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相关论文: Emergent interlayer magnetic order via strain-indu…

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Symmetric anisotropic interaction can be ferromagnetic and antiferromagnetic at the same time but for different crystallographic axes. We show that inducing competition of anisotropic interactions of orthogonal irreducible representations…

强关联电子 · 物理学 2022-07-11 S. Pandey , H. Zhang , J. Yang , A. F. May , J. Sanchez , Z. Liu , J. -H. Chu , J. W. Kim , P. J. Ryan , H. D. Zhou , J. Liu

With decreasing temperature Sr$_2$VO$_4$ undergoes two structural phase transitions, tetragonal-to-orthorhombic-to-tetragonal, without long-range magnetic order. Recent experiments suggest, that only at very low temperature Sr$_{2}$VO$_{4}$…

材料科学 · 物理学 2017-11-15 Bongjae Kim , Sergii Khmelevskyi , Peter Mohn , Cesare Franchini

Layered 5$d$ transition iridium oxides, Sr$_2$(Ir,Rh)O$_4$, are described as unconventional Mott insulators with strong spin-orbit coupling. The undoped compound, Sr$_2$IrO$_4$, is a nearly ideal two-dimensional pseudospin-$1/2$ Heisenberg…

强关联电子 · 物理学 2017-05-02 Jaehong Jeong , Yvan Sidis , Alex Louat , Véronique Brouet , Philippe Bourges

The layered 5d transition metal oxide Sr2IrO4 has been shown to host a novel Jeff=1/2 Mott spin orbit insulating state with antiferromagnetic ordering, leading to comparisons with the layered cuprates. Here we study the effect of…

强关联电子 · 物理学 2015-03-20 S. Calder , G. -X. Cao , M. D. Lumsden , J. W. Kim , Z. Gai , B. C. Sales , D. Mandrus , A. D. Christianson

In this work, we report observation of strain effect on physical properties of Sr2IrO4 thin films grown on SrTiO3 (001) and LaAlO3 (001) substrates. It is found that the film on LaAlO3 with compressive strain has a lower antiferromagnetic…

强关联电子 · 物理学 2023-09-19 N. Hu , Y. K. Weng , K. Chen , B. You , Y. Liu , Y. T. Chang , R. Xiong , S. Dong , C. L. Lu

The orbital, which represents the shape of the electron cloud, very often strongly influences the manifestation of various exotic phenomena, e.g., magnetism, metal-insulator transition, colossal magnetoresistance, unconventional…

Sr2IrO4 and Sr3Ir2O7 form two families of spin-orbit Mott insulators with quite different charge gaps and an antiferromagnetic (AF) ground state. This offers a unique opportunity to study the impact of long-range magnetic order in Mott…

We investigate the magnetic properties of the series Sr2Ir1-xRuxO4 with neutron, resonant x-ray and magnetization measurements. The results indicate an evolution and coexistence of magnetic structures via a spin flop transition from…

We used single-crystal x-ray and neutron diffraction to investigate the crystal and magnetic structures of trigonal lattice iridate Ca2Sr2IrO6. The crystal structure is determined to be $R\bar3$ with two distinct Ir sites. The system…

High quality epitaxial thin films of Jeff=1/2 Mott insulator Sr2IrO4 with increasing in-plane tensile strain have been grown on top of SrTiO3(001) substrates. Increasing the in-plane tensile strain up to ~0.3% was observed to drop the c/a…

Using resonant x-ray diffraction, we observe an easy c-axis collinear antiferromagnetic structure for the bilayer Sr$_3$Ir$_2$O$_7$, a significant contrast to the single layer Sr$_2$IrO$_4$ with in-plane canted moments. Based on a…

强关联电子 · 物理学 2012-12-11 J. W. Kim , Y. Choi , Jungho Kim , J. F. Mitchell , G. Jackeli , M. Daghofer , J. van den Brink , G. Khaliullin , B. J. Kim

We discuss the notions of spin-orbital polarization and ordering in paramagnetic materials, and address their consequences in transition metal oxides. Extending the combined density functional and dynamical mean field theory scheme to the…

强关联电子 · 物理学 2014-12-16 Cyril Martins , Markus Aichhorn , Loig Vaugier , Silke Biermann

Symmetry engineering is explicitly effective to manipulate and even create phases and orderings in strongly correlated materials. Flexural stress is universally practical to break the space-inversion or time-reversal symmetry. Here, by…

Sr2IrO4 is one of the prime candidates for realizing exotic quantum spin orders owing to the subtle combination of spin-orbit coupling and electron correlation. Sensitive local magnetization measurement can serve as a powerful tool to study…

材料科学 · 物理学 2025-03-26 Hyeokjun Heo , Jeongha An , Junyoung Kwon , Kwangrae Kim , Youngoh Son , B. J. Kim , Joonho Jang

Protected by the interplay of on-site Coulomb interactions and spin-orbit coupling, Sr$_2$IrO$_4$ at high pressure is a rare example of a Mott insulator with a paramagnetic ground state. Here, using optical Raman scattering, we measure both…

We performed resonant and nonresonant x-ray diffraction studies of a Nd0.5Sr0.5MnO3 thin film that exhibits a clear first-order transition. Lattice parameters vary drastically at the metal-insulator transition at 170K (=T_MI), and…

强关联电子 · 物理学 2009-11-11 Y. Wakabayashi , D. Bizen , H. Nakao , Y. Murakami , M. Nakamura , Y. Ogimoto , M. Izumi , K. Miyano , H. Sawa

We have carried out Raman spectroscopy experiments to investigate two-magnon excitations in epitaxial thin films of the quasi-two-dimensional antiferromagnetic Mott insulator Sr$_2$IrO$_4$ under in-plane misfit strain. With in-plane biaxial…

X-ray and Neutron diffraction as well as muon spin relaxation and M\"ossbauer experiments performed on SrFe$_2$As$_2$ polycrystalls confirm a sharp first order transition at $T_0 = 205$,K corresponding to an orthorhombic phase distortion…

In the high spin-orbit coupled Sr2IrO4, the high sensitivity of the ground state to the details of the local lattice structure shows a large potential for the manipulation of the functional properties by inducing local lattice distortions.…

Sr4Ru3O10 is a Ruddlesden-Popper compound with triple Ru-O perovskite layers separated by Sr-O alkali layers. This compound presents a rare coexistence of interlayer (c-axis) ferromagnetism and intralayer (basal-plane) metamagnetism at…

强关联电子 · 物理学 2018-08-29 H. Zheng , W. H. Song , J. Terzic , H. D. Zhao , Y. Zhang , Y. F. Ni , L. E. DeLong , P. Schlottmann , G. Cao
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