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We report on isothermal magnetization, M\"ossbauer spectroscopy, and magnetostriction as well as temperature-dependent alternating-current (ac) susceptibility, specific heat, and thermal expansion of single crystalline and polycrstalline…

We report a comprehensive high-field/high-frequency electron spin resonance (ESR) study on single crystals of the van der Waals magnet CrCl$_3$. This material, although being known for quite a while, has received recent significant…

材料科学 · 物理学 2020-06-09 J. Zeisner , K. Mehlawat , A. Alfonsov , M. Roslova , T. Doert , A. Isaeva , B. Büchner , V. Kataev

We present detailed ESR investigations on single crystals of the low-dimensional quantum magnet TiOCl. The anisotropy of the g-factor indicates a stable orbital configuration below room temperature, and allows to estimate the energy of the…

In this work, we report on the thermomagnetic characterization and crystalline-electric field (CEF) energy scheme of the disordered defect-fluorite Ho2Zr2O7. This structural phase is distinguished by the coexistence of magnetic frustration…

The phase diagrams of EuFe$_{2-x}$Co$_x$As$_2$ $(0 \leq x \leq 0.4)$ and EuFe$_2$As$_{2-y}$P$_y$ $(0 \leq y \leq 0.43)$ are investigated by Eu$^{2+}$ electron spin resonance (ESR) in single crystals. From the temperature dependence of the…

We performed high-field magnetization, magnetocaloric effect (MCE), and NMR measurements on the Ising triangular-lattice antiferromagnet Rb$_2$Co(SeO$_3$)$_2$. The observations of the 1/3-magnetization plateau, the split NMR lines, and the…

We present comprehensive electron spin resonance (ESR) studies of in-plane oriented single crystals of $\alpha$-RuCl$_3$, a quasi-two-dimensional material with honeycomb structure, focusing on its high-field spin dynamics. The measurements…

CsYbSe$_2$, a recently identified quantum spin liquid (QSL) candidate, exhibits strong crystal electric field (CEF) excitations. Here, we identify phonon and CEF modes with Raman spectroscopy and observe strong CEF-phonon mixing resulting…

Measurements of the coefficient of thermal expansion on the spin-liquid candidate $\kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$ have revealed distinct and strongly anisotropic lattice effects around 6 K - a possible spin-liquid instability. In…

强关联电子 · 物理学 2012-05-09 Rudra Sekhar Manna , Mariano de Souza , John A. Schlueter , Michael Lang

We have investigated the non-centrosymmetric tetragonal heavy-fermion compound CeAuAl3 using muon spin rotation (muSR), neutron diffraction (ND) and inelastic neutron scattering (INS) measurements. We have also revisited the magnetic,…

The magnetic excitation spectrum of the unconventional ferromagnet CeRh$_{3}$B$_{2}$ was measured by inelastic neutron scattering on single crystal sample in the magnetically ordered and paramagnetic phases. The spin-wave excitation…

强关联电子 · 物理学 2012-02-29 S. Raymond , J. Panarin , F. Givord , A. P. Murani , J. X. Boucherle , P. Lejay

M\"ossbauer spectroscopy was used to probe the site specific information of the $K_{0.84}Fe_{1.99}Se_2$ superconductor. Possibility of coexistence of superconductivity and magnetism is discussed. A spin excitation gap, $\Delta E…

超导电性 · 物理学 2012-04-03 Zhiwei Li , Xiaoming Ma , Hua Pang , Fashen Li

We report specific heat ($C$) and magnetization ($M$) of single crystalline Ce$_4$Pt$_{12}$Sn$_{25}$ at temperature down to $\sim$50mK and in fields up to 3T. $C/T$ exhibits a sharp anomaly at 180mK, with a large $\Delta…

We investigate the magnetic field dependence of the physical properties of f^2-configuration systems with a crystalline-electric field (CEF) singlet ground state, which gives rise to a non- Fermi liquid (NFL) fixed point due to the…

强关联电子 · 物理学 2015-03-19 Shinya Nishiyama , Kazumasa Miyake

Using linear-response density-functional theory, magnetic excitations in the striped phase of CaFe$_{2}$As$_{2}$ are studied as a function of local moment amplitude. We find a new kind of excitation: sharp resonances of Stoner-like…

材料科学 · 物理学 2012-09-11 L. Ke , M. van Schilfgaarde , J. J. Pulikkotil , T. Kotani , V. P. Antropov

We have studied the magnetism of the Pr3+ ions in PrFeAsO_1-xF_x (x = 0; 0.15) and its interaction with the Fe magnetic order (for x = 0). Specific heat data confirm the presence of a first excited crystal electric field (CEF) level around…

超导电性 · 物理学 2015-06-05 U. Stockert , N. Leps , L. Wang , G. Behr , S. Wurmehl , B. Büchner , R. Klingeler

Temperature dependent electron spin resonance (ESR) measurements are reported on stage 1 potassium doped graphite, a model system of biased graphene. The ESR linewidth is nearly isotropic and although the g-factor has a sizeable anisotropy,…

The physical properties of the semiconductor FeSi with very narrow band gap, anomalous behavior of the magnetic susceptibility and metal-insulator transition at elevated temperatures attract gross interest due to the still controversial…

强关联电子 · 物理学 2018-09-26 Sergii Khmelevskyi , Georg Kresse , Peter Mohn

A significant number of Kondo-lattice ferromagnets order perpendicular to the easy magnetization axis dictated by the crystalline electric field. The nature of this phenomenon has attracted considerable attention, but remains poorly…

强关联电子 · 物理学 2021-10-04 S. E. Nikitin , A. Podlesnyak , J. Xu , D. Voneshen , M. Duc Le , S. L. Bud'ko , P. C. Canfield , D. A. Sokolov

The strong coupling between spin, lattice and electronic degrees of freedom in magnetic materials can produce interesting phenomena, including multiferroic and magnetodielectric (MD) behavior, and exotic coupled excitations, such as…

强关联电子 · 物理学 2019-05-08 A. Sethi , J. E. Slimak , T. Kolodiazhnyi , S. L. Cooper