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In order to better understand the variation mechanism of ozone abundance in the middle atmosphere, the simultaneous monitoring of ozone and other minor molecular species, which are related to ozone depletion, is the most fundamental and…

Second-harmonic and sum-frequency mixing phenomena associated with 3D-localized photonic modes are studied in InP-based planar photonic crystal microcavities excited by short-pulse radiation near 1550 nm. Three-missing-hole microcavities…

We present results of meson and baryon spectroscopy using the Chirally Improved Dirac operator on lattices of size 16**3 x 32 with two mass-degenerate light sea quarks. Three ensembles with pion masses of 322(5), 470(4) and 525(7) MeV and…

高能物理 - 格点 · 物理学 2015-03-17 Georg P. Engel , C. B. Lang , Markus Limmer , Daniel Mohler , Andreas Schäfer

The results of a spectral survey of the region of massive star formation DR21OH in the 4-mm wavelength range are presented. Sixty-nine molecules and their isotopologues have been detected, ranging from simple diatomic or triatomic species…

星系天体物理 · 物理学 2024-01-31 S. V. Kalenskii , E. A. Mikheeva

Recently, quadrupole helix chirality and its domain structure was observed in resonant x-ray diffraction experiments on DyFe$_3$(BO$_3$)$_4$ using circularly polarized x rays [T. Usui et al., Nature Materials 13, 611 (2014)]. We show that…

High-precision tests of fundamental symmetries are looking for the parity- (P), time-reversal- (T) violating electric dipole moment of the electron (eEDM) as proof of physics beyond the Standard Model. Particularly, in polyatomic molecules,…

Pure rotational spectra of three polycyclic aromatic hydrocarbons - acenaphthene, acenaphthylene and fluorene - have been obtained by Fourier transform microwave spectroscopy of a molecular beam and subsequently by millimeter wave…

天体物理学 · 物理学 2015-06-24 S. Thorwirth , P. Theule , C. A. Gottlieb , M. C. McCarthy , P. Thaddeus

We demonstrate chirality-induced three-wave mixing in the microwave regime, using rotational transitions in cold gas-phase samples of 1,2-propanediol and 1,3-butanediol. We show that bulk three-wave mixing, which can only be realized in a…

化学物理 · 物理学 2015-06-16 David Patterson , John M. Doyle

Mid-infrared high-resolution spectroscopy has proven an invaluable tool for the study of the structure and dynamics of molecules in the gas phase. The advent of frequency combs advances the frontiers of precise molecular spectroscopy. Here…

光学 · 物理学 2019-02-28 Zaijun Chen , Theodor W. Hänsch , Nathalie Picqué

While powerful techniques exist to accurately account for anharmonicity in vibrational molecular spectroscopy, they are computationally very expensive and cannot be routinely employed for large species and/or at non- zero vibrational…

化学物理 · 物理学 2018-10-17 Giacomo Mulas , Cyril Falvo , Patrick Cassam-Chenaï , Christine Joblin

We present here the microwave surface impedance of a high purity crystal of $YBa_2Cu_3O_{6.99}$ measured at 5 frequencies between 1 and 75 GHz. This data set reveals the main features of the conductivity spectrum of the thermally excited…

超导电性 · 物理学 2009-10-31 A. Hosseini , R. Harris , Saeid Kamal , P. Dosanjh , J. Preston , Ruixing Liang , W. N. Hardy , D. A. Bonn

In order to study a molecular-cloud-scale chemical composition, we have conducted a mapping spectral line survey toward the Galactic molecular cloud W3(OH), which is one of the most active star forming regions in the Perseus arm, with the…

We present a study of the spectral properties like the energy spectrum, the eigenmodes and density of states of a classical finite system of two-dimensional (2D) charged particles which are confined by a quadratic potential. Using the…

凝聚态物理 · 物理学 2007-05-23 V. A. Schweigert , F. M. Peeters

Fine control of the chiral light-matter interaction at the nanoscale, by exploiting designed metamaterial architecture, represents a cutting-edge craft in the field of biosensing, quantum and classic nanophotonics. Recently, artificially…

The effect of pressure on the structural and vibrational properties of the layered molecular crystal 1,1-diamino-2,2-dinitroethelene (FOX-7) are explored by first principles calculations. We observe significant changes in the calculated…

材料科学 · 物理学 2014-02-18 S. Appalakondaiah , G. Vaitheeswaran , S. Lebègue

By applying a circularly polarized and slightly blue-detuned microwave field with respect to the first excited rotational state of a dipolar molecule, one can engineer a long-range, shallow potential well in the entrance channel of the two…

量子气体 · 物理学 2018-10-24 Lucas Lassablière , Goulven Quéméner

The mid-infrared spectra of large PAHs ranging from C54H18 to C130H28 are determined computationally using Density Functional Theory. Trends in the band positions and intensities as a function of PAH size, charge and geometry are discussed.…

天体物理学 · 物理学 2012-08-27 Charles W. Bauschlicher, , Els Peeters , Louis J. Allamandola

The lack of coherent room-temperature sources in the whole terahertz spectral window (0.3-10 THz) has significantly hampered the growth of scientific and technological applications in this range. Among them, high-precision frequency…

Tunneling spectroscopy measurements have been carried out on a single molecule device formed by two Pd nanocrystals (dia, $\sim$5 nm) electronically coupled by a conducting molecule, dimercaptodiphenylacetylene. The I-V data, obtained by…

材料科学 · 物理学 2007-05-23 Ved Varun Agrawal , Reji Thomas , G. U. Kulkarni , C. N. R. Rao

Multilayer stacks of twisted optical metasurfaces are considered as a prospective platform for chiral nanophotonic devices. Such structures are primarily used for the realization of circularly polarized light sources, artificial optical…

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