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We investigate the infrared optical transitions between excitons of the yellow, green and blue series in the cuprous oxide Cu$_{\mathrm{2}}$O. We show that in many cases the dipole approximation is inadequate and, in particular, that it…

介观与纳米尺度物理 · 物理学 2019-08-05 Sjard Ole Krüger , Stefan Scheel

We experimentally and numerically investigate the exchange interaction of the yellow excitons in cuprous oxide. By varying the material parameters in the numerical calculations, we can interpret experimental findings and understand their…

材料科学 · 物理学 2021-02-19 Patric Rommel , Jörg Main , Andreas Farenbruch , Dmitri R. Yakovlev , Manfred Bayer

When an electron in a semiconductor gets excited to the conduction band the missing electron can be viewed as a positively charged particle, the hole. Due to the Coulomb interaction electrons and holes can form a hydrogen-like bound state…

介观与纳米尺度物理 · 物理学 2024-10-03 Jan Ertl , Sebastian Rentschler , Jörg Main

The complex valence band structure of bulk cuprous oxide necessitates going beyond the parabolic approximation to precisely estimate exciton binding energies. The same is true for excitons in cuprous oxide quantum wells, for which many…

介观与纳米尺度物理 · 物理学 2026-03-13 Niklas Scheuler , Jörg Main , Patric Rommel , Frieder Pfeiffer , Stefan Scheel , Pavel A. Belov

We numerically investigate the odd parity states of the green exciton series in cuprous oxide. Taking into account the coupling to the yellow series and especially to the yellow continuum, the green excitons are quasi-bound resonances with…

材料科学 · 物理学 2020-03-02 Patric Rommel , Patrik Zielinski , Jörg Main

Recent high-resolution absorption spectroscopy on excited excitons in cuprous oxide [Nature (London) 514, 343 (2014)] has revealed significant deviations of their spectrum from that of the ideal hydrogen-like series. Here we show that the…

We report experimental and theoretical investigations of interacting excitons of the yellow series in cuprous oxide (Cu$_2$O) with principal quantum numbers up to $n=7$ by means of second harmonic generation (SHG). Using picosecond pulsed…

Excitons with a radius of a few lattice constants can be affected by strong central-cell corrections, leading to significant deviations of the optical spectrum from the hydrogen-like Rydberg series, and also to an enhancement of the exciton…

材料科学 · 物理学 2018-01-30 Andreas Alvermann , Holger Fehske

Excitons, as bound states of electrons and holes, embody the solid state analogue of the hydrogen atom, whose quantum spectrum is explained within a classical framework by the Bohr-Sommerfeld atomic model. In a first hydrogenlike…

介观与纳米尺度物理 · 物理学 2024-04-17 Jan Ertl , Michael Marquardt , Moritz Schumacher , Patric Rommel , Jörg Main , Manfred Bayer

We report on the observation of the yellow exciton Lyman series up to the fourth term in Cu2O by time-resolved mid-infrared spectroscopy. The dependence of the oscillator strength on the principal quantum number n can be well reproduced…

材料科学 · 物理学 2009-11-11 Takeshi Tayagaki , Andre Mysyrowicz , Makoto Kuwata-Gonokami

Recent experiments on trilayer transition-metal dichalcogenide heterostructures have revealed the rich behavior of dipolar excitons. Motivated by these experimental observations, we investigate the collective dynamics of planar quantum…

介观与纳米尺度物理 · 物理学 2025-12-19 Michal Zimmerman , Daniel Podolsky , Ronen Rapaport , Snir Gazit

We study the absorption spectra of the yellow excitons in Cu$_2$O in high magnetic fields using polarization-resolved optical absorption measurements with a high frequency resolution. We show that the symmetry of the yellow exciton results…

The recent observation of dipole-allowed $P$-excitons up to principal quantum numbers of $n=25$ in cuprous oxide has given insight into exciton states with unprecedented spectral resolution. While so far the exciton description as a…

We calculate the spectrum of interlayer neutral excitons in transition-metal-dichalcogenide WeSe$_2$/MoSe$_2$ heterobilayers in the $R$-stacking configuration. Most saliently, we show that, similarly to neutral excitons and trions in…

介观与纳米尺度物理 · 物理学 2024-08-09 Houssem Eddine Hannachi , Mark-Oliver Goerbig , Sihem Jaziri

We theoretically demonstrate the formation of multiple bi-stability regions in the temperature pattern on the interface between a cuprous oxide quantum well and DCM2:CA:PS organic compound. The Frenkel molecular exciton of the DCM2 is…

材料科学 · 物理学 2009-11-13 Oleksiy Roslyak , Joseph L. Birman

In this paper we present a study of an exciton system where electrons and holes are confined in double quantum well structures. The dominating interaction between excitons in such systems is a dipole - dipole repulsion. We show that the…

量子气体 · 物理学 2015-05-13 B. Laikhtman , R. Rapaport

A resonant inelastic x-ray scattering study of the electronic structure of the semiconductor cuprous oxide, $\rm Cu_2O$, is reported. When the incident x-ray energy is tuned to the Cu K-absorption edge, large enhancements of the spectral…

材料科学 · 物理学 2012-06-18 Young-June Kim , J. P. Hill , H. Yamaguchi , T. Gog , D. Casa

We study a family of excitonic quantum phase transitions describing the evolution of a bilayer metallic state to an inter-layer coherent state where excitons condense. We argue that such transitions can be continuous and exhibit a non-Fermi…

强关联电子 · 物理学 2024-06-28 Zhengyan Darius Shi , Hart Goldman , Zhihuan Dong , T. Senthil

In this paper, we study the third-order nonlinear optical response due to transitions between excitonic levels in two-dimensional transition metal dichalcogeniedes. To accomplish this, we use methods not applied to the description of…

介观与纳米尺度物理 · 物理学 2021-06-14 J. C. G. Henriques , Høgni C. Kamban , Thomas G. Pedersen , N. M. R. Peres

Coulomb bound electron-hole pairs, excitons, govern the optical properties of semi-conducting transition metal dichalcogenides like MoS$_2$ and WSe$_2$. We study optical transitions at the K-point for 2H homobilayer MoS$_2$ in Density…

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