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In addition to their strong nonlinear optical response, transition metal dichalcogenides (TMDCs) possess a high refractive index in the visible and infrared regime. Therefore, by patterning those TMDCs into dielectric nanoresonators, one…

Twisted transition metal dichalcogenides (TMDs) present an intriguing platform for exploring excitons and their transport properties. By introducing a twist angle, a moir\'e superlattice forms, providing a spatially dependent exciton energy…

介观与纳米尺度物理 · 物理学 2024-01-17 Willy Knorr , Samuel Brem , Giuseppe Meneghini , Ermin Malic

Transition metal dichalcogenides (TMDs), such as MoS$_2$, are known to undergo a structural phase transformation as well as a change in the electronic conductivity upon Li intercalation. These properties make them candidates for…

材料科学 · 物理学 2021-07-28 C. D. Spataru , M. D. Witman , R. E. Jones

Cross-plane thermal conductivity in homogeneous transition metal dichalcogenides (TMDs) exhibits a strong dependence on twist angle, originating from atomic reconstruction within moir\'e superlattices. This reconstruction redistributes…

材料科学 · 物理学 2025-05-02 Wenwu Jiang , Ting Liang , Hekai Bu , Jianbin Xu , Wengen Ouyang

It is of fundamental importance but challenging to simultaneously identify atomic and magnetic configurations of two-dimensional van der Waals materials. In this work, we show that the nonreciprocal second-harmonic generation (SHG) can be a…

材料科学 · 物理学 2020-07-15 Wenshen Song , Ruixiang Fei , Li Yang

The polarization analysis of optical transitions in monolayer and bilayer transition-metal dichalcogenides provides invaluable information on the spin and valley (pseudospin) degrees of freedom. To explain optical properties of a given…

材料科学 · 物理学 2015-10-06 Hanan Dery , Yang Song

High-order harmonic generation (HHG) is a fundamental process which can be simplified as the production of high energetic photons from a material subjected to a strong driving laser field. This highly nonlinear optical process contains rich…

光学 · 物理学 2021-12-21 Dasol Kim , Yeon Lee , Alexis Chacón , Dong Eon Kim

Motivated by the recent excitement around the physics of twisted transition metal dichalcogenide (TMD) multilayer systems, we study strongly correlated phases of TMD heterobilayers under the influence of light. We consider both waveguide…

强关联电子 · 物理学 2022-12-20 Michael Vogl , Swati Chaudhary , Gregory A. Fiete

Two-dimensional layered materials offer the possibility to create artificial vertically stacked structures possessing an additional degree of freedom - $the$ $interlayer$ $twist$. We present a comprehensive optical study of artificially…

Mott-Hubbard and Hund electron correlations have been realized thus far in separate classes of materials. Here, we show that a single moir\'e homobilayer encompasses both kinds of physics in a controllable manner. We develop a microscopic…

强关联电子 · 物理学 2023-01-26 Siheon Ryee , Tim O. Wehling

We theoretically investigate detuning-dependent properties of high-order harmonic generation (HHG) in monolayer transition metal dichalcogenides (TMDCs). In contrast to HHG in conventional materials, TMDCs show both parallel and…

材料科学 · 物理学 2018-04-18 Tomohiro Tamaya , Satoru Konabe , Shiro Kawabata

Optical harmonic generation on excitons is found in ZnSe/BeTe quantum wells with type-II band alignment. Two experimental approaches with spectrally-broad femtosecond laser pulses and spectrally-narrow picosecond pulses are used for…

We present a comprehensive theoretical investigation of the photo-generated excitons in transition-metal dichalcogenide monolayers (TMD-ML's) by Laguerre-Gaussian beams, a celebrated kind of twisted lights (TL's) carrying quantized orbital…

介观与纳米尺度物理 · 物理学 2022-03-07 Guan-Hao Peng , Oscar Javier Gomez Sanchez , Wei-Hua Li , Ping-Yuan Lo , Shun-Jen Cheng

In 1H monolayer transition metal dichalcogenide, the inversion symmetry is broken, while the reflection symmetry is maintained. On the contrary, in the bilayer, the inversion symmetry is restored, but the reflection symmetry is broken. As a…

Moir\'e excitons are emergent optical excitations in 2D semiconductors with deep moir\'e superlattice potentials. While these excitations have been realized in several platforms, a system with dynamically tunable moir\'e potential to tailor…

We theoretically investigate the second harmonic generation (SHG) of topological insulator surface states in a perpendicular magnetic field. Our theory is based on the microscopic expression of the second-order magneto-optical conductivity…

介观与纳米尺度物理 · 物理学 2024-11-27 Kainan Chang , Muhammad Zubair , Jin Luo Cheng , Wang-Kong Tse

Moir\'e superlattices in van der Waals heterostructures provide a tunable platform to study emergent properties that are absent in the natural crystal form. Twisted bilayer transition metal dichalcogenides (TB-TMDs) can host moir\'e flat…

介观与纳米尺度物理 · 物理学 2021-09-27 En Li , Jin-Xin Hu , Xuemeng Feng , Zishu Zhou , Liheng An , Kam Tuen Law , Ning Wang , Nian Lin

Monolayer transition metal dichalcogenides (TMDs) exhibit high nonlinear optical (NLO) susceptibilities. Experiments on MoS$_2$ have indeed revealed very large second-order ($\chi^{(2)}$) and third-order ($\chi^{(3)}$) optical…

Recent experiments in twisted bilayer transition-metal dichalcogenides have revealed a variety of strongly correlated phenomena. To theoretically explore their origin, we combine here ab initio calculations with correlated model approaches…

强关联电子 · 物理学 2025-10-03 Marta Brzezińska , Sergii Grytsiuk , Malte Rösner , Marco Gibertini , Louk Rademaker

Exciton-phonon interactions in transition metal dichalcogenides (TMD) are strong and lead to phenomena such as coherent phonon generation. When stacked and twisted, their properties can be tuned by the twisting angle. In experiments with…

材料科学 · 物理学 2026-05-01 Rafael R. Del Grande , David A. Strubbe
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