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The origin of insulating ferromagnetism in epitaxial LaCoO3 films under tensile strain remains elusive despite extensive research efforts have been devoted. Surprisingly, the spin state of its Co ions, the main parameter of its…

The electronic structure of epitaxial films on LaCoO3(LCO) has been studied within first principle electronic structure calculations. A spin state transition is found to take place as a function of lattice strain which freezes in the…

强关联电子 · 物理学 2009-01-05 Kapil Gupta , Priya Mahadevan

LaCoO3 thin films grown under epitaxial tensile strain exhibit a robust ferromagnetic insulating state that is absent in the bulk. Despite many studies, both experimental and computational, the microscopic origin of this phenomenon is not…

Epitaxial strain imposed in complex oxide thin films by heteroepitaxy is recognized as a powerful tool for identifying new properties and exploring the vast potential of materials performance. A particular example is LaCoO3, a zero spin,…

Single phase and strained LuMnO3 thin films are discovered to display co-existing ferromagnetic and antiferromagnetic orders. A large moment ferromagnetism (approx. 1 muB), which is absent in bulk samples, is shown to display a magnetic…

Epitaxial strain provides important pathways to control the magnetic and electronic states in transition metal oxides. However, the large strain is usually accompanied by a strong reduction of the oxygen vacancy formation energy, which…

Using spectroscopic ellipsometry, we studied the optical conductivity of LaCoO$_3$ with various degrees of strain. The optical response of the compressively strained \lco\ film is qualitatively similar to the one of the unstrained LaCoO$_3$…

强关联电子 · 物理学 2025-03-13 F. Abadizaman , M. Kiaba , A. Dubroka

It has been well established that both in bulk at ambient pressure and for films under modest strains, cubic SrCoO$_{3-\delta}$ ($\delta < 0.2$) is a ferromagnetic metal. Recent theoretical work, however, indicates that a magnetic phase…

材料科学 · 物理学 2015-06-23 S. J. Callori , S. Hu , J. Bertinshaw , Z. Yue , S. Danilkin , X. L. Wang , V. Nagarajan , F. Klose , J. Seidel , C. Ulrich

The intrinsic magnetic state (ferromagnetic or antiferromagnetic) of ultra-thin LaMnO$_3$ films on the mostly used SrTiO$_3$ substrate is a long-existing question under debate. Either strain effect or non-stoichiometry was argued to be…

材料科学 · 物理学 2017-12-19 Ming An , Yakui Weng , Huimin Zhang , Jun-Jie Zhang , Yang Zhang , Shuai Dong

Ferromagnetic insulators play a crucial role in the development of low-dissipation quantum magnetic devices for spintronics. Epitaxial LaCoO3 thin film is a prominent ferromagnetic insulator, in which the robust ferromagnetic ordering…

材料科学 · 物理学 2022-06-17 Dongwon Shin , Sangmoon Yoon , Sehwan Song , Sungkyun Park , Ho Nyung Lee , Woo Seok Choi

We report on the observation of a strain-induced insulator state in ferromagnetic La_0.7Sr_0.3CoO_3 films. Tensile strain above 1% is found to enhance the resistivity by several orders of magnitude. Reversible strain of 0.15% applied using…

强关联电子 · 物理学 2009-11-13 A. D. Rata , A. Herklotz , K. Nenkov , L. Schultz , K. Doerr

By combining genetic algorithm optimizations, first-principles calculations and the double-exchange model studies, we have unveiled that the exotic insulating ferromagnetism in LaMnO3 thin film originates from the previously unreported…

强关联电子 · 物理学 2015-05-20 Yusheng Hou , Hongjun Xiang , Xingao Gong

The enigma of the emergent ferromagnetic state in tensile-strained LaCoO3 thin films remains to be explored because of the lack of a well agreed explanation. The direct magnetic imaging technique using a low-temperature magnetic force…

We study ferromagnetic ordering and microscopic inhomogeneity in tensile strained LaCoO$_3$ using numerical simulations. We argue that both phenomena originate from effective superexchange interactions between atoms in the high-spin (HS)…

强关联电子 · 物理学 2020-06-03 Andrii Sotnikov , Kyo-Hoon Ahn , Jan Kuneš

Magnetism in lanthanum cobaltite (LCO, LaCoO$_3$) appears to be strongly dependent on strain, defects, and nanostructuring. LCO on strontium titanate (STO, SrTiO$_3$) is a ferromagnet with an interesting strain relaxation mechanism that…

We show that a ferromagnetic (FM) order in the orthorhombic CaRuO3, which is a non-magnetic and iso-structural analog of FM system SrRuO3, can be established and stabilized by the means of tensile epitaxial strain. Investigations on the…

材料科学 · 物理学 2013-01-15 Shivendra Tripathi , Rakesh Rana , Parul Pandey , R. S. Singh , D. S. Rana

TbMnO$_{3}$ films have been grown under compressive strain on (001)-oriented SrTiO$_{3}$ crystals. They have an orthorhombic structure and display the (001) orientation. With increasing thickness, the structure evolves from a more symmetric…

Epitaxial strain in transition-metal oxides can induce dramatic changes in electronic and magnetic properties. A recent study on the epitaxially strained SrCoO$_3$ thin films revealed persistent ferromagnetism even across a metal-insulator…

The epitaxial strain effects on the magnetic ground state of YTiO$_3$ films grown on LaAlO$_3$ substrates have been studied using the first-principles density-functional theory. With the in-plane compressive strain induced by LaAlO$_3$…

材料科学 · 物理学 2013-04-04 Xin Huang , Yankun Tang , Shuai Dong

The ferromagnetic properties of epitaxial La$_{0.5}$Sr$_{0.5}$CoO$_3$ thin films have been studied. The magnetic transition is affected by both strain and finite thickness. We have used a series of films of different thickness and on…

材料科学 · 物理学 2009-11-13 Changkun Xie , J. I. Budnick , B. O. Wells , J. C. Woicik
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