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We study the crystallization of a colloidal model system in presence of secondary nanoparticles acting as impurities. Using confocal microscopy, we show that the nanoparticles segregate in the grain boundaries of the colloidal polycrystal.…

软凝聚态物质 · 物理学 2012-05-25 Neda Ghofraniha , Elisa Tamborini , Julian Oberdisse , Luca Cipelletti , Laurence Ramos

NPs are ultrafine-grain crystal or amorphous substances which are as small as 100nm. They have unique physical, chemical and mechanical properties, which are very different from those of large scale materials. This uniqueness is attributed…

材料科学 · 物理学 2018-10-19 A Titlov , G Krushenko , C Reshetnikova , K Borodianskiy

At very fine grain sizes, grain boundary segregation can deviate from conventional behavior due to triple junction effects. While this issue has been addressed in prior work for substitutional alloys, here we develop a framework that…

材料科学 · 物理学 2024-11-28 Nutth Tuchinda , Malik Wagih , Christopher A. Schuh

We report on the structural properties of mixed aggregates made from rare-earth inorganic nanoparticles (radius 20 Angstroms) and polyelectrolyte-neutral block copolymers in aqueous solutions. Using scattering experiments and Monte Carlo…

软凝聚态物质 · 物理学 2021-09-27 K. Yokota , M. Morvan , J. -F. Berret , J. Oberdisse

At the nanometric scale, the synthesis of a random alloy (i.e. without phase segregation, whatever the composition) by chemical synthesis remains a not easy task, even for simple binary type systems. In this context, a unique approach based…

In this work, we discuss the quantum mechanics of many-body systems i.e. hybrid microgel consisting of negatively charged anionic microgels possessing thick sheath of water molecules solvating its protruding anionic moieties and…

综合物理 · 物理学 2017-06-06 Mirza Wasif Baig , Muhammad Siddiq

Grain size engineering, particularly reducing grain size into the nanocrystalline regime, offers a promising pathway to further improve the strength-to-weight ratio of Al alloys. Unfortunately, the fabrication of nanocrystalline metals…

材料科学 · 物理学 2021-10-07 Tianjiao Lei , Jungho Shin , Daniel S. Gianola , Timothy J. Rupert

Grain boundaries are dominant imperfections in nanocrystalline materials that form a complex 3-dimensional (3D) network. Solute segregation to grain boundaries is strongly coupled to the grain boundary character, which governs the stability…

The incorporation of impurities during the chemical synthesis of nanomaterials is usually uncontrolled and rarely reported because of the formidable challenge that constitutes measuring trace amounts of often light elements with sub…

Incorporating nanomaterials into hydrogels allows for the creation of versatile materials with properties that can be precisely tailored by manipulating their nanoscale structures, leading to a wide range of bulk properties. Investigating…

软凝聚态物质 · 物理学 2024-11-13 Irfan Khan , Snigdharani Panda , Sugam Kumar , Sunita Srivastava

A number of metal-based nanopowders such kinds as Fe, Co, Fe/Co alloy, Fe/C, Fe/organic shell were successfully produced by aerosol synthesis method. The mechanism of nanoparticles formation and the influence of experimental parameters on…

材料科学 · 物理学 2007-08-13 E. S. Vasilieva , O. V. Tolochko , V. E. Yudin , D. Kim , D. -W. Lee

The discovery of superfluid $^{3}$He in high porosity silica aerogels, and subsequent experimental and theoretical work, have led to a better general understanding of quasiparticle scattering from impurities in unconventional pairing…

超导电性 · 物理学 2009-04-24 W. P. Halperin , H. Choi , J. P. Davis , J. Pollanen

Tailoring the nanoscale distribution of chemical species at grain boundaries is a powerful method to dramatically influence the properties of polycrystalline materials. However, classical approaches to the problem have tacitly assumed that…

材料科学 · 物理学 2024-11-11 Malik Wagih , Yannick Naunheim , Tianjiao Lei , Christopher A. Schuh

Tuning of the electronic properties of pre-synthesized colloidal semiconductor nanocrystals (NCs) by doping plays a key role in the prospect of implementing them in printed electronics devices such as transistors, and photodetectors. While…

材料科学 · 物理学 2021-05-25 Yorai Amit , Yuanyuan Li , Anatoly I. Frenkel , Uri Banin

Segregated impurities at grain boundaries can dramatically change the mechanical behavior of metals, while the mechanism is still obscure in some cases. Here, we suggest an unified approach to investigate segregation and its effects on the…

材料科学 · 物理学 2017-12-20 Yunguo Li , Pavel Korzhavyi , Rolf Sandström , Christina Lilja

The electronic properties of low-dimensional materials can be engineered by doping, but in the case of graphene nanoribbons (GNR) the proximity of two symmetry-breaking edges introduces an additional dependence on the location of an…

介观与纳米尺度物理 · 物理学 2010-10-05 S. R. Power , V. M. de Menezes , S. B. Fagan , M. S. Ferreira

We investigate by scattering techniques the structure of water-based soft composite materials comprising a crystal made of Pluronic block-copolymer micelles arranged in a face-centered cubic lattice and a small amount (at most 2% by volume)…

软凝聚态物质 · 物理学 2012-06-07 Elisa Tamborini , Neda Ghofraniha , Julian Oberdisse , Luca Cipelletti , Laurence Ramos

Deciphering the three-dimensional atomic structure of solid-solid interfaces in core-shell nanomaterials is the key to understand their remarkable catalytical, optical and electronic properties. Here, we probe the three-dimensional atomic…

材料科学 · 物理学 2023-06-21 Zezhou Li , Zhiheng Xie , Yao Zhang , Xilong Mu , Hai-jing Yin , Ya-wen Zhang , Colin Ophus , Jihan Zhou

Bio-conjugated nanomaterials play a promising role in the development of novel supramolecular structures, molecular machines, and biosensing devices. In this study, lipid-conjugated gold nanoparticles were synthesized and allowed to form a…

材料科学 · 物理学 2012-07-24 Subhasish Chatterjee , Markrete Krikorian , Harry D. Gafney , Bonnie Gersten

Here, we propose an easy and robust strategy for the versatile preparation of hybrid plasmonic nanopores by means of controlled deposition of single flakes of MoS2 directly on top of metallic holes. The device is realized on silicon nitride…

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