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Using the sensitivity of magneto-induced second harmonic generation to spin currents (SC), we demonstrate in Fe/Au/Fe/MgO(001) pseudo spin valves the generation of 250 fs-long SC pulses. Their temporal profile indicates that superdiffusive…

A time domain approach to probe hot carrier-induced spin dynamics is demonstrated. The experiments are performed in epitaxial Au/Fe/MgO(001), where spin-polarized hot carriers are excited in the Fe layer by 35 fs laser pulses. They…

This paper is concerned with a theoretical analysis of the behavior of optically excited spin currents in bilayer and multilayer systems of ferromagnetic and normal metals. As the propagation, control and manipulation of the spin currents…

介观与纳米尺度物理 · 物理学 2023-08-16 J. Briones , M. Weber , B. Stadtmüller , H. C. Schneider , B. Rethfeld

In condensed matter, scattering processes determine the transport of charge carriers. In case of heterostructures, interfaces determine many dynamic properties like charge transfer and transport and spin current dynamics. Here we discuss…

We describe a theoretical approach for spin-polarized hot-electron transport, as it occurs after excitation by ultrafast optical pulses in heterostructures formed by ferromagnetic and normal metals. We formulate a spin-dependent…

材料科学 · 物理学 2018-12-19 Dennis M. Nenno , Bärbel Rethfeld , Hans Christian Schneider

In spin-based electronics, information is encoded by the spin state of electron bunches. Processing this information requires the controlled transport of spin angular momentum through a solid, preferably at frequencies reaching the so far…

介观与纳米尺度物理 · 物理学 2013-09-03 T. Kampfrath , M. Battiato , P. Maldonado , G. Eilers , J. Nötzold , I. Radu , F. Freimuth , Y. Mokrousov , S. Blügel , M. Wolf , P. M. Oppeneer , M. Münzenberg

The idea to utilize not only the charge but also the spin of electrons in the operation of electronic devices has led to the development of spintronics, causing a revolution in how information is stored and processed. A novel advancement…

介观与纳米尺度物理 · 物理学 2016-02-10 T. J. Huisman , R. V. Mikhaylovskiy , J. D. Costa , F. Freimuth , E. Paz , J. Ventura , P. P. Freitas , S. Blügel , Y. Mokrousov , Th. Rasing , A. V. Kimel

The generation of short spin-current pulses is essential for fast spintronic devices. So far, spin current pulses are generated by femtosecond laser pulses which drive spins from a ferromagnetic metal layer. However, the need for…

介观与纳米尺度物理 · 物理学 2023-12-22 Piotr Graczyk , Maria Pugaczowa-Michalska , Maciej Krawczyk

Ultrafast demagnetization induced by femtosecond laser pulses in thin metallic layers is caused by the outflow of spin-polarized hot electron currents describable by the superdiffusive transport model. These laser-generated spin currents…

介观与纳米尺度物理 · 物理学 2023-05-24 Pavel Baláž , Maciej Zwierzycki , Francesco Cosco , Karel Carva , Pablo Maldonado , Peter M. Oppeneer

A systematic investigation of spin injection behavior in Au/FM (FM = Fe and Ni) multilayers is performed using the superdiffusive spin transport theory. By exciting the nonmagnetic layer, the laser-induced hot electrons may transfer spin…

介观与纳米尺度物理 · 物理学 2023-11-20 Wen-Tian Lu , Zhe Yuan , Xiaohong Xu

The transport of optically excited, hot electrons in heterostructures is analyzed by femtosecond, time-resolved two-photon photoelectron emission spectroscopy (2PPE) for epitaxial Au/Fe/MgO(001). We compare the temporal evolution of the…

Understanding the microscopic spatio-temporal dynamics of nonequilibrium charge carriers in heterosystems promises optimization of process and device design towards desired energy transfer. Hot electron transport is governed by scattering…

Ultrashort spin current pulses have a great potential of becoming the carriers of information in future ultrafast spintronics. They present the outstanding property of an extremely compressed time profile, which can allow for the building…

材料科学 · 物理学 2018-03-28 Marco Battiato

We provide a complete toolkit for coherent control experiments on the nano-scale. By exploiting the second harmonic emission from single (150 nm) nonlinear nano-particles, we show that ultrafast femtosecond laser pulses can be compressed…

Spin and charge-current dynamics after ultrafast spin-polarized excitation in a normal metal are studied theoretically using a wave-diffusion theory. It is shown analytically how this macroscopic approach correctly describes the ballistic…

材料科学 · 物理学 2011-11-22 Steffen Kaltenborn , Yao-Hui Zhu , Hans Christian Schneider

We study the spatiotemporal dynamics of ultrafast electron spin transport across nanometer-thick copper layers using broadband terahertz spectroscopy. Our analysis of temporal delays, broadening and attenuation of the spin-current pulse…

Ultrafast demagnetization of magnetic layers pumped by a femtosecond laser pulse is accompanied by a nonthermal spin-polarized current of hot electrons. These spin currents are studied here theoretically in a spin valve with noncollinear…

介观与纳米尺度物理 · 物理学 2018-02-26 Pavel Baláž , Martin Žonda , Karel Carva , Pablo Maldonado , Peter M. Oppeneer

Ultrashort electron pulses are crucial for time-resolved electron diffraction and microscopy of fundamental light-matter interaction. In this work, we study experimentally and theoretically the generation and characterization of attosecond…

光学 · 物理学 2018-03-21 Yuya Morimoto , Peter Baum

Efficient and fast manipulation of antiferromagnets has to date remained a challenging task, hindering their application in spintronic devices. For ultrafast operation of such devices, it is highly desirable to be able to control the…

材料科学 · 物理学 2023-05-31 Markus Weißenhofer , Francesco Foggetti , Ulrich Nowak , Peter M. Oppeneer

Employing electron spin instead of charge to develop spintronic devices holds the merits of low-power consumption in information technologies. Meanwhile, the demand for increasing speed in spintronics beyond current CMOS technology has…

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