相关论文: Steady State Photoisomerization Quantum Yield of M…
Kinetic proofreading mechanisms explain the extraordinary accuracy observed in central biological events in terms of the enhanced specificity of substrate selection networks under a nonequilibrium environment. The nonequilibrium steady…
In chemical reactions, the interplay between coherent evolution and dissipation is central to determining key properties such as the rate and yield. Of particular interest are cases where two potential energy surfaces cross at features…
Processes that break molecular bonds are typically observed with molecules occupying a mixture of quantum states and successfully described with quasiclassical models, while a few studies have explored the distinctly quantum mechanical…
Nonequilibrium steady state of isothermal biochemical cycle kinetics has been extensively studied, but much less investigated under non-isothermal conditions. However, once the heat exchange between subsystems is rather slow, the isothermal…
A quantum model on the chemically and physically induced pluripotency in stem cells is proposed. Based on the conformational Hamiltonian and the idea of slow variables (molecular torsions) slaving fast ones the conversion from the…
We discuss how the thermalization of an elementary quantum system is modified when the system is placed in an environment out of thermal equilibrium. To this aim we provide a detailed investigation of the dynamics of an atomic system placed…
We consider the role of quantum effects in the transfer of hyrogen-like species in enzyme-catalysed reactions. This study is stimulated by claims that the observed magnitude and temperature dependence of kinetic isotope effects imply that…
The thermoelectric effect in a quantum dot system connected to two electron reservoirs in the presence of a photon cavity is investigated using a quantum master equation in the steady-state regime. If a quantized photon field is applied to…
Full quantum state tomography is used to characterize the state of an ensemble based qubit implemented through two hyperfine levels in Pr3+ ions, doped into a Y2SiO5 crystal. We experimentally verify that single-qubit rotation errors due to…
We study the energy distribution during the emergence of a quasi-equilibrium (QE) state in the course of relaxation to equipartition in slow-fast Hamiltonian systems. A bead-spring model where beads (masses) are connected by springs is…
We consider a finite quantum system S coupled to two environments of different nature. One is a heat reservoir R (continuous interaction) and the other one is a chain C of independent quantum systems E (repeated interaction). The…
Under certain conditions, focused laser excitation in semiconductor quantum well structures can lead to charge separation and a circular reaction front, which is visible as a ring-shaped photoluminescence pattern. The diffusion-reaction…
Photoisomerization, a photochemical process underlying many biological mechanisms, has been modeled recently within the quantum resource theory of thermodynamics. This approach has emerged as a promising tool for studying fundamental…
Cold molecules are important for many applications, from fundamental precision measurements, quantum information processing, quantum-controlled chemistry, to understanding the cold interstellar medium. Molecular ions are known to be cooled…
We report that under some specific conditions a single qubit model weakly interacting with information environments can be referred to as a quantum classifier. We exploit the additivity and the divisibility properties of the completely…
We follow the passage from complex amplitude bistability to phase bistability in the driven dissipative Jaynes-Cummings oscillator. Quasidistribution functions in the steady state are employed, for varying qubit-cavity detuning and drive…
The quantum Rabi model (QRM), composed of a qubit interacting with a quantized photonic field, is a cornerstone of quantum optics. The QRM with dominant unitary dynamics has been demonstrated in circuit quantum electrodynamics (QED)…
We develop a unified theoretical framework for the efficient description of multiphoton states generated and propagating in loop-based optical networks which contain nonlinear elements. These active optical components are modeled as…
A uniform minimal model of rhodopsin photoisomerization induced by either coherent laser light or low level incoherent light (e.g. moonlight) is provided. Realistic timescales for both processes, which differ by ten orders of magnitude, are…
This paper introduces a Lyapunov-based control approach with homodyne measurement. We study two filtering approaches: (i) the traditional quantum filtering and (ii) a modified version of the extended Kalman filtering. We examine both…