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Uniformity in the excitonic spectrum is a key requirement for accessing intrinsic excitonic physics in two-dimensional semiconductors; however, in transition-metal dichalcogenide (TMD) monolayers supported on substrates, exciton energies…

Monolayer transition metal dichalcogenides (TMDs) host deeply bound excitons interacting with itinerant electrons, and as such they represent an exciting new quantum many-body Bose-Fermi mixture. Here, we demonstrate that electrons…

超导电性 · 物理学 2022-10-24 Aleksi Julku , Jami J. Kinnunen , Arturo Camacho-Guardian , Georg M. Bruun

Optical properties of transition metal dichalcogenides monolayers are controlled by the Wannier-Mott excitons forming a series of $1s$, $2s$, $2p$,... hydrogen-like states. We develop the theory of the excited excitonic states energy…

介观与纳米尺度物理 · 物理学 2017-02-01 M. M. Glazov , L. E. Golub , G. Wang , X. Marie , T. Amand , B. Urbaszek

The two-dimensional transition-metal dichalcogenides (2D TMDCs) are an intriguing platform for studying light-matter interactions because they combine the electronic properties of conventional semiconductors with the optical resonances…

介观与纳米尺度物理 · 物理学 2022-05-02 Aaron H. Rose , Taylor J. Aubry , Hanyu Zhang , Jao van de Lagemaat

The dynamics of exciton formation in transition metal dichalcogenides is difficult to measure experimentally, since many momentum-indirect exciton states are not accessible to optical interband spectroscopy. Here, we combine a tuneable…

Excitons, Coulomb-bound electron-hole pairs, play a fundamental role in both optical excitation and correlated phenomena in solids. When an exciton interacts with other quasi-particles, few- and many-body excited states, such as trions,…

Transition-metal dichalcogenide heterostructures exhibit moir\'e patterns that spatially modulate the electronic structure across the material's plane. For certain material pairs, this modulation acts as a potential landscape with deep,…

介观与纳米尺度物理 · 物理学 2021-03-12 David A. Ruiz-Tijerina , Isaac Soltero , Francisco Mireles

Exciton spectroscopy serves as a sensitive probe of electronic states in two-dimensional semiconductors. A prominent feature in optical spectra is the trion peak arising from the binding of a charge carrier to an exciton. The splitting…

介观与纳米尺度物理 · 物理学 2025-07-23 Arthur Christianen , Atac Imamoglu

Novel excitonic phenomena emerging in transition metal dichalcogenide (TMDC) heterostructures belong to the most exciting topics in contemporary physics of van der Waals materials. Interlayer excitons (IXs) stand out among those due to…

We determine the zero temeperature phase diagram of excitons in the symmetric transition-metal dichalcogenide tri-layer heterosctructure WSe2/MoSe2/WSe2. First principle calculations reveal two distinct types of interlayer excitonic states,…

We propose a continuum model for the theoretical study of hybridized moir\'e excitons in transition metal dichalcogenides heterobilayers, and we use a variational method to solve the exciton wavefunction and calculate the optical absorption…

介观与纳米尺度物理 · 物理学 2023-10-23 Yao-Wen Chang

In order to fully exploit the potential of transition metal dichalcogenide monolayers (TMD-MLs), the well-controlled creation of atomically sharp lateral heterojunctions within these materials is highly desirable. A promising approach to…

介观与纳米尺度物理 · 物理学 2017-10-11 Sven Borghardt , Jhih-Sian Tu , Florian Winkler , Jürgen Schubert , Willi Zander , Kristján Lesson , Beata E. Kardynał

In monolayer transition metal dichalcogenide semiconductors, valley coherence degrades rapidly due to a combination of fast scattering and inter-valley exchange interaction. This leads to a sub-picosecond valley coherence time, making…

介观与纳米尺度物理 · 物理学 2023-07-21 Garima Gupta , Kenji Watanabe , Takashi Taniguchi , Kausik Majumdar

Excitons in thin layers of semiconducting transition metal dichalcogenides are highly subject to the strongly modified Coulomb electron-hole interaction in these materials. Therefore, they do not follow the model system of a two-dimensional…

Van der Waals (vdW) heterostructures have attracted great interest because of their rich material combinations.The discovery of two-dimensional magnets has provided a new platform for magnetic vdW heterointerfaces; however, research on…

We present a many-body formalism for the simulation of time-resolved nonlinear spectroscopy and apply it to study the coherent interaction between excitons and trions in doped transition-metal dichalcogenides. Although the formalism can be…

材料科学 · 物理学 2019-09-11 Roel Tempelaar , Timothy C. Berkelbach

Monolayers (MLs) of MoS2 and WSe2 are 2D semiconductors with strong, direct optical transitions that are governed by tightly Coulomb bound eletron-hole pairs (excitons). The optoelectronic properties of these transition metal…

材料科学 · 物理学 2015-03-06 G. Wang , X. Marie , I. Gerber , T. Amand , D. Lagarde , L. Bouet , M. Vidal , A. Balocchi , B. Urbaszek

We study in-plane lateral heterostructures of commensurate transition-metal dichalcogenides, such as MoS$_{2}$-WS$_{2}$ and MoSe$_{2}$-WSe$_{2}$, and find interfacial and edge states that are highly localized to these regions of the…

介观与纳米尺度物理 · 物理学 2019-01-04 Oscar Ávalos-Ovando , Diego Mastrogiuseppe , Sergio E. Ulloa

Moir\'e patterns with angular mismatch in van der Waals heterostructures composed of atomically thin semiconducting materials are a fascinating platform to engineer the optically generated excitonic properties towards novel quantum…

介观与纳米尺度物理 · 物理学 2020-12-17 Keisuke Shinokita , Yuhei Miyauchi , Kenji Watanabe , Takashi Taniguchi , Kazunari Matsuda

Excitons with binding energies of a few hundreds of meV control the optical properties of transition metal dichalcogenide monolayers. Knowledge of the fine structure of these excitons is therefore essential to understand the optoelectronic…