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High-harmonic generation (HHG) spectrum from a LiH molecule induced by an intense laser pulse is computed and analyzed with potential energy surfaces for electron motion (ePES) constructed from a model of localized electron wave packets…

化学物理 · 物理学 2020-03-18 Koji Ando

We explore the roles of electronic band structure and Coulomb interactions in solid-state HHG by studying the optical response of linear atomic chains and carbon nanotubes to intense ultrashort pulses. Specifically, we simulate electron…

介观与纳米尺度物理 · 物理学 2020-03-18 Sandra de Vega , Joel D. Cox , Fernando Sols , F. Javier García de Abajo

An interesting property of high harmonic generation in solids is its laser polarization dependent nature which in turn provides information about the crystal and band structure of the generation medium. Here we report on the linear…

The spectra produced by high-harmonic generation (HHG) typically exhibit well-defined peaks at odd integers times the laser frequency. However, in recent investigations of HHG from correlated materials, spectra exhibit signals at noninteger…

原子物理 · 物理学 2024-06-05 Christian Saugbjerg Lange , Thomas Hansen , Lars Bojer Madsen

The strong ellipticity dependence of high-harmonic generation in gases enables numerous experimental techniques that are nowadays routinely used, for instance, to create isolated attosecond pulses. Extending such techniques to high-harmonic…

High-order harmonic generation (HHG) results from strong-field laser matter interaction and it is one of the main processes that are used to extract electron structural and dynamical information about the atomic or molecular targets with…

In this work we numerically study a self-guiding process in which ionization plays a dominant role and analyze its effect on high-order harmonic generation (HHG) in gases. Although this type of self-guiding --- termed as plasma-core induced…

We study high-order harmonic generation (HHG) from aligned molecules in strong elliptically polarized laser fields numerically and analytically. Our simulations show that the spectra and polarization of HHG depend strongly on the molecular…

原子物理 · 物理学 2021-05-19 F. J. Sun , C. Chen , W. Y. Li , X. Liu , W. Li , Y. J. Chen

Anomalous high-harmonic generation (HHG) arises in certain solids when irradiated by an intense laser field, as the result of a nonlinear perpendicular current akin to a Hall current. Here, we theoretically characterize the anomalous HHG…

光学 · 物理学 2023-05-03 Lun Yue , Mette B. Gaarde

We theoretically investigate correlated electron dynamics in high-harmonic generation (HHG), using all-electron \emph{ab initio} simulations for three-dimensional real alkali-metal atoms. The resulting harmonic spectra exhibit a plateau…

原子物理 · 物理学 2019-04-10 Yang Li , Takeshi Sato , Kenichi L. Ishikawa

We theoretically study multielectron effects in high-harmonic generation (HHG), using all-electron first-principles simulations for a one-dimensional (1D) model atom. In addition to usual plateau and cutoff (from a cation in the present…

原子物理 · 物理学 2017-05-24 Iliya Tikhomirov , Takeshi Sato , Kenichi L. Ishikawa

We employ the two-band density-matrix equations and time-dependent density functional theory to calculate high-order harmonic generation (HOHG) in graphene under a femtosecond laser irradiation. Our investigation uncovers a striking…

原子物理 · 物理学 2023-07-25 Fulong Dong , Qinzhi Xia , Jie Liu

A theory for laser-driven electron dynamics and high-harmonic generation in bulk solids with two lattice sites per unit cell of arbitrary dimension is formulated. In tight-binding approximation, such solids can be described by $2\times 2$…

介观与纳米尺度物理 · 物理学 2024-03-12 Daniel Moos , Hannah Jürß , Dieter Bauer

We investigate electron correlation effects in internuclear-distance-dependent enhanced ionization of $\mathrm{H}_2$, $\mathrm{LiH}$, and $\mathrm{HF}$ molecules by intense near-infrared laser pulses using a 3D description of the systems…

原子物理 · 物理学 2019-02-27 Siddhartha Chattopadhyay , Lars Bojer Madsen

We present a comprehensive theoretical investigation of high-order harmonic generation in H$_2^+$ molecular ions within a quantum optical framework. Our study focuses on characterizing various quantum optical and quantum information…

The generation of high harmonics is a strongly nonlinear effect that allows to probe properties of the target and to study electron dynamics in matter. It has been investigated in many different kinds of targets, including molecular gases,…

量子物理 · 物理学 2026-05-06 Lina Bielke , Samuel Schöpa , Falk-Erik Wiechmann , Franziska Fennel , Dieter Bauer

We present single-molecule and macroscopic calculations showing that laser-induced Stark shifts contribute significantly to the phase of high-order harmonics from polar molecules. This is important for orbital tomography, where phases of…

量子物理 · 物理学 2015-06-05 Adam Etches , Mette B. Gaarde , Lars Bojer Madsen

We find that a donor-doped band-gap material can enhance the overall high-order harmonic generation (HHG) efficiency by several orders of magnitude, compared with undoped and acceptor-doped materials. This significant enhancement, predicted…

光学 · 物理学 2019-01-30 Chuan Yu , Kenneth K. Hansen , Lars Bojer Madsen

We numerically study models of $\mathrm{H}_2$ and $\mathrm{LiH}$ molecules, aligned collinearly with the linear polarization of the external field, to elucidate the possible role of correlation in the enhanced-ionization phenomena.…

原子物理 · 物理学 2016-01-06 S. Chattopadhyay , S. Bauch , L. B. Madsen

High harmonic generation (HHG) is a striking phenomenon, which reflects the ultrafast dynamics of electrons. Recently, it has been demonstrated that HHG can be used to reconstruct not only the energy band structure but also the geometric…

介观与纳米尺度物理 · 物理学 2024-09-10 Atsushi Ono , Shun Okumura , Shohei Imai , Yutaka Akagi