High-harmonic generation driven by temporal-mode quantum states of light
Abstract
We develop a theoretical framework for high-harmonic generation (HHG) driven by quantum states of light based on a temporal-mode expansion of the electromagnetic field. This approach extends previous single plane-wave mode treatments to realistic pulse configurations, resolving conceptual inconsistencies arising from non-normalizable infinite plane waves and establishing consistency between analytical and numerical methods. We derive a correction factor that quantifies deviations from the single-mode approximation and show that it remains below for intensities typical of HHG (W/cm). This result confirms that free-space HHG driven by any quantum state of light is accurately described by averaging semi-classical calculations over the Husimi distribution, with no observable genuine quantum effects. The absence of such effects is attributed to the large photon numbers () required to reach HHG intensities in free space, which render quantum fluctuations negligible. We discuss nanophotonic environments with ultrasmall mode volumes as potential platforms where few-photon strong-field processes could exhibit genuine quantum signatures.
Cite
@article{arxiv.2512.06602,
title = {High-harmonic generation driven by temporal-mode quantum states of light},
author = {Juan M. González-Monge and Johannes Feist},
journal= {arXiv preprint arXiv:2512.06602},
year = {2025}
}