semiconductor nanostructures, always produces an observable…

强关联电子 · 物理学 2009-10-31 S. Das Sarma , Daw-Wei Wang

Stokes Raman scattering is known to be a particularly robust nonlinearity, occurring in virtually every material, with spectra defined by the material and strengths dependent on the material as well as light intensities. This ubiquity has…

光学 · 物理学 2021-08-10 Xiao Liu , Zelin Ma , Aku Antikainen , Siddharth Ramachandran

Raman scattering underlies a broad range of spectroscopic and light-generation techniques, yet its conventional description, based on the Raman gain spectrum, accurately describes only long-pulse, steady-state dynamics. We present a…

We theoretically propose a method to enhance Raman scattering by injecting a seeded light field which is correlated with the initially prepared atomic spin wave. Such a light-atom correlation leads to an interference in the Raman…

量子物理 · 物理学 2013-05-29 Chun-Hua Yuan , L. Q. Chen , Z. Y. Ou , Weiping Zhang

Raman spectroscopy is a powerful technique to characterize materials. It probes non-destructively chemical composition, crystallinity, defects, strain and coupling phenomena. However, the Raman response of surfaces or thin films is often…

Raman scattering is an excellent method for simultaneously determining the dynamics of lattice, spin, and charge degrees of freedom. Furthermore, polarization selection rules in Raman scattering enable momentum-resolved quasiparticle…

强关联电子 · 物理学 2024-09-04 Reshma Kumawat , Shubham Farswan , Simranjeet Kaur , Smriti Bhatia , Kaushik Sen

Raman spectroscopy reveals chemically specific information and provides label-free insight into the molecular world. However, the signals are intrinsically weak and call for enhancement techniques. Here, we demonstrate Purcell enhancement…

Quantum electrodynamics theory of the resonance Raman scattering is developed for an atom in a close proximity to a carbon nanotube. The theory predicts a dramatic enhancement of the Raman intensity in the strong atomic coupling regime to…

介观与纳米尺度物理 · 物理学 2015-12-07 I. V. Bondarev

We present an X-ray based stimulated Raman approach to control the preparation of optically dark electronic states in generic molecular systems. Leveraging on the unique properties of core-level excited states, we demonstrate that optically…

Iron-based superconducting layered compounds have the second highest transition temperature after cuprate superconductors. Their discovery is a milestone in the history of high-temperature superconductivity and will have profound…

超导电性 · 物理学 2012-10-11 A. M. Zhang , Q. M. Zhang

Raman scattering, an inelastic scattering mechanism, provides information about molecular excitation energies and can be used to identify chemical compounds. Albeit being a powerful analysis tool, especially for label-free biomedical…

光学 · 物理学 2018-10-12 Sebastian Karpf , Matthias Eibl , Wolfgang Wieser , Thomas Klein , Robert Huber
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