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While it is widely acknowledged that system-spanning particulate structures contribute to the observed yield stress and shear-thinning in attractive colloidal gels, a comprehensive understanding of the underlying microscopic mechanisms…

软凝聚态物质 · 物理学 2025-04-08 Rishabh More , Gareth Mckinley

Strong particulate gels are widely believed to behave poroelastically in compression, e.g. in sedimentation, even though they consolidate irreversibly because of the stickiness of the particles. Particulate gels are usually adhesive as well…

软凝聚态物质 · 物理学 2009-03-06 Richard Buscall

Dynamical heterogeneities in a colloidal fluid close to gelation are studied by means of computer simulations. A clear distinction between some fast particles and the rest, slow ones, is observed, yielding a picture of the gel composed by…

软凝聚态物质 · 物理学 2009-11-10 Antonio M. Puertas , Matthias Fuchs , Michael E. Cates

Simple models based on isotropic interparticle attractions often fail to capture experimentally observed structures of colloidal gels formed through spinodal decomposition and subsequent arrest: the resulting gels are typically denser and…

软凝聚态物质 · 物理学 2021-08-27 Jasper N. Immink , J. J. Erik Maris , Peter Schurtenberger , Joakim Stenhammar

The ordering of particles in the drying process of a colloidal suspension is crucial in determining the properties of the resulting film. For example, microscopic inhomogeneities can lead to the formation of cracks and defects that can…

软凝聚态物质 · 物理学 2021-10-04 Maarten Wouters , Othmane Aouane , Marcello Sega , Jens Harting

Extreme deformation of soft matter is central to our understanding of the effects of shock, fracture, and phase change in a variety of systems. Yet, despite, the increasing interest in this area, far-from-equilibrium behaviours of soft…

软凝聚态物质 · 物理学 2020-07-07 Axel Huerre , Marco De Corato , Valeria Garbin

The macroscopic mechanical properties of densely packed coagulated colloidal particle gels strongly depend on the local arrangement of the powder particles on length scales of a few particle diameters. Heterogeneous microstructures exhibit…

软凝聚态物质 · 物理学 2009-11-09 Iwan Schenker , Frank T. Filser , Tomaso Aste , Ludwig J. Gauckler

Soft materials, such as colloidal suspensions, polymer solutions, and biological systems, are typically multicomponent mixtures of macromolecules and simpler components (e.g., microions, monomers, solvent) that can assemble into complex…

软凝聚态物质 · 物理学 2015-05-13 Alan R. Denton

Particles added to a fluid interface can be used as a surface stabilizer in the food, oil and cosmetic industries. As an alternative to rigid particles, it is promising to consider highly deformable particles that can adapt their…

软凝聚态物质 · 物理学 2016-10-27 Hadi Mehrabian , Jens Harting , Jacco H. Snoeijer

Thermosensitive microgels are widely studied hybrid systems combining properties of polymers and colloidal particles in a unique way. Due to their complex morphology their interactions and packing, and consequentially the viscoelastcity of…

软凝聚态物质 · 物理学 2019-06-19 Gaurasundar M. Conley , James L. Harden , Frank Scheffold

Colloidal gels are out of equilibrium soft solids composed of attractive Brownian particles that form a space-spanning network at low volume fractions. The elastic properties of these systems result from the network microstructure, which is…

We discuss a class of models for particulate gels in which the particle contacts are described by an effective interaction combining a two-body attraction and a three-body angular repulsion. Using molecular dynamics, we show how varying the…

软凝聚态物质 · 物理学 2021-08-05 Minaspi Bantawa , Wayan A. Fontaine-Seiler , Peter D. Olmsted , Emanuela Del Gado

Dense suspensions of soft colloidal particles display a broad range of physical and rheological properties which are still far from being fully understood. To elucidate the role of deformability on colloidal flow, we employ computer…

软凝聚态物质 · 物理学 2018-08-31 M. Foglino , A. N. Morozov , D. Marenduzzo

Foams made of complex fluids such as particle suspensions have a great potential for the development of advanced aerated materials. In this paper we study the rheological behavior of liquid foams loaded with granular suspensions. We focus…

软凝聚态物质 · 物理学 2017-04-26 François Gorlier , Yacine Khidas , Abdoulaye Fall , Olivier Pitois

We consider the sedimentation of a colloidal gel under confinement in the direction of gravity. The confinement allows us to compare directly experiments and computer simulations, for the same system size in the vertical direction. The…

Soft materials such as colloidal suspensions, polymer solutions and liquid crystals are constituted by mesoscopic entities held together by weak forces. Their mechanical moduli are several orders of magnitude lower than those of atomic…

软凝聚态物质 · 物理学 2015-06-16 Ranjini Bandyopadhyay

We consider an elastic composite material containing particulate inclusions in a soft elastic matrix that is bounded by a rigid wall, e.g., the substrate. If such a composite serves as a soft actuator, forces are imposed on or induced…

软凝聚态物质 · 物理学 2017-05-12 Andreas M. Menzel

Colloidal dispersions are prized as model systems to understand basic properties of materials, and are central to a wide range of industries from cosmetics to foods to agrichemicals. Among the key developments in using colloids to address…

软凝聚态物质 · 物理学 2022-06-22 Jun Dong , Francesco Turci , Robert L. Jack , Malcolm A. Faers , C. Patrick Royall

We consider a dilute system of small hard beads or hard fibers immersed in a very soft gel able to withstand large elastic deformations. Because of its low to very low shear modulus, this system is very sensitive to small forces. We…

软凝聚态物质 · 物理学 2014-05-05 Serge Mora , Yves Pomeau

We present a simulation study of colloidal particles having very short range attractions. In particular, we investigate the interplay between the effective attractive range and the viscoelastic properties of the gels that form when the…

软凝聚态物质 · 物理学 2013-07-16 P. H. S. Santos , O. H. Campanella , M. A. Carignano