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We explore the total cross section of ground state polar molecules in an electric field at various energies, focusing on RbCs and RbK. An external electric field polarizes the molecules and induces strong dipolar interactions leading to…

原子物理 · 物理学 2009-11-13 Christopher Ticknor

Nonlinear Thomson scattering of an electron motion in a combining field constituted by an elliptically polarized laser and a background magnetic field is investigated. The dependence of the electron trajectories, the fundamental frequency,…

光学 · 物理学 2022-06-28 Hong Xiao , Cui-Wen Zhang , Hai-Bo Sang , Bai-Song Xie

The photoelectric effect describes the ejection of an electron upon absorption of one or several photons. The kinetic energy of this electron is determined by the photon energy reduced by the binding energy of the electron and, if strong…

Molecular orientation is a fundamental requisite in the study of stereodirected dynamics of collisional and photoinitiated processes. In this last decade, variable hexapolar electric filters have been developed and employed for the…

We demonstrate the breakdown of molecular-frame dynamics induced by the uncoupling of molecular rotation from electronic motion in molecular Rydberg states. We observe this non-Born-Oppenheimer regime in the time domain through…

原子与分子团簇 · 物理学 2017-07-05 Lucas J. Zipp , Adi Natan , Philip H. Bucksbaum

Biological molecules are characterized by an intrinsic asymmetry known as homochirality. The result is optical activity of biological materials and circular polarization in the light scattered by microorganisms, cells of living organisms,…

地球与行星天体物理 · 物理学 2014-06-13 Lev Nagdimunov , Ludmilla Kolokolova , Daniel Mackowski

Using a model of particle acceleration and transport in solar flares, we investigate the height distribution of coronal electrons by focusing on the energy-dependent pitch-angle scattering. When pitch-angle scattering is not included, the…

太阳与恒星天体物理 · 物理学 2015-05-27 Takashi Minoshima , Satoshi Masuda , Yoshizumi Miyoshi , Kanya Kusano

Photoionization of randomly oriented chiral molecules with circularly polarized light leads to a strong forward/backward asymmetry in the photoelectron angular distribution. This chiroptical effect, referred to as Photoelectron Circular…

We investigate theoretically the photoelectron momentum distribution (PMD) of the ionized atoms irradiated by a linearly polarized intense laser, focusing on the holography interference patterns in PMD that carry important information of…

原子物理 · 物理学 2022-06-01 L. G. Liao , Q. Z. Xia , J. Cai , J. Liu

Metal-organic hybrid structures have been demonstrated a versatile platform to study primary aspects of light-matter interaction by means of emerging states comprising excitonic and plasmonic properties. Here we are studying the wave-vector…

A theoretical study is performed for the excitation of a single atom localized in the center of twisted light modes. Here we present the explicit dependence of excitation rates on critical parameters, such as the polarization of light, its…

原子物理 · 物理学 2020-07-29 S. A. -L. Schulz , A. A. Peshkov , R. A. Müller , R. Lange , N. Huntemann , Chr. Tamm , E. Peik , A. Surzhykov

It is demonstrated for the first time that in spite of well known big similarities between atomic ionization by photons and fast electrons, a qualitative difference exists in angular anisotropy parameters of electrons knocked out in these…

原子物理 · 物理学 2015-05-30 M. Ya. Amusia , L. V. Chernysheva , E. Z. Liverts

Photoelectron momentum distributions (PMDs) from atoms and molecules undergo qualitative changes as laser parameters are varied. We present a model to interpret the shape of the PMDs. The electron's motion is guided by a fictitious particle…

混沌动力学 · 物理学 2018-09-19 Jonathan Dubois , Simon Berman , Cristel Chandre , Turgay Uzer

We studied the photoelectron spectra generated by an intense few-cycle infrared laser pulse. By focusing on the angular distributions of the back rescattered high energy photoelectrons, we show that accurate differential elastic scattering…

原子物理 · 物理学 2008-04-04 T Morishita , A. T. Le , Z. Chen , C. D. Lin

We report the observation of macroscopic field-free orientation, i.e. more than 73 % of CO molecules pointing in the same direction. This is achieved through an all-optical scheme operating at high particle densities ($>10^{17}$cm$^{-3}$)…

化学物理 · 物理学 2014-07-09 P. M. Kraus , D. Baykusheva , H. J. Wörner

We investigate here the fast electron scattering upon endohedral atoms that present a fullerene CN staffed by an atom A, A@CN. We calculate the inelastic scattering cross-section expressing it via generalized oscillator strengths (GOS)…

原子与分子团簇 · 物理学 2012-03-06 M. Ya. Amusia , L. V. Chernysheva , E. Z. Liverts

A general expression for the double differential cross section of fluorescence radiation following photorecombination (PRF) of polarized electrons and polarized ions is derived by using usual atomic theory methods and is represented in the…

原子物理 · 物理学 2009-11-11 A. Kupliauskiene

Strong-field photoelectron momentum imaging of the prototypical biomolecule indole was disentangled in a combined experimental and computational approach. Experimentally, strong control over the molecules enabled the acquisition of…

原子物理 · 物理学 2021-02-03 Joss Wiese , Jolijn Onvlee , Sebastian Trippel , Jochen Küpper

The elastic scattering of twisted electrons by diatomic molecules is studied within the framework of the non-relativistic first Born approximation. In this process, the coherent interaction of incident electrons with two molecular centers…

原子物理 · 物理学 2018-10-17 A. V. Maiorova , S. Fritzsche , R. A. Mueller , A. Surzhykov

A survey of atomic binding energies used by general purpose Monte Carlo systems is reported. Various compilations of these parameters have been evaluated; their accuracy is estimated with respect to experimental data. Their effects on…