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A quantum-mechanical model to calculate the electron energy-loss spectra (EELS) for the system of a closely located metallic nanoshell and a molecule has been developed. At the resonance between the molecular excitation and plasmon modes in…

原子物理 · 物理学 2014-10-07 I. Yu. Goliney , Ye. V. Onykienko

Progress in electron-beam spectroscopies has recently enabled the study of optical excitations with combined space, energy and time resolution in the nanometer, millielectronvolt and femtosecond domain, thus providing unique access into…

光学 · 物理学 2019-11-13 Albert Polman , Mathieu Kociak , F. Javier García de Abajo

Low-loss electron energy loss spectroscopy (EELS) has emerged as a technique of choice for exploring the localization of plasmonic phenomena at the nanometer level, necessitating analysis of physical behaviors from 3D spectral data sets.…

Electron energy loss spectroscopy is consolidating as a powerful tool to explore electronic (as well as vibrational) excitations of matter, including molecules. Performed in a scanning transmission electron microscope, this technique is…

化学物理 · 物理学 2021-03-05 Ciro A. Guido , Enzo Rotunno , Matteo Zanfrognini , Stefano Corni , Vincenzo Grillo

Electron energy-loss spectroscopy (EELS) performed in transmission electron microscopes is shown to directly render the photonic local density of states (LDOS) with unprecedented spatial resolution, currently below the nanometer. Two…

材料科学 · 物理学 2012-11-13 F. J. Garcia de Abajo , M. Kociak

Electron energy loss spectroscopy (EELS) has been established as a powerful analytical technique for investigating the oxidation state, band structure, and dielectric properties of materials with exceptional spatial resolution. Inspired by…

Fine structure analysis of core electron excitation spectra is a cornerstone characterization technique across the physical sciences. Spectra are most commonly measured with synchrotron radiation and X-ray spot sizes on the {\mu}m to mm…

Free electron beams such as those employed in electron microscopes have evolved into powerful tools to investigate photonic nanostructures with an unrivaled combination of spatial and spectral precision through the analysis of electron…

量子物理 · 物理学 2021-04-22 F. Javier García de Abajo , Valerio Di Giulio

Inelastic scattering of electrons incident on a solid surface is determined by the two properties: (i) electronic response of the target system and (ii) the detailed quantum-mechanical motion of the projectile electron inside and in the…

材料科学 · 物理学 2016-01-06 V. U. Nazarov , V. M. Silkin , E. E. Krasovskii

In a recently developed methodology termed photon induced near-field electron microscopy (PINEM), the inelastic scattering of electrons off illuminated nanostructures provides direct experimental access to the structure of optical…

介观与纳米尺度物理 · 物理学 2024-05-21 Niklas Müller , Gerrit Vosse , Ferdinand Evers , Sascha Schäfer

Circular dichroism spectroscopy is an essential technique for understanding molecular structure and magnetic materials, but spatial resolution is limited by the wavelength of light, and sensitivity sufficient for single-molecule…

Strong nanoscale light-matter interaction is often accompanied by ultra-confined photonic modes and large momentum polaritons existing far beyond the light cone. A direct probe of such phenomena is difficult due to the momentum mismatch of…

光学 · 物理学 2017-04-10 Prashant Shekhar , Marek Malac , Vaibhav Gaind , Neda Dalili , Al Meldrum , Zubin Jacob

Nanoscale materials usually can trap light and strongly interact with it leading to many photonic device applications. The light-matter interactions are commonly probed by optical spectroscopy, which, however, have some limitations such as…

介观与纳米尺度物理 · 物理学 2022-08-24 Jinlong Du , Jin-hui Chen , Yuehui Li , Ruochen Shi , Mei Wu , Yun-Feng Xiao , Peng Gao

In the last decades, the blossoming of experimental breakthroughs in the domain of electron energy loss spectroscopy (EELS) has triggered a variety of theoretical developments. Those have to deal with completely different situations, from…

介观与纳米尺度物理 · 物理学 2021-02-10 Hugo Lourenço-Martins , Axel Lubk , Mathieu Kociak

We theoretically demonstrate the ability of electron beams to probe the nonlinear photonic response with nanometer spatial resolution, well beyond the capabilities of existing optical techniques. Although the interaction of electron beams…

介观与纳米尺度物理 · 物理学 2020-12-30 Andrea Konečná , Valerio Di Giulio , Vahagn Mkhitaryan , Claus Ropers , F. Javier García de Abajo

The inelastic scattering of electrons is one route to study the vibrational and electronic properties of materials. Such experiments, also called electron energy-loss spectroscopy, are particularly useful for the investigation of the…

材料科学 · 物理学 2014-06-24 Friedrich Roth , Andreas König , Jörg Fink , Bernd Büchner , Martin Knupfer

Electron spectroscopy implemented in electron microscopes provides high spatial resolution, down to the atomic scale, of the chemical, electronic, vibrational and optical properties of materials. In this review, we will describe how…

材料科学 · 物理学 2025-11-11 Luiz H. G. Tizei , Yves Auad , Florian Castioni , Mathieu Kociak

We introduce a special kind of nonreciprocal electromagnetic response which gives rise to backscattering suppression in the bulk, a long-sought feature in topological photonics, as well as nonreciprocal lensing - an effect when the same…

光学 · 物理学 2026-02-11 Dmitry Vagin , Maxim A. Gorlach

Interactions between photons and electrons are ubiquitous in astrophysics. Photons can be down scattered (Compton scattering) or up scattered (inverse Compton scattering) by moving electrons. Inverse Compton scattering, in particular, is an…

高能天体物理现象 · 物理学 2023-04-05 Anderson C. M. Lai , Kenny C. Y. Ng

Swift electrons passing near or through metallic structures have proven to be an excellent tool for studying plasmons and other types of confined optical modes involving collective charge oscillations in the materials hybridized with…

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