相关论文: Giant chiro-optical response in high harmonic gene…
Strongly driven systems of emitters offer an attractive source of light over broad spectral ranges up to the X-ray region. A key limitation of these systems is that the light they emit is for the most part classical. We challenge this…
High-harmonic spectroscopy driven by circularly-polarized laser pulses and their counter-rotating second harmonic is a new branch of attosecond science which currently lacks quantitative interpretations. We extend this technique to the…
An analytic description of high harmonic generation (HHG) in solids induced by intense low-frequency pulses is presented within an adiabatic approach, which treats laser-matter interactions nonperturbatively. We derive the analytical…
High-order harmonic generation is a powerful and sensitive tool for probing atomic and molecular structures, combining in the same measurement an unprecedented attosecond temporal resolution with a high spatial resolution, of the order of…
Attosecond light sources based on high-order harmonic generation (HHG) constitute to date the only table-top solution for producing coherent broadband radiation covering the spectral range from the extreme ultraviolet to the soft X-rays.…
Bianisotropy is a powerful concept enabling asymmetric optical response, including asymmetric reflection, absorption, optical forces, light trapping, and lasing. The physical origin of these asymmetric effects can be understood from…
The influence of large permanent dipoles on molecular orbital tomography via high-order harmonic generation (HHG) is investigated in this work. It is found that, owing to the modification of the angle-dependent ionization rate resulting…
Chiral quantum optics is a growing field of research where light-matter interactions become asymmetrically dependent on momentum and spin, offering novel control over photonic and electronic degrees of freedom. Recently, the platforms for…
Second-harmonic generation (SHG) is a fundamental nonlinear optical process widely used in photonics; however, it is strictly forbidden in the bulk of centrosymmetric materials due to their inversion symmetry. Nevertheless, applying an…
In high harmonic generation (HHG), non-dipole effects become increasingly significant at long driving wavelengths, as the magnetic field leads to a lateral drift of the continuum electron, which disrupts the electron recollision and…
High-harmonic generation (HHG) in solids has rapidly emerged as a promising platform for creating compact attosecond sources and probing ultrafast electron dynamics. Resonant metasurfaces are essential for enhancement of the otherwise small…
Chirality, a fundamental concept describing an object cannot superpose with its mirror image, is crucial in optics and photonics and leads to various exotic phenomena, such as circular dichroism, and optical activity. Recent findings reveal…
We introduce and theoretically analyze the concept of manipulating optical chirality via strong coupling of the optical modes of chiral nanostructures with excitonic transitions in molecular layers or semiconductors. With chirality being…
Chiral light-matter interactions have traditionally been understood in terms of electric-magnetic dipolar interference driven by light with spin angular momentum. Here, we show that optical chirality can also originate from the orbital…
The Quantitative Rescattering Theory (QRS) for high-order harmonic generation (HHG) by intense laser pulses is presented. According to the QRS, HHG spectra can be expressed as a product of a returning electron wave packet and the…
We report about the experimental observation and characterization of nonlinear optical properties of individual silicon nanowires of different dimensions. Our results show that the nonlinear light has different components, one of them…
Accelerating and colliding particles has been a key strategy to explore the texture of matter. Strong lightwaves can control and recollide electronic wavepackets, generating high-harmonic (HH) radiation which encodes the structure and…
In quantum optics, it is common to assume that atoms are point-like objects compared to the wavelength of the electromagnetic field they interact with. However, this dipole approximation is not always valid, e.g., if atoms couple to the…
We develop a theoretical framework for high-harmonic generation (HHG) driven by quantum states of light based on a temporal-mode expansion of the electromagnetic field. This approach extends previous single plane-wave mode treatments to…
We theoretically investigate circular dichroism (CD) in second- and third-harmonic generation (SHG and THG) in the chiral topological semimetal CoSi. We demonstrate that both SHG and THG exhibit dichroic responses of order unity, while…